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We have developed a thermodynamic model of the catalytic growth of multiwall carbon nanotubes from hydrocarbon precursors at elevated temperature. Using this model we have computed the heat distribution, and carbon concentration in the…

Materials Science · Physics 2015-07-20 Christian Klinke , Jean-Marc Bonard , Klaus Kern

The evolution of a continuous Fe(NO3)3 catalyst film was observed by in-situ annealing in a Transmission Electron Microscope (TEM). Such catalysts are routinely used in the catalytic growth of carbon nanotubes. The experiments reveal that…

Materials Science · Physics 2015-07-20 Christian Klinke , Jean-Marc Bonard , Klaus Kern

This investigation deals with the effect of growth temperature on the growth behavior of Fe filled multiwalled carbon nanotubes (MWCNTs). Carbon nanotube (CNT) synthesis was carried out in a thermal chemical vapor deposition (CVD) reactor…

Materials Science · Physics 2019-08-07 Joydip Sengupta , Chacko Jacob

Growth of carbon nanotubes (CNTs) was performed by atmospheric pressure chemical vapour deposition (APCVD) of propane on Si(111) with a pre-treated Ni overlayer acting as a catalyst. Prior to the growth of CNTs, a thin film of Ni was…

Materials Science · Physics 2019-06-04 J Sengupta , SK Panda , C Jacob

In this study, the synthesis of multi-walled carbon nanotubes (MWCNTs) was carried out by chemical vapor deposition (CVD) using propane as the carbon source and Si as the catalyst support. The effect of CVD process variables such as…

Applied Physics · Physics 2018-08-21 Joydip Sengupta

Fe filled carbon nanotubes were synthesized by atmospheric pressure chemical vapor deposition using a simple mixture of iron acetylacetonate with a conventional photoresist and the effect of growth temperature from 550 to 950 {\deg}C on Fe…

Applied Physics · Physics 2020-04-28 Joydip Sengupta , Avijit Jana , N. D. Pradeep Singh , Chacko Jacob

We prepared three ferrite nanocatalysts: (i) copper ferrite (CuFe2O4), (ii) ferrite where cobalt was substituted by nickel (NixCo1-xFe2O4, with x= 0, 0.2, 0.4, 0.6), and (iii) ferrite where nickel was substituted by zinc (ZnyNi1-yFe2O4 with…

Materials Science · Physics 2011-09-01 R. Hosseini Akbarnejad , V. Daadmehr , F. Shahbaz Tehrani , F. Aghakhani , S. Gholipour

We investigate the growth of the recently demonstrated composite material composed of vertically aligned carbon nanotubes capped by few graphene layers. We show that the carbon nanotubes grow epitaxially under the few graphene layers. By…

Materials Science · Physics 2011-03-24 V. Jousseaume , J. Cuzzocrea , N. Bernier , Vincent Thomas Francois Renard

Various diameters of alumina-supported Fe catalysts are used to grow single-walled carbon nanotubes (SWCNTs) with chemical vapor decomposition. We find that the reduction of the catalyst size requires an increase of the minimum temperature…

Materials Science · Physics 2009-11-13 A. R. Harutyunyan , N. Awasthi , A. Jiang , W. Setyawan , E. Mora , T. Tokune , K. Bolton , S. Curtarolo

Optimized growth of Single Wall Carbon Nanotubes requires a full knowledge of the actual state of the catalyst nanoparticle and its interface with the tube. Using Tight Binding based atomistic computer simulations, we calculate carbon…

Materials Science · Physics 2015-06-05 Mamadou Diarra , Alexandre Zappelli , Hakim Amara , François Ducastelle , Christophe Bichara

A parametric study of so-called "super growth" of single-walled carbon nanotubes(SWNTs) was done by using combinatorial libraries of iron/aluminum oxide catalysts. Millimeter-thick forests of nanotubes grew within 10 min, and those grown by…

Materials Science · Physics 2009-11-13 S. Noda , K. Hasegawa , H. Sugime , K. Kakehi , Z. Zhang , S. Maruyama , Y. Yamaguchi

The molecular dynamics method, based on an empirical potential energy surface, was used to study the effect of catalyst particle size on the growth mechanism and structure of single-walled carbon nanotubes (SWNTs). The temperature for…

Materials Science · Physics 2009-11-11 Feng Ding , Arne Rosen , Kim Bolton

We investigate iron-cobalt (Fe-Co) alloys as a representative high-performance catalyst system for SWCNT growth in a systematic manner by combining chemical vapor deposition (CVD) experiments with chirality-resolved spectroscopic analysis,…

We used microcontact printing to pattern a silicon surface with an iron-containing catalytic solution. Multi-wall carbon nanotubes were subsequently grown on the patterned areas by chemical vapor deposition at temperatures between 650 and…

Materials Science · Physics 2015-07-20 Christian Klinke , Ralph Kurt , Jean-Marc Bonard , Klaus Kern

The ability to integrate carbon nanotubes, especially single-walled carbon nanotubes, seamlessly onto silicon would expand the range of applications considerably. Though direct integration using chemical vapor deposition is the simplest…

Materials Science · Physics 2007-10-10 J. M. Simmons , B. M. Nichols , Matthew S. Marcus , O. M. Castellini , R. J. Hamers , M. A. Eriksson

Carbon nanotubes have properties depending on the arrangement of carbon atoms on the tube walls, called chirality. Also it has been tried to grow nanotubes of only one chirality for more than a decade it is still not possible today. A…

Materials Science · Physics 2013-05-02 Heiko Dumlich , John Robertson , Stephanie Reich

Chemical vapor deposition synthesis of single-walled carbon nanotubes experiments, using Fe catalyst, and alternating methane and carbon monoxide as carbon feedstocks, lead to the reversible formation of junctions between tubes of different…

We have studied nickel, gold, and ferritin coatings on catalytically grown multiwall carbon nanotubes, as well as the generation of secondary nanotubes by resubmitting the decorated nanotubes to the chemical vapor deposition process. Nickel…

Materials Science · Physics 2015-07-20 Christian Klinke , Erik Delvigne , Johannes V. Barth , Klaus Kern

The surface reconstruction of the Fe catalyst films due to high temperature processing in hydrogen prior to nanotube nucleation and its effect on the growth morphologies of partially filled carbon nanotubes (CNTs) synthesized using…

Applied Physics · Physics 2020-04-27 Joydip Sengupta , Chacko Jacob

Metal catalysts supporting the growth of Single Wall Carbon Nanotubes display different carbon solubilities and chemical reactivities. In order to specifically assess the role of carbon solubility, we take advantage of the physical…

Materials Science · Physics 2017-02-23 Juan-Manuel Aguiar-Hualde , Yann Magnin , Hakim Amara , Christophe Bichara
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