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In high magnetic fields, the exciton absorption spectrum of a semiconducting single-walled carbon nanotube splits as a result of Aharonov-Bohm magnetic flux. A magnetic field of 370 T, generated by the electro-magnetic flux compression…

Materials Science · Physics 2015-05-26 D. Nakamura , T. Sasaki , W. Zhou , H. Liu , H. Kataura , S. Takeyama

We report high field magneto-optical study on the first and second sub-band transitions of single-chirality single-walled carbon nanotubes. The ordering and relative energy splitting between bright and dark excitonic states were found to be…

Mesoscale and Nanoscale Physics · Physics 2015-06-15 Weihang Zhou , Tatsuya Sasaki , Daisuke Nakamura , Huaping Liu , Hiromichi Kataura , Shojiro Takeyama

We report the direct observation of the spin-singlet dark excitonic state in individual single-walled carbon nanotubes through low-temperature micro-photoluminescence spectroscopy in magnetic fields. A magnetic field up to 5 T, applied…

Mesoscale and Nanoscale Physics · Physics 2008-08-22 A. Srivastava , H. Htoon , V. I. Klimov , J. Kono

The Ajiki-Ando (A-A) splitting of single-walled carbon nanotubes(SWNT) originating from the Aharanov-Bohm effect was observed in chiral specific SWNTs by the magneto-absorption measurements conducted at magnetic fields of up to 78 T. The…

Mesoscale and Nanoscale Physics · Physics 2015-05-28 Shojiro Takeyama , Hirofumi Suzuki , Hiroyuki Yokoi , Yoichi Murakami , Shigeo Maruyama

Often a modification of microscopic symmetry in a system can result in a dramatic change in its macroscopic properties. Here we report that symmetry breaking by a tube-threading magnetic field can drastically increase the photoluminescence…

Mesoscale and Nanoscale Physics · Physics 2015-06-25 J. Shaver , J. Kono , O. Portugall , V. Krstic , G. L. J. A. Rikken , Y. Miyauchi , S. Maruyama , V. Perebeinos

The optical absorption spectrum of the carbon (4,2) nanotube is computed using an ab-initio many-body approach which takes into account excitonic effects. We develop a new method involving a local basis set which is symmetric with respect…

Materials Science · Physics 2009-11-10 Eric Chang , Giovanni Bussi , Alice Ruini , Elisa Molinari

It is strong Coulomb effects in carbon nanotubes that lead to formation of the so-called "bright" and "dark" (forbidden one-photon optical transition) exciton states, and dramatically decrease the efficiency of one-photon light emission via…

Quantum Physics · Physics 2009-02-09 Nikolai G. Kalugin , Yuri V. Rostovtsev

We investigate the lowest many-body excited states in carbon nanotubes by means of ab initio calculations. On the basis of these calculations and an additional theoretical analysis of the excitons, we demonstrate that the splitting between…

Materials Science · Physics 2007-05-23 Eric Chang , Deborah Prezzi , Alice Ruini , Elisa Molinari

We find that the optical properties of carbon nanotubes reflect remarkably strong effects of exciton-phonon coupling. Tight-binding calculations show that a significant fraction of the spectral weight of the absorption peak is transferred…

Materials Science · Physics 2009-11-10 Vasili Perebeinos , J. Tersoff , Phaedon Avouris

We study theoretically the interactions of excitonic states with surface electromagnetic modes of small-diameter (~1 nm) semiconducting single-walled carbon nanotubes. We show that these interactions can result in strong…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 I. V. Bondarev , K. Tatur , L. M. Woods

One- and two-photon luminescence excitation spectroscopy showed a series of distinct excitonic states in single-walled carbon nanotubes. The energy splitting between one- and two-photon-active exciton states of different wavefunction…

Materials Science · Physics 2007-05-23 J. Maultzsch , R. Pomraenke , S. Reich , E. Chang , D. Prezzi , A. Ruini , E. Molinari , M. S. Strano , C. Thomsen , C. Lienau

Recent measurements in single-walled carbon nanotubes show that, on resonance, all nanotubes display the same peak optical conductivity of approximately 8 $e^2/h$, independent of radius or chirality [Joh \emph{et al.}, \emph{Nature…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 Jesse M. Kinder , Jiwoong Park , Garnet Kin-Lic Chan

We present direct experimental observation of exciton-phonon bound states in the photoluminescence excitation spectra of isolated single walled carbon nanotubes in aqueous suspension. The photoluminescence excitation spectra from several…

Materials Science · Physics 2009-11-11 Flavio Plentz , Henrique B. Ribeiro , Ado Jorio , Marcos A. Pimenta , Michael S. Strano

We show that the optical absorption spectra of boron nitride (BN) nanotubes are dominated by strongly bound excitons. Our first-principles calculations indicate that the binding energy for the first and dominant excitonic peak depends…

Materials Science · Physics 2013-08-07 Ludger Wirtz , Andrea Marini , Angel Rubio

Single-walled carbon nanotubes are strongly correlated systems with large Coulomb repulsion between two electrons occupying the same $p_z$ orbital. Within a molecular Hamiltonian appropriate for correlated $\pi$-electron systems, we show…

Materials Science · Physics 2009-02-15 Zhendong Wang , Demetra Psiachos , Roberto F. Badilla , Sumit Mazumdar

We have investigated excitons in highly-aligned single-walled carbon nanotubes (SWCNTs) through optical spectroscopy at low temperature (1.5 K) and high magnetic fields ($\textbf{\textit{B}}$) up to 55 T. SWCNT/polyacrylic acid films were…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 J. Shaver , S. A. Crooker , J. A. Fagan , E. K. Hobbie , N. Ubrig , O. Portugall , V. Perebeinos , Ph. Avouris , J. Kono

The gap oscillations caused by a magnetic flux penetrating a carbon nanotube represent one of the most spectacular observation of the Aharonov-Bohm effect at the nano--scale. Our understanding of this effect is, however, based on the…

Mesoscale and Nanoscale Physics · Physics 2012-06-04 Davide Sangalli , Andrea Marini

We report a femtosecond mid-infrared study of the broadband low-energy response of individually separated (6,5) and (7,5) single-walled carbon nanotubes. Strong photoinduced absorption is observed around 200 meV, whose transition energy,…

Mesoscale and Nanoscale Physics · Physics 2010-07-16 Jigang Wang , Matt W. Graham , Yingzhong Ma , Graham R. Fleming , Robert A. Kaindl

We show theoretically that an undoped carbon nanotube might be an excitonic insulator---the long-sought phase of matter proposed by Keldysh, Kohn and others fifty years ago. We predict that the condensation of triplet excitons, driven by…

Strongly Correlated Electrons · Physics 2014-11-12 Massimo Rontani

An analytical expression is obtained for the biexciton binding energy as a function of the inter-exciton distance and binding energy of constituent quasi-one-dimensional excitons in carbon nanotubes. This allows one to trace biexciton…

Mesoscale and Nanoscale Physics · Physics 2015-05-20 I. V. Bondarev
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