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Using in-field single crystal neutron diffraction we have determined the magnetic structure of TbMnO3 in the high field P||a phase. We unambiguously establish that the ferroelectric polarization arises from a cycloidal Mn spins ordering,…

Strongly Correlated Electrons · Physics 2010-07-20 N. Aliouane , K. Schmalzl , D. Senff , A. Maljuk , K. Prokes , M. Braden , D. N. Argyriou

We report on the linear optical properties of the chiral magnet Cu2OSeO3, specifically associated with the absence of inversion symmetry, the chiral crystallographic structure, and magnetic order. Through spectroscopic ellipsometry, we…

Magnetoelectric coupling in insulating multiferroic materials is invaluable for both fundamental research and multifunctional device applications. However, material realization remains a significant challenge. We employ first-principles…

Materials Science · Physics 2025-07-08 Xilong Xu , Li Yang

We uncover a new pathway towards multiferroicity, showing how magnetism can drive ferroelectricity without relying on inversion symmetry breaking of the magnetic ordering. Our free-energy analysis demonstrates that any commensurate…

Materials Science · Physics 2009-11-11 Joseph J. Betouras , Gianluca Giovannetti , Jeroen van den Brink

We have synthesized single crystalline sample of Mn$_2$V$_2$O$_7$ using floating zone technique and investigated the ground state using magnetic susceptibility, heat capacity and neutron diffraction. Our magnetic susceptibility and heat…

Strongly Correlated Electrons · Physics 2019-11-27 J. Sannigrahi , D. T. Adroja , R. Perry , M. J. Gutmann , V. Petricek , D. Khalyavin

We have investigated the effects of substituting In for Mn on the antiferromagnetic phase transition in YMnO3 using magnetic, dielectric, and specific heat measurements. We prepared a set of isostructural phase pure hexagonal…

Materials Science · Physics 2015-05-14 A. Dixit , Andrew E. Smith , M. A. Subramanian , G. Lawes

The magnetic phase diagram in a single crystal of copper metaborate CuB_2O_4 in a magnetic field parallel to a tetragonal axis $c$ has been investigated. From the resonant, magnetic and magnetostrictive data the phase diagram of CuB_2O_4 on…

We have revisited the magnetic structure of manganese phosphorus trisulfide MnPS3 using neutron diffrac- tion and polarimetry. MnPS3 undergoes a transition toward a collinear antiferromagnetic order at 78 K. The resulting magnetic…

Strongly Correlated Electrons · Physics 2010-12-06 Eric Ressouche , Mickael Loire , Virginie Simonet , Rafik Ballou , Anne Stunault , Andrew Wildes

The local structure about the Mn site in the half doped system La0.5Ca0.5MnO3 was measured in magnetic fields up 10 T to probe the melting of the charge ordered state. Examination of the Mn-O and Mn-Mn correlations reveal three distinct…

Strongly Correlated Electrons · Physics 2009-11-10 T. A. Tyson , M. Deleon , M. Crof , V. G. Harris , C. -C. Kao , J. Kirkland , S. -W. Cheong

The ZFC and FC magnetization dependence on temperature was measured for BiFeO3 ceramics at the applied magnetic field up to H=10T in 2K-1000K range. The antiferromagnetic order was detected from the hysteresis loops below the Neel…

Materials Science · Physics 2013-05-15 B. Andrzejewski , A. Molak , B. Hilczer , A. Budziak , R. Bujakiewicz-Koronska

We have studied the crystal and magnetic structures of the magnetoelectric materials RMn2O5 (R = Tb, Ho, Dy) using neutron diffraction as a function of temperature. All three materials display incommensurate antiferromagnetic ordering below…

Strongly Correlated Electrons · Physics 2009-11-11 G. R. Blake , L. C. Chapon , P. G. Radaelli , S. Park , N. Hur , S-W. Cheong , J. Rodriguez-Carvajal

Based on measurements of soft x-ray magnetic diffraction under in-situ applied electric field, wereport on significantly manipulation and exciting of commensurate magnetic order in multiferroic ErMn2O5. The induced magnetic scattering…

Strongly Correlated Electrons · Physics 2009-11-13 Y. Bodenthin , U. Staub , M. Garcia-Fernandez , M. Janoschek , J. Schlappa , E. I. Golovenchits , V. A. Sanina , S. G. Lushnikov

Precise magnetic structures of RMn2O5, with R= Y, Ho, Bi in the commensurate/ferroelectric regime, have been determined by single-crystal neutron diffraction. For each system, the integrated intensities of a large number of independent…

Materials Science · Physics 2007-10-11 C. Vecchini L. C. Chapon , P. J. Brown , T. Chatterji , S. Park S-W. Cheong , P. G. Radaelli

The dielectric constant of multiferroic hexagonal HoMnO_3 exhibits an unprecedented diversity of anomalies at low temperatures (1.8 K< T <10 K) and under external magnetic fields related to magnetic phase transitions in the coupled system…

Strongly Correlated Electrons · Physics 2009-11-11 F. Yen , C. R. dela Cruz , B. Lorenz , Y. Y. Sun , Y. Q. Wang , M. M. Gospodinov , C. W. Chu

Elastic neutron scattering is used to study the spin correlations in the multiferroic $\rm Mn_{1-x}Fe_{x}WO_4$ with $x=0.035, 0.05$ and 0.10. The noncollinear, incommensurate (ICM) magnetic structure associated with the ferroelectric (FE)…

Strongly Correlated Electrons · Physics 2008-11-03 F. Ye , Y. Ren , J. A. Fernandez-Baca , H. A. Mook , J. W. Lynn , R. P. Chaudhury , Y. -Q. Wang , B. Lorenz , C. W. Chu

The magnetic-field-induced 90-degree flop of ferroelectric polarization P in a spin-spiral multiferroic material TbMnO3 is theoretically studied based on a microscopic spin model. We find that the direction of the P-flop or the choice of…

Strongly Correlated Electrons · Physics 2016-01-20 Masahito Mochizuki

We have successfully induced multiferroic behavior in the A-type antiferromagnet SmMnO3 by the substitution of Y at the Sm site. A magnetic transition develops at 24 K for Sm1-xYxMnO3 (x=0.4,0.5) which is not present in the parent compound.…

Strongly Correlated Electrons · Physics 2011-05-17 D. O'Flynn , C. V. Tomy , M. R. Lees , A. Daoud-Aladine , G. Balakrishnan

Using x-ray resonant magnetic scattering and x-ray magnetic circular dichroism, techniques that are element specific, we have elucidated the role of Ho3+ in multiferroic HoMnO3. In zero field, Ho3+ orders antiferromagnetically with moments…

Other Condensed Matter · Physics 2009-04-04 S. Nandi , A. Kreyssig , L. Tan , J. W. Kim , J. Q. Yan , J. C. Lang , D. Haskel , R. J. McQueeney , A. I. Goldman

The specific properties of incommensurate multiferroic phases resulting from the coupling of order-parameter replicates are worked out using the illustrative example of iron vanadate. The dephasing between the order-parameter copies induces…

Materials Science · Physics 2015-05-27 Bruno Mettout , Pierre Toledano

There has been tremendous research activity in the field of magneto-electric (ME) multiferroics after Kimura et al. [1] showed that antiferromagnetic and ferroelectric order coexist in orthorhom- bically distorted perovskite TbMnO3 and are…

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