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We study how spin and orbital effects influence the capability of promoting Dzyaloshinskii-Moriya (DM) interaction by studying the two magnetic polar materials, Cu(IO3)2 (S = 1/2 with orbital contribution) and Mn(IO3)2 (S = 5/2 with…

The electronic ground state of Ca3LiOsO6 was recently considered within an intermediate coupling regime that revealed J=3/2 spin-orbit entangled magnetic moments. Through inelastic neutron scattering and density functional theory we…

Strongly Correlated Electrons · Physics 2017-11-29 S. Calder , D. J. Singh , V. O. Garlea , M. D. Lumsden , Y. G. Shi , K. Yamaura , A. D. Christianson

We present our results of a local probe study on EuFe$_{2}$(As$_{1-x}$P$_{x}$)$_{2}$ single crystals with $x$=0.13, 0.19 and 0.28 by means of muon spin rotation and ${}^{57}$Fe M\"ossbauer spectroscopy. We focus our discussion on the sample…

We report on the physical properties of single crystalline EuRhSi$_3$ and polycrystalline EuIrSi$_3$, inferred from magnetisation, electrical transport, heat capacity and $^{151}$Eu M\"ossbauer spectroscopy. These previously known compounds…

Strongly Correlated Electrons · Physics 2015-09-02 A. Maurya , P. Bonville , A. Thamizhavel , S. K. Dhar

The investigation of crystallographic, electronic, and magnetic characteristics, especially the mixed valences of Eu$^{2+}$ and Eu$^{3+}$ under pressure of a novel europium-based bismuth selenide compound, Eu$_4$Bi$_6$Se$_{13}$, presented.…

The exchange interactions and magnetic structure in layered system CuMnO2 (mineral crednerite) and in nonstoichiometric system Cu1.04Mn0.96O2, with triangular layers distorted due to orbital ordering of the Mn3+ ions, are studied by…

Strongly Correlated Electrons · Physics 2014-01-21 A. V. Ushakov , S. V. Streltsov , D. I. Khomskii

Magnetic excitations and magnetic structure of EuRbFe$_4$As$_4$ were investigated by inelastic neutron scattering (INS), neutron diffraction, and random phase approximation (RPA) calculations. Below the superconducting transition…

A ferromagnetic coupling between localized Mn spins was predicted in a series of \textit{ab initio} and tight binding calculations and experimentally verified for the dilute magnetic semiconductor Ga$_{1-x}$Mn$_x$N. In the limit of small Mn…

Materials Science · Physics 2020-12-30 D. Sztenkiel , K. Gas , J. Z. Domagala , D. Hommel , M. Sawicki

Sr$_{3}$ZnIrO$_{6}$ is an effective spin one-half Mott insulating iridate belonging to a family of magnets which includes a number of quasi-one dimensional systems as well as materials exhibiting three dimensional order. Here we present the…

Strongly Correlated Electrons · Physics 2020-05-19 P. A. McClarty , A. D. Hillier , D. T. Adroja D. D. Khalyavin , S. Rayaprol , P. Manuel , W. Kockelmann , E. V. Sampathkumaran

The magnetic properties of single crystalline EuPtGe$_3$, crystallizing in the non-centrosymmetric BaNiSn$_3$-type crystal structure, have been studied by means of magnetisation, electrical resistivity, heat capacity and $^{151}$Eu…

Strongly Correlated Electrons · Physics 2011-12-22 Neeraj Kumar , Pranab Kumar Das , Ruta Kulkarni , A. Thamizhavel , S. K. Dhar , P. Bonville

Two-dimensional van der Waals compounds with magnetic ions on a honeycomb lattice are hosts to a variety of exotic behavior. The magnetic interactions in one such compound, MnPSe$_3$, are investigated with elastic and inelastic neutron…

Strongly Correlated Electrons · Physics 2021-01-20 S. Calder , A. V. Haglund , A. I. Kolesnikov , D. Mandrus

Iridates abound with interesting magnetic behaviours because of their strong spin-orbit coupling. Sr$_3$NiIrO$_6$ brings together the spin-orbital entanglement of the Ir$^{4+}$ ion with a 3$d$ Ni cation and a one-dimensional crystal…

Materials Science · Physics 2018-10-19 Turan Birol , Kristjan Haule , David Vanderbilt

The significance of the spin-orbit interaction is very well known in compounds containing heavier elements such as the rare-earth Eu ion. Here, through density functional calculations, we investigated the effect of the spin-orbit…

The rational combination of existing magnetic topological compounds presents a promising route for designing new topological materials. We report the synthesis and comprehensive characterization of the layered quaternary intergrowth…

The spin-orbital entangled states are of great interest as they hold exotic phases and intriguing properties. Here we use first-principles calculations to investigate the electronic and magnetic properties of RuI$_{3}$ and RuCl$_{3}$ in…

Strongly Correlated Electrons · Physics 2023-04-21 Lu Liu , Ke Yang , Guangyu Wang , Di Lu , Yaozhenghang Ma , Hua Wu

Neutron reflectivity studies of EuS/SrS, EuS/PbSe, and EuS/PbTe all-semiconductor superlattices were carried out in search for exchange interlayer coupling. A relatively weak antiferromagnetic coupling was found in EuS/SrS and in EuS/PbSe…

Materials Science · Physics 2009-11-13 H. Kepa , C. F. Majkrzak , A. Sipatov , A. G. Fedorov , T. A. Samburskaya , T. M. Giebultowicz

$\gamma$-triclinic and $\alpha$-monoclinic polymorphs of CoV$_{2}$O$_{6}$ are two of the few known transition metal ion based materials that display stepped $1/3$ magnetization plateaus at low temperatures. Neutron diffraction [M. Markkula…

Strongly Correlated Electrons · Physics 2015-12-23 F. Wallington , A. M. Arevalo-Lopez , J. W. Taylor , J. R. Stewart , V. Garcia-Sakai , J. P. Attfield , C. Stock

Magnetic, thermal and transport properties of the non-centrosymmetric compound Eu$_2$Pd$_2$Sn are revisited after including new measurements. In its paramagnetic phase, the outstanding feature of this compound is the formation of Eu$^{2+}$…

Strongly Correlated Electrons · Physics 2023-08-02 J. G. Sereni , I. Čurlik , M. Reiffers , M. Goivannini

We report on the microscopic magnetic model of a spin-1/2 magnet BaV$_3$O$_8$. In contrast to earlier phenomenological analysis, our density-functional band-structure calculations combined with quantum Monte-Carlo simulations establish a…

Materials Science · Physics 2014-01-09 Alexander A. Tsirlin

Europium nitride is semiconducting and contains non-magnetic \3+, but sub-stoichiometric EuN has Eu in a mix of 2+ and 3+ charge states. We show that at \2+ ~concentrations near 15-20% EuN is ferromagnetic with a Curie temperature as high…

Materials Science · Physics 2013-10-30 Do Le Binh , B. J. Ruck , F. Natali , H. Warring , H. J. Trodahl , E. -M. Anton , C. Meyer , L. Ranno , F. Wilhelm , A. Rogalev