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The optical absorption of a single spherical semiconductor quantum dot in an electrical field is studied taking into account the nonlocal coupling between the field of the light and the polarizability of the semiconductor. These nonlocal…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 F. Thiele , Ch. Fuchs , R. v. Baltz

A microscopic theory of optical transitions in quantum dots with carrier-phonon interaction is developed. Virtual transitions into higher confined states with acoustic phonon assistance add a quadratic phonon coupling to the standard linear…

Condensed Matter · Physics 2009-11-10 E. A. Muljarov , R. Zimmermann

Theoretical and numerical calculations of the optical absorption spectra of excitons interacting with longitudinal-optical phonons in quasi-2D polar semiconductors are presented. In II-VI semiconductor quantum wells, exciton binding energy…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 F. J. Rodriguez

A new microscopic approach to the optical transitions in quantum dots and quantum dot molecules, which accounts for both diagonal and non-diagonal exciton-phonon interaction, is developed. The cumulant expansion of the linear polarization…

Other Condensed Matter · Physics 2015-06-25 E. A. Muljarov , T. Takagahara , R. Zimmermann

We investigate a quantum dot (QD) system coupled to a vibrational environment with a super-Ohmic spectral density and weakly to a leaky cavity mode, a model relevant for semiconductor-based single-photon sources. The phonon coupling induces…

Mesoscale and Nanoscale Physics · Physics 2024-12-31 Sebastian Toivonen , Kimmo Luoma

The optical properties of quantum dots embedded in a catalytically grown semiconductor nanowire are studied theoretically. In comparison to dots in a bulk environment, the excitonic absorption is strongly modified by the one-dimensional…

Mesoscale and Nanoscale Physics · Physics 2007-08-22 Greta Lindwall , Andreas Wacker , Carsten Weber , Andreas Knorr

We provide a self-contained review of master equation approaches to modelling phonon effects in optically driven self-assembled quantum dots. Coupling of the (quasi) two-level excitonic system to phonons leads to dissipation and dephasing,…

Mesoscale and Nanoscale Physics · Physics 2016-06-14 Ahsan Nazir , Dara P. S. McCutcheon

Phonons strongly influence the optical control of semiconductor quantum dots. When modeling the electron-phonon interaction in several theoretical approaches the quantum dot geometry is approximated by a spherical structure, though typical…

Mesoscale and Nanoscale Physics · Physics 2018-01-17 S. Lüker , T. Kuhn , D. E. Reiter

Photon absorption in a semiconductor produces bright excitons that recombine very fast into photons. We here show that in a quantum dot set close to a p-doped reservoir, this absorption can produce a dark duo, i.e., an electron-hole pair…

Mesoscale and Nanoscale Physics · Physics 2020-04-22 Shiue-Yuan Shiau , Benoit Eble , Valia Voliotis , Monique Combescot

It is shown that in many cases an adequate description of optical spectra of semiconductor quantum dots requires a treatment beyond the commonly used adiabatic approximation. We have developed a theory of phonon-assisted optical transitions…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 J. T. Devreese , V. M. Fomin , E. P. Pokatilov , V. N. Gladilin , S. N. Klimin

The relaxation of electrons in quantum dots via phonon emission is hindered by the discrete nature of the dot levels (phonon bottleneck). In order to clarify the issue theoretically we consider a system of $N$ discrete fermionic states (dot…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 T. Stauber , R. Zimmermann , H. Castella

The effect of phonons on a nonlinear optical response of a quantum dot-cavity system in quantum strong coupling regime can be accounted for by a fully analytical treatment, provided that the exciton-phonon dynamics is much faster than the…

Mesoscale and Nanoscale Physics · Physics 2023-06-30 L. S. Sirkina , E. A. Muljarov

We find for the first time the ground state energy and the optical absorption spectra for N electrons (holes) interacting with each other and with the longitudinal optical (LO) phonons at an arbitrary electron-phonon coupling strength…

Strongly Correlated Electrons · Physics 2007-05-23 J. T. Devreese , S. N. Klimin , V. M. Fomin , F. Brosens

A detailed analysis of the electro-optical response of single as well as coupled semiconductor quantum dots is presented. This is based on a realistic ---i.e., fully tridimensional--- description of Coulomb-correlated few-electron states,…

Condensed Matter · Physics 2009-11-07 Eliana Biolatti , Irene D'Amico , Paolo Zanardi , Fausto Rossi

Coupling to phonon modes is a primary mechanism of excitonic dephasing and energy loss in semiconductors. However, low-energy phonons in colloidal quantum dots and their coupling to excitons are poorly understood, since their experimental…

Mesoscale and Nanoscale Physics · Physics 2019-10-22 Albert Liu , Diogo B. Almeida , Wan-Ki Bae , Lazaro A. Padilha , Steven T. Cundiff

Polar optical phonons are studied in the framework of the dielectric continuum approach for a prototypical quantum-dot/quantum-well (QD/QW) heterostructure, including the derivation of the electron-phonon interaction Hamiltonian and a…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 F. Comas , Nelson Studart

Multiphonon processes in a model quantum dot (QD) containing two electronic states and several optical phonon modes are considered taking into account both intra- and inter-level terms. The Hamiltonian is exactly diagonalized including a…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 M. I. Vasilevskiy , E. V. Anda , S. S. Makler

We theoretically study the optical properties of an InAs/GaAs quantum dot (QD) near the area of the second-order resonance between an electron confined in the QD and two longitudinal optical phonons. We present the absorption spectra of an…

Mesoscale and Nanoscale Physics · Physics 2015-05-20 Piotr Kaczmarkiewicz , Paweł Machnikowski

Here we embark on a thorough investigation of the magneto-optical absorption in semiconducting {\em spherical} quantum dots characterized by a confining harmonic potential and an applied magnetic field in the symmetric gauge. This is done…

Mesoscale and Nanoscale Physics · Physics 2016-04-13 Manvir S. Kushwaha

A theory of photoluminescence in semiconductor quantum dots is developed which relies on two key ingredients. First, it takes into account non-adiabaticity of the exciton-phonon system. Second, it includes the multimode dielectric model of…

Mesoscale and Nanoscale Physics · Physics 2015-06-24 J. T. Devreese , V. M. Fomin , V. N. Gladilin , S. N. Klimin
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