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Related papers: Rectification Mechanism in Di-Block Oligomer Molec…

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We present a theory of tunneling and resonant transitions in one-dimensional molecular systems which is based on Green's function theory of electron sub-barrier scattering off the structural units (or functional groups) of a molecular…

Other Condensed Matter · Physics 2007-05-23 I. I. Oleynik , M. A. Kozhushner , V. S. Posvyanskii

Asymmetric current--voltage ($I(V)$) curves, known as the diode or rectification effect, in one--dimensional electronic conductors can have their origin from scattering off a single asymmetric impurity in the system. We investigate this…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Bernd Braunecker , D. E. Feldman , J. B. Marston

The transport properties of a octane-dithiol (ODT) molecule coupled to Au(001) leads are analyzed using density functional theory and non-equilibrium Green functions. It is shown that a symmetric molecule can turn into a diode under…

Mesoscale and Nanoscale Physics · Physics 2010-02-09 Tomasz Kostyrko , Víctor M. García-Suárez , Colin J. Lambert , Bogdan R. Bułka

We demonstrate large rectification ratios (> 100) in single-molecule junctions based on a metal-oxide cluster (polyoxometalate), using a scanning tunneling microscope (STM) both at ambient conditions and at low temperature. These…

Mesoscale and Nanoscale Physics · Physics 2015-06-25 Siya Sherif , G Rubio-Bollinger , E. Pinilla-Cienfuegos , E. Coronado , J. C. Cuevas , Nicolas Agrait

Resonant electron transport through a mesoscopic region (quantum dot or single molecule) with electron-phonon interaction is considered at finite voltage. In this case the standard Landauer-B\"uttiker approach cannot be applied. Using the…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 D. A. Ryndyk , J. Keller

We examine the robustness of single-molecule tunneling diodes to thermal-environmental effects. The diode comprises three fragments: two different conjugated chemical groups at the boundaries, and a saturated moiety in between, breaking…

Mesoscale and Nanoscale Physics · Physics 2015-12-29 Michael Kilgour , Dvira Segal

The concept of single molecule rectifiers proposed in a theoretical work by Aviram and Ratner in 1974 was the starting point of the now vibrant field of molecular electronics. In the meantime, a built-in asymmetry in the conductance of…

Mesoscale and Nanoscale Physics · Physics 2008-03-28 R Stadler , V Geskin , J Cornil

Motivated by recent experimental refinements of stellar reaction rates, we establish a non-perturbative Green's function formalism based on the exact solution of the Dyson equation for sub-barrier proton-nucleus resonant scattering. By…

Nuclear Theory · Physics 2026-03-19 Bahruz Suleymanli , Kutsal Bozkurt

We study current rectification effect in an asymmetric molecule HOOC-C$_6$H$_4$-(CH$_2$)$_n$ sandwiched between two Aluminum electrodes using an {\sl ab initio} nonequilibrium Green function method. The conductance of the system decreases…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Yan-hong Zhou , Xiao-hong Zheng , Ying Xu , Zhao Yang Zeng

A minimal model for coherent transport through a donor/acceptor molecular junction is presented. The two donor and acceptor sites are described by single levels energetically separated by an intramolecular tunnel barrier. In the limit of…

Disordered Systems and Neural Networks · Physics 2009-11-11 Florian Pump , Gianaurelio Cuniberti

A mechanism of quantum-mechanical tunneling is based on electron-wavefunction and is used to explain ohmic contact as well as tunnel and Zener diodes. Tunneling is the important example of wave-particle duality. In this study, an attempt is…

Applied Physics · Physics 2026-03-25 Jianming Li

Quantum transport through single molecules is very sensitive to the strength of the molecule-electrode contact. Here, we investigate the behavior of a model molecular junction weakly coupled to external electrodes in the case where charging…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Bo Song , Dmitry A. Ryndyk , Gianaurelio Cuniberti

We investigate the electronic transport through a molecule in the Kondo regime. The tunneling between the electrode and the molecule is asymmetrically modulated by the oscillations of the molecule, i.e., if the molecule gets closer to one…

Mesoscale and Nanoscale Physics · Physics 2008-12-09 J. Mravlje , A. Ramsak

We investigate nonlinear thermal transport properties of a single interacting quantum dot with two energy levels tunnel-coupled to two electrodes using nonequilibrium Green function method and Hartree-Fock decoupling approximation. In the…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Chen Xue-Ou , Bing Dong , X. L. Lei

A quantum statistical theory of spin-dependent tunneling through asymmetric magnetic double barrier junctions is presented which describes $both$ ballistic and diffuse tunneling by a single analytical expression. It is evidenced that the…

Materials Science · Physics 2009-11-07 M. Chshiev , D. Stoeffler , A. Vedyayev , K. Ounadjela

A self-consistent method for calculating electron transport through a molecular device is proposed. It is based on density functional theory electronic structure calculations under periodic boundary conditions and implemented in the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 San-Huang Ke , Harold U. Baranger , Weitao Yang

Transport properties of asymmetric molecular structure are studied within the kinetic equation approach, taking into consideration the electron interaction in the self-consistent manner (SCF procedure). The device is made of a molecule…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Kamil Walczak

Asymmetric double tunnel barriers with the center electrode being a metal cluster in the quantum regime are studied. The zero dimensionality of the clusters used and the associated quantized energy spectra are manifest in well-defined steps…

Other Condensed Matter · Physics 2009-11-11 A. Iovan , D. B. Haviland , V. Korenivski

The bias dependence of the tunnel magnetoresistance (TMR) of Fe/MgO/Fe tunnel junctions is investigated theoretically with a fully self-consistent scheme that combines the non-equilibrium Green's functions method with density functional…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Ivan Rungger , Oleg N. Mryasov , Stefano Sanvito

Within a quasiclassical transport theory for 2D electron system we analyze a recently observed effect of microwave rectification at the boundary between two 2D metals of different carrier densities. Nonlinear response is employed to explain…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Natalya A. Zimbovskaya
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