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We have performed non-equilibrium dynamics simulations of a binary Lennard-Jones mixture in which an external force is applied on a single tagged particle. For the diffusive properties of this particle parallel to the force superdiffusive…

Statistical Mechanics · Physics 2015-06-11 Carsten F. E. Schroer , Andreas Heuer

We present the results of a large scale molecular dynamics computer simulation study in which we investigate whether a supercooled Lennard-Jones liquid exhibits dynamical heterogeneities. We evaluate the non-Gaussian parameter for the self…

Disordered Systems and Neural Networks · Physics 2009-10-30 Walter Kob , Claudio Donati , Steven J. Plimpton , Peter H. Poole , Sharon C. Glotzer

Non-Gaussian displacement distributions are universal predictors of dynamic heterogeneity in slowly varying environments. Here, we explore heterogeneous dynamics in supercooled liquid using molecular dynamics simulations and show the…

Soft Condensed Matter · Physics 2023-08-29 Vinay Vaibhav , Suman Dutta

We present molecular dynamics simulations of a binary Lennard-Jones mixture at temperatures below the kinetic glass transition. The ``mobility'' of a particle is characterized by the amplitude of its fluctuation around its average position.…

Statistical Mechanics · Physics 2009-11-07 Katharina Vollmayr-Lee , Walter Kob , Kurt Binder , Annette Zippelius

The diffusivity of tagged particles is demonstrated to be heterogeneous on time scales comparable to or less than the structural relaxation time %taking place at the interparticle distance in a highly supercooled liquid via 3D molecular…

Soft Condensed Matter · Physics 2009-10-31 Ryoichi Yamamoto , Akira Onuki

Non-Gaussian nature of the probability distribution of particles' displacements in the supercooled temperature regime in glass-forming liquids are believed to be one of the major hallmarks of glass transition. It is already been established…

Statistical Mechanics · Physics 2018-08-29 Bhanu Prasad Bhowmik , Indrajit Tah , Smarajit Karmakar

We report an investigation of the heterogeneity in super-cooled liquids and glasses using the non-Gaussianity parameter. We simulate selenium and a binary Lennard-Jones system by molecular dynamics. In the non-Gaussianity three time domains…

Disordered Systems and Neural Networks · Physics 2007-05-23 D. Caprion , J. Matsui , H. R. Schober

According to the classical theory of Brownian motion, the mean squared displacement of diffusing particles evolves linearly with time whereas the distribution of their displacements is Gaussian. However, recent experiments on mesoscopic…

Soft Condensed Matter · Physics 2021-08-24 J. M. Miotto , S. Pigolotti , A. V. Chechkin , S. Roldán-Vargas

Recent progresses in single particle tracking have shown evidences of non-Gaussian distribution of displacements in living cells, both near the cellular membrane and inside the cytoskeleton. A similar behavior has also been observed in…

Biological Physics · Physics 2019-05-30 Yann Lanoiselée , Denis S. Grebenkov

The diffusivity of tagged particles is demonstrated to be very heterogeneous on time scales comparable to or shorter than the $\alpha$ relaxation time $\tau_{\alpha}$ ($\cong$ the stress relaxation time) in a highly supercooled liquid via…

Soft Condensed Matter · Physics 2009-10-31 Ryoichi Yamamoto , Akira Onuki

We have carried out extensive molecular dynamics simulations of a supercooled polydisperse Lennard-Jones liquid with large variations in temperature at a fixed pressure. The particles in the system are considered to be polydisperse both in…

Soft Condensed Matter · Physics 2009-11-07 Rajesh K. Murarka , Biman Bagchi

Comment on `Fickian Non-Gaussian Diffusion in Glass-Forming Liquids', by Rusciano et al., Phys. Rev. Lett. 128, 168001 (2022). In a recent Letter, Rusciano et al. examined the statistics of individual particles displacements in…

Statistical Mechanics · Physics 2023-10-05 Ludovic Berthier , Elijah Flenner , Grzegorz Szamel

We study the effect of randomly distributed diffusivities and speeds in two models for active particle dynamics with active and passive fluctuations. We demonstrate how non-Gaussian displacement distributions emerge in these models in the…

Statistical Mechanics · Physics 2023-02-01 Elisabeth Lemaitre , Igor M. Sokolov , Ralf Metzler , Aleksei V. Chechkin

Non-Gaussianity indicates complex dynamics related to extreme events or significant outliers. However, the correlation between non-Gaussianity and the dynamics of heterogeneous environments in anomalous diffusion remains uncertain. Inspired…

Soft Condensed Matter · Physics 2023-11-22 Haolan Xu , Xu Zheng , Xinghua Shi

Anomalous diffusion and non-Gaussian statistics are detected experimentally in a two-dimensional driven-dissipative system. A single-layer dusty plasma suspension with a Yukawa interaction and frictional dissipation is heated with laser…

Soft Condensed Matter · Physics 2009-11-13 Bin Liu , J. Goree

The non-Gaussian normal diffusion, i.e., the probability distribution function (PDF) is non-Gaussian but the mean squared displacement (MSD) depends on time linearly, has been observed in particle motions. Here we show by numerical…

Disordered Systems and Neural Networks · Physics 2016-04-06 Jianjin Wang , Yong Zhang , Hong Zhao

Dynamic heterogeneity, believed to be one of the hallmarks of the dynamics of supercooled liquids, is expected to affect the diffusion of the particles comprising the liquid. We have carried out extensive molecular dynamics simulations of…

Soft Condensed Matter · Physics 2019-12-23 Rajsekhar Das , Chandan Dasgupta , Smarajit Karmakar

The existence of heterogeneity in the dynamics of supercooled liquids is believed to be one of the hallmarks of the glass transition. Intense research has been carried out in the past to understand the origin of this heterogeneity in…

Soft Condensed Matter · Physics 2020-07-01 Indrajit Tah , Smarajit Karmakar

The use of the isoconfigurational ensemble to explore structure-dynamic correlations in supercooled liquids is examined. The statistical error of the dynamic propensity and its spatial distribution are determined. The authors present the…

Statistical Mechanics · Physics 2011-09-08 Asaph Widmer-Cooper , Peter Harrowell

Spherical Janus particles are one of the most prominent examples for active Brownian objects. Here, we study the diffusiophoretic motion of such microswimmers in experiment and in theory. Three stages are found: simple Brownian motion at…

Soft Condensed Matter · Physics 2013-10-08 Xu Zheng , Borge ten Hagen , Andreas Kaiser , Meiling Wu , Haihang Cui , Zhanhua Silber-Li , Hartmut Löwen
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