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We apply density functional theory band structure calculations and quantum Monte Carlo simulations to investigate the Bose-Einstein condensation in the spin-1/2 quantum magnet Pb2V3O9. In contrast to previous conjectures on the…

Strongly Correlated Electrons · Physics 2011-02-21 Alexander A. Tsirlin , Helge Rosner

The compound BaCuSi2O6 is a quantum magnet with antiferromagnetic dimers of S = 1/2 moments on a quasi-2D square lattice. We have investigated its spin dynamics by inelastic neutron scattering experiments on single crystals with an energy…

Strongly Correlated Electrons · Physics 2008-04-24 Ch. Rüegg , D. F. McMorrow , B. Normand , H. M. Ronnow , S. E. Sebastian , I. R. Fisher , C. D. Batista , S. Gvasaliya , Ch. Niedermayer , J. Stahn

In the first part we investigate in detail if the Bose-Einstein condensation scenario for magnons can quantitatively explain the observed field-induced magnetic ordering in TlCuCl$_3$. We use a bond-operator approach to map the spin system…

Strongly Correlated Electrons · Physics 2013-06-20 J. Sirker , A. Weiße , O. P. Sushkov

We present inelastic neutron scattering data on the quantum paramagnet AgVOAsO4 that establish the system is a S=1/2 alternating spin chain compound and provide a direct measurement of the spin gap. We also present experimental evidence for…

We present a $^{63,65}$Cu and $^{29}$Si NMR study of the quasi-2D coupled spin 1/2 dimer compound BaCuSi$_2$O$_6$ in the magnetic field range 13-26 T and at temperatures as low as 50 mK. NMR data in the gapped phase reveal that below 90 K…

Strongly Correlated Electrons · Physics 2008-02-11 S. Kramer , R. Stern , M. Horvatic , C. Berthier , T. Kimura , I. R. Fisher

We propose and analyze a general mechanism of disorder-induced order in two-component Bose-Einstein condensates, analogous to corresponding effects established for XY spin models. We show that a random Raman coupling induces a relative…

Magnetization measurements were performed to investigate the critical behavior of the field-induced magnetic ordering in gapped spin system TlCuCl$_3$. The critical density of the magnons was obtained as a function of temperature and the…

Strongly Correlated Electrons · Physics 2015-05-13 Fumiko Yamada , Toshio Ono , Hidekazu Tanaka , Gregoire Misguich , Masaki Oshikawa , Toshiro Sakakibara

Bose-Einstein condensation (BEC) underpins exotic forms of order ranging from superconductivity to superfluid 4 He. In quantum magnetic materials, ordered phases induced by an applied magnetic field can be described as the BEC of magnon…

We study magnetic field-induced three-dimensional ordering transitions in low-dimensional quantum spin liquids, such as weakly coupled, antiferromagnetic spin-1/2 Heisenberg dimers and ladders. Using stochastic series expansion quantum…

Strongly Correlated Electrons · Physics 2009-11-07 Stefan Wessel , Maxim Olshanii , Stephan Haas

Bose-Einstein condensation (BEC) of triplet excitations triggered by a magnetic field, sometimes called magnon BEC, in dimerized antiferromagnets gives rise to a long-range antiferromagnetic order in the plane perpendicular to the applied…

Strongly Correlated Electrons · Physics 2022-04-08 Qi-Rong Zhao , Meng-Jie Sun , Zheng-Xin Liu , Jiucai Wang

In ordered magnets, the elementary excitations are spin waves (magnons), which obey Bose-Einstein statistics. Similarly to Cooper pairs in superconductors, magnons can be paired into bound states under attractive interactions. The Zeeman…

Starting from a phenomenological standard energy functional to describe the condensation of a dilute gas of bosonic quasiparticles in magnetic insulators, we find that the inclusion of a perturbation term that explicitly violates the axial…

Strongly Correlated Electrons · Physics 2012-12-18 A. Schilling

We report an experimental determination of the phase boundary between a quantum paramagnetic state and the proposed spin Bose-Einstein condensate of triplons in the spin gap compound BaCuSi2O6. The ordering temperature is related to the…

Strongly Correlated Electrons · Physics 2011-12-08 S. E. Sebastian , P. A. Sharma , M. Jaime , N. Harrison , V. Correa , L. Balicas , N. Kawashima , C. D. Batista , I. R. Fisher

The dimerized S=1/2 spins of the Cu ions in TlCuCl3 are ordered antiferromagnetically in the presence of a field larger than about 54 kOe in the zero-temperature limit. Within the mean-field approximation all thermal effects are frozen out…

Strongly Correlated Electrons · Physics 2015-05-13 Jens Jensen , Henrik Smith

Besides being an ancient pigment, BaCuSi$_2$O$_6$ is a quasi-2D magnetic insulator with a gapped spin dimer ground state. The application of strong magnetic fields closes this gap creating a gas of bosonic spin triplet excitations called…

Strongly Correlated Electrons · Physics 2009-11-10 M. Jaime , V. F. Correa , N. Harrison , C. D. Batista , N. Kawashima , Y. Kazuma , G. A. Jorge , R. Stern , I. Heinmaa , S. A. Zvyagin , Y. Sasago , K. Uchinokura

We study field-induced magnetic order in cubic lattices of dimers with antiferromagnetic Heisenberg interactions. The thermal critical exponents at the quantum phase transition from a spin liquid to a magnetically ordered phase are…

Strongly Correlated Electrons · Physics 2009-11-10 Omid Nohadani , Stefan Wessel , Bruce Normand , Stephan Haas

The recent observation [Oosawa et al. J. Phys. : Condens. Matter {\bf 11}, 265 (1999)] of the field-induced N\'{e}el ordering in a spin-gap magnetic compound TlCuCl$_3$ is interpreted as a Bose-Einstein Condensation of magnons. A mean-field…

Statistical Mechanics · Physics 2016-08-31 T. Nikuni , M. Oshikawa , A. Oosawa , H. Tanaka

Motivated by recent experiments on Ba$_{3}$Cr$_{2}$O$_8$, a new spin-dimer compound with spin-1/2 moments of Cr$^{5+}$ ions, we theoretically investigate the field-induced magnetic ordering in this material in view of the Bose-Einstein…

Strongly Correlated Electrons · Physics 2010-03-09 Tyler Dodds , Bohm-Jung Yang , Yong Baek Kim

The magnetic properties of the interacting dimer system TlCuCl3 are investigated within a bond-operator formulation. The observed field-induced staggered magnetic order perpendicular to the field is described as a Bose condensation of…

Strongly Correlated Electrons · Physics 2009-11-07 Masashige Matsumoto , B. Normand , T. M. Rice , Manfred Sigrist

We synthesized single crystals of composition Ba$_2$CuSi$_2$O$_6$Cl$_2$ and investigated its quantum magnetic properties. The crystal structure is closely related to that of the quasi-two-dimensional (2D) dimerized magnet BaCuSi$_2$O$_6$…

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