Related papers: Explanation of quantum dot blinking without long-l…
Colloidal semiconductor quantum dots (QDs) are excellent luminescent nanomaterials for a broad range of optoelectronic applications. Their photoluminescence blinking, however, hinders their practical use in many aspects. It has been shown…
The observed intermittent light emission from colloidal semiconductor nanocrystals has long been associated with Auger recombination assisted quenching. We test this view by observing transient emission dynamics of CdSe/CdS/ZnS…
The photoluminescence intermittency (blinking) of quantum dots is interesting because it is an easily-measured quantum process whose transition statistics cannot be explained by Fermi's Golden Rule. Commonly, the transition statistics are…
We study time series produced by the blinking quantum dots, by means of an aging experiment, and we examine the results of this experiment in the light of two distinct approaches to complexity, renewal and slow modulation. We find that the…
Three models of single colloidal quantum dot emission fluctuations (blinking) based on spectral diffusion were considered analytically and numerically. It was shown that the only one of them, namely the Frantsuzov and Marcus model…
We theoretically investigate the spectrum of the fluorescence from triple quantum-dot molecules and demonstrate that it is possible to use tunneling to induce dark states. Unlike the atomic system, in quantum-dot molecules we can use…
Photo-luminescence intermittency (blinking) in semiconductor nanocrystals (NCs), a phenomenon ubiquitous to single-emitters, is generally considered to be temporally random intensity fluctuations between bright (On) and dark (Off) states.…
We demonstrate that the cycling between internal states of quantum dots during fluorescence blinking can be used to tune the near-field coupling with a sharp tip. In particular, the balance between tip-induced field enhancement and energy…
Tunneling excitations of electrons in dry-etched modulation-doped AlGaAs/GaAs coupled quantum dots (QDs) are probed by resonant inelastic light scattering. A sequence of intra- and intershell excitations are found at energies determined by…
We demonstrate the extension of coherence between all four two-electron spin ground states of an InAs quantum dot molecule (QDM) via non-local suppression of nuclear spin fluctuations in both constituent quantum dots (QDs), while optically…
In quantum dots (QDs) the Auger recombination is a non-radiative process, where the electron-hole recombination energy is transferred to an additional carrier. It has been studied mostly in colloidal QDs, where the Auger recombination time…
We theoretically analyze the scattering process of an electron on a graphene quantum dot (GQD) exposed to an external light irradiation. We prove that for suitable choices of the light polarization state, there emerge scattering resonances,…
Colloidal core/shell InP/ZnSe quantum dots (QDs), recently produced using an improved synthesis method, have a great potential in life-science applications as well as in integrated quantum photonics and quantum information processing as…
A quantum cascade laser where the quantum wells in the active regions are replaced by quantum dots with their atom-like discrete energy levels is an interesting system to study novel features in optical spectroscopy. We study structures…
Recently we predicted a random blinking, i.e. macroscopic quantum jumps, in the fluorescence of a laser-driven atom-cavity system [Metz et al., Phys. Rev. Lett. 97, 040503 (2006)]. Here we analyse the dynamics underlying this effect in…
We discuss the possibility of non-exponential Auger decay of atoms irradiated by X-ray photons. This effect can occur at times, which are greater than the lifetime of a system under consideration. The mechanism for non-exponential depletion…
The problems of the luminescent enhancement and life time shortening for the inverted quantum system (QS) are analysed. The commonly accepted in publications approach appears to be questionable from the point of view of basic principles. An…
We study the localization of dressed Dirac electrons in a cylindrical quantum dot (QD) formed on monolayer and bilayer graphene by spatially different potential profiles. Short lived excitonic states which are too broad to be resolved in…
Bistability in quantum dot structures is examined by a drift-diffusion model in combination with electron capture and emission processes. Our simulations provide a dynamic scenario with extremely long switching times of the order of months…
Photoluminescence (PL) intermittency is a ubiquitous phenomenon detrimentally reducing the temporal emission intensity stability of single colloidal quantum dots (CQDs) and the emission quantum yield of their ensembles. Despite efforts for…