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Magneto-electric multiferroics exemplified by TbMnO3 possess both magnetic and ferroelectric long-range order. The magnetic order is mostly understood, whereas the nature of the ferroelectricity has remained more elusive. Competing models…

Strongly Correlated Electrons · Physics 2011-10-14 H. C. Walker , F. Fabrizi , L. Paolasini , F. de Bergevin , J. Herrero-Martin , A. T. Boothroyd , D. Prabhakaran , D. F. McMorrow

Understanding the multiferroic coupling is one of the key issues in the feld of multiferroics. As shown here theoretically, the ferromagnetic resonance (FMR) renders possible an access to the magnetoelectric coupling coefficient in…

Materials Science · Physics 2013-09-17 A. Sukhov , P. P. Horley , C. -L. Jia , J. Berakdar

We report high-resolution dilatometry studies on single crystals of the Shastry-Sutherland-lattice magnet NdB$_4$ supported by specific heat and magnetometry data. Our dilatometric studies evidence pronounced anomalies at the phase…

The pressure ($p$) -- temperature ($T$) phase diagram for microscopic magnetism in the multiferroic compound HoMn$_{2}$O$_{5}$ was established using neutron diffraction measurements under a hydrostatic pressure up to 1.25 GPa. At ambient…

Strongly Correlated Electrons · Physics 2009-11-13 Hiroyuki Kimura , Keisuke Nishihata , Yukio Noda , Naofumi Aso , Kazuyuki Matsubayashi , Yoshiya Uwatoko , Tetsuya Fujiwara

Using single crystal neutron scattering we show that the magnetic structure Ni$_3$TeO$_6$ at fields above 8.6 T along the $c$ axis changes from a commensurate collinear antiferromagnetic structure with spins along c and ordering vector…

Orthorhombic HoMnO3 is a multiferroic in which Mn antiferromagnetic order induces ferroelectricity. A second transition occurs within the multiferroic phase, in which a strong enhancement of the ferroelectric polarization occurs…

Strongly Correlated Electrons · Physics 2021-01-04 Y. W. Windsor , M. Ramakrishnan , L. Rettig , A. Alberca , T. Lippert , C. W. Schneider , U. Staub

The control of multiferroic domains through external electric fields has been studied by dielectric measurements and by polarized neutron diffraction on single-crystalline TbMnO$_3$. Full hysteresis cycles were recorded by varying an…

Strongly Correlated Electrons · Physics 2016-02-10 Jonas Stein , Max Baum , Simon Holbein , Vladimir Hutanu , Alexander C. Komarek , Markus Braden

Linearly polarized spectra of far-infrared (IR) transmission in HoMn2O5 multiferroic single crystals have been studied in the frequency range between 8.5 and 105 cm-1 and for temperatures between 5 K and 300 K. Polarization of IR-active…

Strongly Correlated Electrons · Physics 2009-11-13 A. A. Sirenko , S. M. O Malley , K. H. Ahn , S. Park , G. L. Carr , S-W. Cheong

The crystal structure of the double tungstate NaFe(WO$_4$)$_2$ arises from that of the spin-driven multiferroic MnWO$_4$ by inserting non-magnetic Na layers. NaFe(WO$_4$)$_2$ exhibits a three-dimensional incommensurate spin-spiral structure…

Strongly Correlated Electrons · Physics 2022-05-17 S. Holbein , M. Ackermann , L. Chapon , P. Steffens , A. Gukasov , A. Sazonov , O. Breunig , Y. Sanders , P. Becker , L. Bohaty , T. Lorenz , M. Braden

Ferroelectric spiral magnets DyMnO3 and TbMnO3 show similar behavior of electric polarization in applied magnetic fields. Studies of the field dependence of lattice modulations on the contrary show a completely different picture. Whereas in…

Strongly Correlated Electrons · Physics 2009-11-13 J. Strempfer , B. Bohnenbuck , M. Mostovoy , N. Aliouane , D. N. Argyriou , F. Schrettle , J. Hemberger , A. Krimmel , M. v. Zimmermann

We present a study of the magnetic and crystallographic structure of TbMnO$_3$ in the presence of crossed electric and magnetic fields using circularly polarised X-ray non-resonant scattering. A comprehensive account is presented of the…

Strongly Correlated Electrons · Physics 2014-01-13 H. C. Walker , F. Fabrizi , L. Paolasini , F. de Bergevin , D. Prabhakaran , A. T. Boothroyd , D. F. McMorrow

Neutron scattering studies of single-crystal LiNiPO$_4$ reveal a spontaneous first-order commensurate-incommensurate magnetic phase transition. Short- and long-range incommensurate phases are intermediate between the high temperature…

Strongly Correlated Electrons · Physics 2009-11-10 D. Vaknin , J. L. Zarestky , J. -P. Rivera , H. Schmid

Ferroelectricity in the incommensurate helical magnetic phase (below TN, 43K) of alpha CaCr2O4 has been confirmed by pyroelectric measurements. Magnetoelectric and magnetodielectric coupling exist below TN and are proportional to the square…

Materials Science · Physics 2012-08-03 Kiran Singh , Charles Simon , Pierre Toledano

We have carried out $^{63,65}$Cu NMR spectra measurements in magnetic field up to about 45~T on single crystal of a multiferroic triangular antiferromagnet CuCrO$_2$. The measurements were performed for magnetic fields aligned along the…

Strongly Correlated Electrons · Physics 2016-12-21 Yu. A. Sakhratov , L. E. Svistov , P. L. Kuhns , H. D. Zhou , A. P. Reyes

Evidence for a strong spin-lattice coupling in multiferroic HoMnO_3 is derived from thermal expansion measurements along a- and c-axis. The magnetoelastic effect results in sizable anomalies of the thermal expansivities at the…

Strongly Correlated Electrons · Physics 2009-11-11 C. dela Cruz , F. Yen , B. Lorenz , Y. Q. Wang , Y. Y. Sun , M. M. Gospodinov , C. W. Chu

The triangular spin lattice of NiBr$_{2}$ is a canonical example of a frustrated helimagnet that shows a temperature-driven phase transition from a collinear commensurate antiferromagnetic structure to an incommensurate spin helix on…

Materials Science · Physics 2019-03-19 S. Babu , K. Prokes , Y. K. Huang , F. Radu , S. K. Mishra

The correlation between static magnetoelectric coupling and magnetic structure was investigated in $TbMn_{0.98}Fe_{0.02}O_{3}$ with magnetic field up to 8 T and down to 2 K. Single-crystal neutron diffraction experiments reveal a…

The spin-driven component of electric polarization in a single crystal of multiferroic BiFeO$_{3}$ was experimentally investigated in pulsed high magnetic fields up to 41 T. Sequential measurements of electric polarization for various…

Strongly Correlated Electrons · Physics 2020-01-08 Shiro Kawachi , Shin Miyahara , Toshimitsu Ito , Atsushi Miyake , Nobuo Furukawa , Jun-ichi Yamaura , Masashi Tokunaga

The structural distortion and magnetoelastic coupling induced through commensurate magnetism has been investigated by neutron diffraction in structurally related MnWO$_4$ and NaFe(WO$_4$)$_2$. Both systems exhibit a competition of…

Strongly Correlated Electrons · Physics 2020-10-28 S. Biesenkamp , N. Qureshi , Y. Sidis , P. Becker , L. Bohatý , M. Braden

Quantum fluctuations in the effective spin one-half layered structure triangular-lattice quantum Heisenberg antiferromagnet Ba$_3$CoSb$_2$O$_9$ lift the classical degeneracy of the antiferromagnetic ground state in magnetic field, producing…

Strongly Correlated Electrons · Physics 2021-06-02 N. A. Fortune , Q. Huang , T. Hong , J. Ma , E. S. Choi , S. T. Hannahs , Z. Y. Zhao , X. F. Sun , Y. Takano , H. D. Zhou