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Related papers: Density functional theory for a macroion suspensio…

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A classical density functional theory is applied to study solvation of solutes in water. An approx- imate form of the excess functional is proposed for water. This functional requires the knowledge of pure solvent direct correlation…

Chemical Physics · Physics 2014-09-01 Guillaume Jeanmairet

Molecular Dynamics simulations are used to study the effective interactions in charged stabilized colloidal suspensions. For not too high macroion charges and sufficiently large screening, the concept of the potential of mean force is known…

Soft Condensed Matter · Physics 2009-11-11 T. Kreer , J. Horbach , A. Chatterji

Shear thickening of particle suspensions is characterized by a transition between lubricated and frictional contacts between the particles. Using 3D numerical simulations, we study how the inter-particle friction coefficient influences the…

Soft Condensed Matter · Physics 2020-01-08 Vishnu Sivadasan , Eric Lorenz , Alfons G. Hoekstra , Daniel Bonn

It has recently been shown that a free energy for Baxter's sticky hard sphere fluid is uniquely defined within the framework of fundamental measure theory (FMT) for the inhomogeneous hard sphere fluid, provided that it obeys scaled-particle…

Soft Condensed Matter · Physics 2015-06-03 Hendrik Hansen-Goos , Mark A. Miller , J. S. Wettlaufer

The Dean-Kawasaki (DK) equation, which is at the basis of stochastic density functional theory (SDFT), was proposed in the mid-nineties to describe the evolution of the density of interacting Brownian particles, which can represent a large…

Soft Condensed Matter · Physics 2025-05-13 Pierre Illien

We consider the Dean-Kawasaki (DK) equation of overdamped Brownian particles that forms the basis of the stochastic density functional theory. Recently, the linearized DK equation has successfully reproduced the full Onsager theory of…

Statistical Mechanics · Physics 2020-01-07 Hiroshi Frusawa

We use the density functional method to examine the properties of the nonuniform (two-phase) fluid of two-level atoms, a part of which is excited. Basing on the analysis of the equation of state of a gas of two-level atoms, a part of which…

Soft Condensed Matter · Physics 2007-05-23 Oleg Derzhko , Vasyl Myhal

In principle, density functional theory yields the correct ground-state densities and energies of electronic systems under the action of a static external potential. However, traditional approximations fail to include Van der Waals energies…

Condensed Matter · Physics 2016-08-31 Walter Kohn , Yigal Meir , Dmitrii E. Makarov

Transition-metal centers are the active sites for many biological and inorganic chemical reactions. Notwithstanding this central importance, density-functional theory calculations based on generalized-gradient approximations often fail to…

Soft Condensed Matter · Physics 2009-11-11 Heather J. Kulik , Matteo Cococcioni , Damian A. Scherlis , Nicola Marzari

We present a numerical study of dense colloidal suspensions in pressure-driven microchannel flow in two dimensions. The colloids are modeled as elastic and frictional spheres suspended in a Newtonian fluid, which we simulate using the…

Soft Condensed Matter · Physics 2017-08-04 Philipp Kanehl , Holger Stark

Using density functional theory we calculate the density profiles of a binary solvent adsorbed around a pair of big solute particles. All species interact via repulsive Gaussian potentials. The solvent exhibits fluid-fluid phase separation…

Soft Condensed Matter · Physics 2007-05-23 A. J. Archer , R. Evans , R. Roth , M. Oettel

The density functional theory is extended to account for self-bound systems. To this end the Hohenberg-Kohn theorem is formulated for the intrinsic density and a Kohn-Sham like procedure for an $N$--body system is derived using the…

Nuclear Theory · Physics 2008-11-26 Nir Barnea

Soft solids like colloidal glasses exhibit a yield stress, above which the system starts to flow. The microscopic analogon in microrheology is the delocalization of a tracer particle subject to an external force exceeding a threshold value,…

Soft Condensed Matter · Physics 2020-02-05 Markus Gruber , Antonio Manuel Puertas , Matthias Fuchs

Phase separation in a low-density gas-like phase and a high-density liquid-like one is a common trait of biological and synthetic self-propelling particles' systems. The competition between motility and stochastic forces is assumed to fix…

Soft Condensed Matter · Physics 2020-04-15 Pin Nie , Joyjit Chattoraj , Antonio Piscitelli , Patrick Doyle , Ran Ni , Massimo Pica Ciamarra

A discrete--dynamics model, which is specified solely in terms of the system's equilibrium structure, is defined for the density correlators of a simple fluid. This model yields results for the evolution of glassy dynamics which are…

Disordered Systems and Neural Networks · Physics 2011-08-12 T. Franosch , W. Götze , M. R. Mayr , A. P. Singh

The derivation of density functional energies from the random phase approximation of self-consistent mean field theory is generalized and applied to a binary blend of diblock copolymers and homopolymers. A nonlocal transformation is…

Soft Condensed Matter · Physics 2023-07-04 Sulin Wang , Yuan Chen , Zengqiang Tan , Keith Promislow

Statistically studied are the equilibrium characteristics of a subsystem of mobile charges of one sort, taking into account the subsystem of fixed charges of the opposite sign creating a compensating electric background. The distribution of…

Other Condensed Matter · Physics 2019-02-07 H. S. Bokun , D. di Caprio

Electrolyte theories enable to describe the structural and dynamical properties of simple electrolytes in solution, such as sodium chloride in water. Using these theories for aqueous solutions of charged nanoparticles is a straightforward…

Soft Condensed Matter · Physics 2020-02-03 Vincent Dahirel , Olivier Bernard , Marie Jardat

Two forms of relativistic density functional are derived from Dirac equation. Based on their structure analysis model of split electron is proposed. In this model electric charge and mass of electron behave like two point-like particles. It…

Quantum Physics · Physics 2015-05-29 Kirill Koshelev

We present several aspects of the screening of charged macromolecules in an electrolyte. After a review of the basic mean field approach, based on the linear Debye-Huckel theory, we consider the case of highly charged macromolecules, where…

Soft Condensed Matter · Physics 2012-04-27 Gabriel Tellez