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Alkali halide (100) surfaces are anomalously poorly wetted by their own melt at the triple point. We carried out simulations for NaCl(100) within a simple (BMHFT) model potential. Calculations of the solid-vapor, solid-liquid and…

Materials Science · Physics 2007-05-23 T. Zykova-Timan , D. Ceresoli , U. Tartaglino , E. Tosatti

The high temperature surface properties of alkali halide crystals are very unusual. Through molecular dynamics simulations based on Tosi-Fumi potentials, we predict that crystalline NaCl(100) should remain stable without any precursor…

Materials Science · Physics 2007-05-23 T. Zykova-Timan , U. Tartaglino , D. Ceresoli , E. Tosatti

Alkali halide (100) crystal surfaces are poorly wetted by their own melt at the triple point. We carried out simulations for NaCl(100) within the well tested BMHFT model potential. Calculations of the solid-vapor, solid-liquid and…

Materials Science · Physics 2008-09-25 D. Ceresoli , T. Zykova-Timan , U. Tartaglino , E. Tosatti

This paper presents a broad theoretical and simulation study of the high temperature behavior of crystalline alkali halide surfaces typified by NaCl(100), of the liquid NaCl surface near freezing, and of the very unusual partial wetting of…

Materials Science · Physics 2007-05-23 T. Zykova-Timan , D. Ceresoli , U. Tartaglino , E. Tosatti

The self-wetting properties of ionic crystal surfaces are studied, using NaCl(100) as a prototype case. The anomalously large contact angle measured long ago by Mutaftschiev is well reproduced by realistic molecular dynamics simulations.…

Materials Science · Physics 2007-05-23 T. Zykova-Timan , U. Tartaglino , D. Ceresoli , W. Sekkal , E. Tosatti

Surfaces which do not exhibit surface melting below the melting point (nonmelting surfaces) have been recently observed to sustain a very large amount of overheating. We present a theory which identifies a maximum overheating temperature,…

Condensed Matter · Physics 2009-10-22 Francesco D. Di Tolla , Furio Ercolessi , Erio Tosatti

We present an extensive but concise review of our present understanding, largely based on theory and simulation work from our group, on the equilibrium behavior of solid surfaces and nanosystems close to the bulk melting point. In the first…

Materials Science · Physics 2007-05-23 U. Tartaglino , T. Zykova-Timan , F. Ercolessi , E. Tosatti

The squeezing of soft solids, the constrained growth of biological tissues, and the swelling of soft elastic solids such as gels can generate large compressive stresses at their surfaces. This causes the otherwise smooth surface of such a…

Soft Condensed Matter · Physics 2014-07-09 Tuomas Tallinen , John S. Biggins , L. Mahadevan

While individual water molecules adsorb strongly on a talc surface (hydrophilic behavior), a droplet of water beads up on the same surface (hydrophobic behavior). To rationalize this dichotomy, we investigate the influence of the…

Chemical Physics · Physics 2011-09-21 Benjamin Rotenberg , Amish J. Patel , David Chandler

Melting behaviors of aluminum (111) perfect/nonperfect surfaces, characterized by structure ordering parameter, have been investigated by classical molecular dynamics simulation with embedded atom method potential. Al (111) perfect surface…

Materials Science · Physics 2015-05-14 F. L. Tang , X. G. Cheng , W. J. Lu , W. Y. Yu

The physics of sliding nanofriction at high temperature near the substrate melting point $\Tmelt$ is so far unexplored. We conducted simulations of hard tips sliding on a prototype non-melting surface, NaCl(100), revealing in this regime…

Materials Science · Physics 2007-05-23 T. Zykova-Timan , D. Ceresoli , E. Tosatti

Alkali halide crystals doped with certain impurity ions show a low temperature behaviour, which differs significantly from that of pure crystals. The origin of these characteristic differences are tunneling centers formed by atomic or…

Disordered Systems and Neural Networks · Physics 2009-11-07 M. Thesen , R. Kühn , C. Enss , S. Ludwig

Wetting transitions have been predicted and observed to occur for various combinations of fluids and surfaces. This paper describes the origin of such transitions, for liquid films on solid surfaces, in terms of the gas-surface interaction…

Materials Science · Physics 2015-05-13 Silvina M. Gatica , Milton W. Cole

In this manuscript we study the liquid-solid coexistence of NaCl-type alkali halides, described by interaction potentials such as Tosi-Fumi (TF), Smith-Dang (SD) and Joung-Cheatham (JC), and compute their melting temperature (Tm) at 1 bar…

Statistical Mechanics · Physics 2012-09-18 J. L. Aragones , E. Sanz , C. Valeriani , C. Vega

To elucidate the atomistic diffusion mechanism responsible for the rapid diffusion in alkali halide nano particles, called Spontaneous Mixing, we execute molecular dynamics simulations with empirical models for KCl-KBr, NaCl-NaBr, RbCl-RbBr…

Mesoscale and Nanoscale Physics · Physics 2016-01-11 Tomoaki Niiyama , Shin-ichi Sawada , Kensuke S. Ikeda , Yasushi Shimizu

Alumina (Al$_{2}$O$_{3}$) is a key material for thin-film growth and heterogeneous catalysis, where the atomic surface structure critically impacts performance. Using noncontact atomic force microscopy (nc-AFM) combined with density…

We investigate theoretically the wetting properties of cholesteric liquid crystals at a planar substrate. If the properties of substrate and of the interface are such that the cholesteric layers are not distorted the wetting properties are…

Motivated by the observations of intracellular phase separations and the wetting of cell membranes by protein droplets, we study the nonequilibrium surface wetting by Monte Carlo simulations of a lattice gas model involving particle…

Biological Physics · Physics 2022-06-23 Kyosuke Adachi , Kyogo Kawaguchi

Al(110) has been studied for temperatures up to 900 K via ensemble density-functional molecular dynamics. The strong anharmonicity displayed by this surface results in a negative coefficient of thermal expansion, where the first interlayer…

Materials Science · Physics 2009-10-31 Nicola Marzari , David Vanderbilt , Alessandro De Vita , M. C. Payne

The high-temperature properties of the Al(111) surface are studied by molecular-dynamics simulation. This surface does not melt below the bulk melting point, but can be superheated. Superheating of metal surfaces has been recently observed…

Materials Science · Physics 2009-10-30 G. Bilalbegovic
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