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We develop a theory of collective spin dynamics triggered by ultrafast optical excitation of ferromagnetic semiconductors. Using the density matrix equations of motion in the mean field approximation and including magnetic anisotropy and…

Strongly Correlated Electrons · Physics 2009-11-13 J. Chovan , I. E. Perakis

Precession of magnetization induced by pulsed optical excitation is observed in a ferromagnetic semiconductor (Ga,Mn)As by time-resolved magneto-optical measurements. It appears as complicated oscillations of polarization plane of…

Materials Science · Physics 2009-11-13 Y. Hashimoto , H. Munekata

We present a study of photo-excited magnetization dynamics in ferromagnetic (Ga,Mn)As films observed by time-resolved magneto-optical measurements. The magnetization precession triggered by linearly polarized optical pulses in the absence…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 Hang Li , Xinyu Liu , Ying-Yuan Zhou , Jacek K. Furdyna , Xinhui Zhang

A quantitative understanding of the processes that trigger light-induced demagnetization on ultrashort timescales is crucial for achieving an ultrafast, radiation-controlled magnetic response in materials. This milestone is essential for…

Irradiating solids with ultrashort laser pulses is known to initiate femtosecond timescale magnetization dynamics. However, sub-femtosecond spin dynamics have not yet been observed or predicted. Here, we explore ultrafast light-driven spin…

Mesoscale and Nanoscale Physics · Physics 2023-03-28 Ofer Neufeld , Nicolas Tancogne-Dejean , Umberto De Giovannini , Hannes Hübener , Angel Rubio

The magnetization of a non-magnetic semiconductor by femtosecond light pulses is crucial to achieve an all-optical control of the spin dynamics in materials and to develop faster memory devices. However, the conditions for its detection are…

Materials Science · Physics 2022-06-29 Giovanni Marini , Matteo Calandra

Electronic excitations in a ferromagnet can trigger ultrafast spin dynamics with potential applications in a speed increase in magnetic recording. The project investigates ultrafast magnetization dynamics, which is driven in metallic layers…

Materials Science · Physics 2010-07-06 Adrian Glaubitz

Non-thermal laser induced spin excitations, recently discovered in conventional oxide and metal ferromagnets, open unprecedented opportunities for research and applications of ultrafast optical manipulation of magnetic systems.…

Materials Science · Physics 2011-01-06 P. Nemec , E. Rozkotova , N. Tesarova , F. Trojanek , K. Olejnik , J. Zemen , V. Novak , M. Cukr , P. Maly , T. Jungwirth

Excitation of a metallic ferromagnet such as Ni with an intensive femtosecond laser pulse causes an ultrafast demagnetization within approximately 300 fs. It was proposed that the ultrafast demagnetization measured in femtosecond…

Materials Science · Physics 2016-09-27 Ritwik Mondal , Marco Berritta , Karel Carva , Peter M. Oppeneer

The non-thermal optical control of magnetic order offers a promising route to ultrafast, energy-efficient information technologies. Although optical manipulation of magnetism in metals has been extensively studied, experimentally…

We use femtosecond optical pulses to induce, control and monitor magnetization precession in ferromagnetic Ga0.965Mn0.035As. At temperatures below ~40 K we observe coherent oscillations of the local Mn spins, triggered by an ultrafast…

Materials Science · Physics 2009-11-13 J. Qi , Y. Xu , N. Tolk , X. Liu , J. K. Furdyna , I. E. Perakis

We propose and analyze a theoretical model of ultrafast light-induced magnetization dynamics in systems of localized spins that are coupled to carriers' spins by sp-d exchange interaction. A prominent example of a class of materials falling…

Mesoscale and Nanoscale Physics · Physics 2008-02-20 L. Cywinski , L. J. Sham

Optically-induced phase transitions of the manganite $\rm Pr_{1/3}Ca_{2/3}MnO_3$ have been simulated using a model Hamiltonian, that captures the dynamics of strongly correlated charge, orbital, lattice, and spin degrees of freedom. Its…

Strongly Correlated Electrons · Physics 2020-12-01 Sangeeta Rajpurohit , Liang Z. Tan , Christian Jooss , P. E. Blöchl

Ultrafast laser pulses provide unique tools to manipulate magnetization dynamics at femtosecond timescales, where the interaction of the electric field -- such as excitation of spin carriers to non-equilibrium states, generation of…

Using density matrix equations of motion, we predict a femtosecond collective spin tilt triggered by nonlinear, near--ultraviolet ($\sim$3eV), coherent photoexcitation of (Ga,Mn)As ferromagnetic semiconductors with linearly polarized light.…

Strongly Correlated Electrons · Physics 2009-08-06 M. D. Kapetanakis , I. E. Perakis , K. J. Wickey , C. Piermarocchi , J. Wang

The ultimate control of magnetic states of matter at femtosecond (or even faster) timescales defines one of the most pursued paradigm shifts for future information technology. In this context, ultrafast laser pulses developed into extremely…

Mesoscale and Nanoscale Physics · Physics 2022-03-15 Hanan Hamamera , Filipe Souza Mendes Guimarães , Manuel dos Santos Dias , Samir Lounis

By using intense coherent electromagnetic radiation, it may be possible to manipulate the properties of quantum materials very quickly, or even induce new and potentially useful phases that are absent in equilibrium. For instance, ultrafast…

Strongly Correlated Electrons · Physics 2023-03-30 Jonathan B. Curtis , Ankit Disa , Michael Fechner , Andrea Cavalleri , Prineha Narang

By comparing the photo-induced magnetization dynamics in simple layered systems we show how light-induced modifications of the magnetic anisotropy directly enhance the magnetization. It is observed that the spin precession in…

We report single-color, time resolved magneto-optical measurements in ferromagnetic semiconductor (Ga,Mn)As. We demonstrate coherent optical control of the magnetization precession by applying two successive ultrashort laser pulses. The…

Materials Science · Physics 2009-11-13 E. Rozkotova , P. Nemec , N. Tesarova , P. Maly , V. Novak , K. Olejnik , M. Cukr , T. Jungwirth

We investigate the impact of non-collinear dual optical excitation on the magnetization precession in a permalloy thin film using two ultrashort laser pulses. By analyzing the magnetization dynamics using time-resolved magneto-optical…

Materials Science · Physics 2024-06-28 Sergii Parchenko , Davide Pecchio , Ritwik Mondal , Peter M. Oppeneer , Andreas Scherz
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