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Adsorption of para-Hydrogen on the surface of graphite pre-plated with a single layer of atomic krypton is studied thoretically by means of Path Integral Ground State Monte Carlo simulations. We compute energetics and density profiles of…

Statistical Mechanics · Physics 2009-11-11 Joseph Turnbull , Massimo Boninsegni

Molecular dynamics simulation is applied to Poiseuille flow of liquid methane in planar graphite channels, covering channel diameters between 3 and 135 nm. On this length scale, a transition is found between the regime where local ordering…

The molecular dynamics in the ambient-pressure solid phase of (1,1,2)-trichloroethane is studied by means of broadband dielectric spectroscopy and molecular dynamics simulations. The dielectric spectra of polycrystalline samples obtained by…

Molecular dynamics simulations have been performed on pure liquid water, aqueous solutions of sodium chloride, and polymer solutions exposed to a strong external electric field with the goal to gain molecular insight into the structural…

Soft Condensed Matter · Physics 2016-08-08 I. Nezbeda , J. Jirsák , F. Moučka , W. R. Smith

Quantum Monte Carlo simulations at zero temperature of a $^3$He monolayer adsorbed on graphite, either clean or preplated with $^4$He, unexpectedly point to a gas-liquid phase transition at a very low areal density of the order of…

Statistical Mechanics · Physics 2016-03-23 Michele Ruggeri , Ettore Vitali , Davide Emilio Galli , Massimo Boninsegni , Saverio Moroni

Polymer-grafted nanoparticles (PGNPs) can provide property profiles than cannot be obtained individually by polymers or nanoparticles (NPs). Here, we have studied the mixing--demixing transition of symmetric copolymer melts of…

Soft Condensed Matter · Physics 2020-01-23 Peter Yatsyshin , Nikolaos G. Fytas , Panagiotis E. Theodorakis

Pentadiamond is a recently proposed new carbon allotrope consisting of a network of pentagonal rings where both sp$^2$ and sp$^3$ hybridization are present. In this work we investigated the mechanical and electronic properties, as well as,…

The adhesion of flowing particles and biological cells over fixed collecting surfaces is vitally important in diverse situations and potentially controlled by small-scale surface heterogeneity on the particle. Differences in the behavior of…

Soft Condensed Matter · Physics 2015-06-19 Marina Bendersky , Maria M. Santore , Jeffrey M. Davis

Although sheets of layered van der Waals solids offer great opportunities to custom-design nanomaterial properties, their weak interlayer adhesion challenges structural stability against mechanical deformation. Here, bending-induced…

Materials Science · Physics 2013-09-05 Pekka Koskinen

Molecular dynamics simulation have shown that after initial surface melting, nanowires can melt via two mechanisms: an interface front moves towards the wire centre; the growth of an instability at the interface can cause the solid to…

Materials Science · Physics 2022-07-11 Kannan M. Ridings , Shaun C. Hendy

We performed first-principles molecular dynamics calculations for lithium using the projector augmented waves method and the generalized gradient approximation as exchange-correlation energy. The melting curve of lithium was computed using…

Materials Science · Physics 2010-10-13 Dafang Li , Ping Zhang , Jun Yan

Multilayer sorption isotherms of 1-propanol on graphite have been measured by means of high-resolution ellipsometry within the liquid regime of the adsorbed film for temperatures ranging from 180 to 260 K. In the first three monolayers the…

Chemical Physics · Physics 2015-03-19 Matthias Wolff , Frank Kruchten , Patrick Huber , Klaus Knorr , Ulrich G. Volkmann

Melting in two-dimensional systems has remained controversial as theory, simulations, and experiments show contrasting results. One issue that obscures this discussion is whether or not theoretical predictions on strictly 2D systems…

Soft Condensed Matter · Physics 2014-07-11 Weikai Qi , Anjan P. Gantapara , Marjolein Dijkstra

We present in this contribution a theoretical investigation of the spontaneous emission and energy transfer rates between quantum systems placed above a monolayer of conducting graphene. The conditions for strong and weak coupling between a…

The rate of melting of a solid and the rate of deformation of the resulting melt due to capillary forces are comparable in additive manufacturing applications. This dynamic structural change of a melting solid is extremely challenging to…

Computational Physics · Physics 2018-04-18 Michael Blank , Prapanch Nair , Thorsten Pöschel

We consider thermodynamic and dynamic phase transitions in plaquette spin models of glasses. The thermodynamic transitions involve coupled (annealed) replicas of the model. We map these coupled-replica systems to a single replica in a…

Statistical Mechanics · Physics 2015-08-19 Robert M. Turner , Robert L. Jack , Juan P. Garrahan

We investigate the crystallization of crosslinked and entangled polymers under external deformation using a coarse-grained poly(vinyl alcohol) (CG-PVA) model and molecular dynamics simulations. Following uniaxial deformation, the systems…

Soft Condensed Matter · Physics 2026-01-19 Atmika Bhardwaj , Huzaifa Shabbir , Jens-Uwe Sommer , Marco Werner

The crystal-melt interfaces of a binary hard-sphere fluid mixture in coexistence with a single-component hard-sphere crystal is investigated using molecular-dynamics simulation. In the system under study, the fluid phase consists of a…

Chemical Physics · Physics 2009-11-07 Rachel Sibug-Aga , Brian B. Laird

We report high-precision heat-capacity measurements of submonolayer $^3$He adsorbed on highly crystalline graphite, revealing new aspects of the commensurate$-$incommensurate transition. Below 1\~K, two possible striped domain-wall phases…

Other Condensed Matter · Physics 2026-03-12 A. Kumashita , J. Usami , S. Komatsu , Y. Yamane , S. Miyasaka , H. Fukuyama , A. Yamaguchi

We perform a femtosecond-THz optical pump-probe spectroscopy to investigate the cooling dynamics of hot carriers in quasi-free standing bilayer epitaxial graphene. We observed longer decay time constants, in the range of 2.6 to 6.4 ps,…

Mesoscale and Nanoscale Physics · Physics 2023-02-03 Sachin Sharma , Rachael L. Myers-Ward , David Kurt Gaskill , Ioannis Chatzakis