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We discuss the factors that determine the overall shape and magnitude of the current-voltage (I-V) characteristics of a variety of molecular conductors sandwiched between two metallic contacts. We analyze the individual influences of the…

Mesoscale and Nanoscale Physics · Physics 2016-08-31 A. W. Ghosh , S. Datta

In recent years, several experimental groups have reported measurements of the current-voltage (I-V) characteristics of individual or small numbers of molecules. Our purpose in this chapter is to provide an intuitive explanation for the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Magnus Paulsson , Ferdows Zahid , Supriyo Datta

We present current-voltage (I-V) curves computed using all-electron basis sets on the conducting molecule. The all-electron results are very similar to previous results obtained using effective core potentials (ECP). A hybrid integration…

Mesoscale and Nanoscale Physics · Physics 2015-06-25 Charles W. Bauschlicher, , John W. Lawson

We investigate the origin of asymmetry in the measured current-voltage (I-V) characteristics of molecules with no inherent spatial asymmetry. We establish that such molecules can exhibit asymmetric I-V characteristics due to unequal…

Mesoscale and Nanoscale Physics · Physics 2016-08-31 Avik W. Ghosh , Ferdows Zahid , Prashant S. Damle , Supriyo Datta

We investigate the origin of asymmetry in various measured current-voltage (I-V) characteristics of molecules with no inherent spatial asymmetry, with particular focus on a recent break junction measurement. We argue that such asymmetry…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 F. Zahid , A. W. Ghosh , M. Paulsson , E. Polizzi , S. Datta

We report first-principles calculations of the inelastic current-voltage (I-V) characteristics of a gold point contact and a molecular junction in the nonresonant regime. Discontinuities in the I-V curves appear in correspondence to the…

Mesoscale and Nanoscale Physics · Physics 2015-06-24 Yu-Chang Chen , Michael Zwolak , Massimiliano Di Ventra

In bulk systems, molecules are routinely identified by their vibrational spectrum using Raman or infrared spectroscopy. In recent years, vibrational excitation lines have been observed in low-temperature conductance measurements on single…

Mesoscale and Nanoscale Physics · Physics 2010-02-25 Johannes S. Seldenthuis , Herre S. J. van der Zant , Mark A. Ratner , Joseph M. Thijssen

We investigate electronic transport through two types of conjugated molecules. Mechanically controlled break-junctions are used to couple thiol endgroups of single molecules to two gold electrodes. Current-voltage characteristics (IVs) of…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 J. Reichert , R. Ochs , D. Beckmann , H. B. Weber , M. Mayor , H. v. Loehneysen

We show that the nonlinear I-V characteristics of mesoscopic samples with metallic conductivity should contain parts which are linear in the magnetic field and quadratic in the electric field. These contributions to the current are entirely…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 B. Spivak , A. Zyuzin

The i-V curve describes the current drawn from a flame as a function of the voltage difference applied across the reaction zone. Since combustion diagnostics and flame control strategies based on electric fields depend on the amount of…

Chemical Physics · Physics 2016-07-20 Jie Han , Memdouh Belhi , Tiernan A. Casey , Fabrizio Bisetti , Hong G. Im , Jyh-Yuan Chen

We present an atomistic theory of electronic transport through single organic molecules that reproduces the important features of the current-voltage characteristics observed in recent experiments. We trace these features to their origin in…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 J. Heurich , J. C. Cuevas , W. Wenzel , G. Schoen

By use of the multi-Josephson junction model, we investigate voltage-biased I-V characteristics. Differently from the case of the single junction, I-V characteristics show a complicated behavior due to inter-layer couplings among…

Superconductivity · Physics 2009-10-31 S. Sakamoto , H. Matsumoto , T. Koyama , M. Machida

A self-consistent method for calculating electron transport through a molecular device is proposed. It is based on density functional theory electronic structure calculations under periodic boundary conditions and implemented in the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 San-Huang Ke , Harold U. Baranger , Weitao Yang

We provide analytical results for the perturbative correction to the current-voltage relation through a vibrating molecule for weak electron-phonon coupling. The nonlinear conductance exhibits a step-like feature at $eV=\hbar \omega_0$,…

Mesoscale and Nanoscale Physics · Physics 2008-03-14 R. Egger , A. O. Gogolin

This article proposes that we should think differently about predicting and interpreting measured field electron emission (FE) current-voltage [I(V)] characteristics. It is commonly assumed that I(V) data interpretation is a problem in…

Mesoscale and Nanoscale Physics · Physics 2023-03-22 Richard G. Forbes

The proposed protocol is an attempt to meet the experimentalists' legitimate desire of reliably and easily extracting microscopic parameters from current-voltage measurements on molecular junctions. It applies to junctions wherein charge…

Mesoscale and Nanoscale Physics · Physics 2024-02-27 Ioan Baldea

The coupling of the charge carriers passing through a molecule bridging two bulky conductors with local vibrational modes of the molecule, gives rise to distinct features in the electronic transport properties on one hand, and to…

Mesoscale and Nanoscale Physics · Physics 2017-02-01 A. Ueda , Y. Utsumi , Y. Tokura , O. Entin-Wohlman , A. Aharony

An analytic approach to the electron transport phenomena in molecular devices is presented. Analyzed devices are composed of organic molecules attached to the two semi-infinite electrodes. Molecular system is described within the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Kamil Walczak

We report a charge based model to establish the analytical equation, describing the nature of capacitance-voltage ($C$-$V$) characteristics of organic solar cells under dark condition (or organic diodes) over a wide range of voltage,…

Applied Physics · Physics 2018-09-25 Prashanth Kumar Manda , Soumya Dutta

The nonlinear I-V characteristics of mesoscopic samples contain parts which are linear in the magnetic field and quadratic in the electric field. These contributions to the current are entirely due to the electron-electron interaction and…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 E. Deyo , B. Spivak , A. Zyuzin
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