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Related papers: Ultrafast dynamics of coherent optical phonons and…

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Anharmonic decay of coherent optical phonons in semimetal Sb has been investigated by using a femtosecond pump-probe technique. The coherent $A_{1g}$ mode is observed in time domain in a wide temperature range of 7 - 290 K. The decay rate…

Materials Science · Physics 2015-01-12 Muneaki Hase , Kiminori Ushida , Masahiro Kitajima

Ultrafast laser measurements probe the non-equilibrium dynamics of excited electrons in metals with increasing temporal resolution. Electronic structure calculations can provide a detailed microscopic understanding of hot electron dynamics,…

Computational Physics · Physics 2016-08-12 Ana M. Brown , Ravishankar Sundararaman , Prineha Narang , William A. Goddard , Harry A. Atwater

We report the lattice dynamics of transition metal thin films by using the ultrafast electron diffraction. We observe a suppression of the diffraction intensity in a few picosecond after the photoexcitation, which is directly interpreted as…

Materials Science · Physics 2016-01-19 A. Nakamura , T. Shimojima , M. Nakano , Y. Iwasa , K. Ishizaka

We investigate the excitation of phonons in photoexcited antimony and demonstrate that the entire electron-lattice interactions, in particular coherent and incoherent electron-phonon coupling, can be probed simultaneously. Using femtosecond…

Quantitative knowledge of electron-phonon coupling is important for many applications as well as for the fundamental understanding of nonequilibrium relaxation processes. Time-resolved diffraction provides direct access to this knowledge…

Materials Science · Physics 2021-11-18 Daniela Zahn , Hélène Seiler , Yoav William Windsor , Ralph Ernstorfer

The advent of pump-probe spectroscopy techniques paved the way to the exploration of the ultrafast dynamics of electrons and phonons in crystalline solids. Following photo-absorption of a pump pulse and the initial electronic…

Materials Science · Physics 2023-07-14 Fabio Caruso , Dino Novko

We employed femtosecond time- and angle-resolved photoelectron spectroscopy to analyze the response of the electronic structure of the 122 Fe-pnictide parent compounds Ba/EuFe_2As_2 and optimally doped BaFe_{1.85}Co_{0.15}As_2 near the…

High-resolution angle-resolved photoemission spectroscopy and ultrafast optical pump-probe spectroscopy were used to study semimetallic 1T - TiTe2 quasiparticle dispersion and dynamics. A kink and a flat band, having the same energy scale…

Femtosecond dynamics of coherent optical phonons in GeTe/Sb$_{2}$Te$_{3}$ superlattices (SLs), a new class of semiconductor SLs with three different states, have been investigated by using a reflection-type pump-probe technique at various…

Materials Science · Physics 2015-03-23 Muneaki Hase , Yoshinobu Miyamoto , Junji Tominaga

Transient responses of the electronic excitation and coherent soft phonon are investigated both above and below the ferroelectric phase transition temperature T$_{c}$ in Pb$_{1-x}$Ge$_{x}$Te by using an optical pump-probe technique. The…

Materials Science · Physics 2007-05-23 Rong Lu , Muneaki Hase , Masahiro Kitajima , Shinichi Nakashima , Shunji Sugai

Utilizing femtosecond optical pump-probe technique, we have studied transient Fano-resonance in zinc. At high excitation levels the Fourier spectrum of the coherent E$_{2g}$ phonon exhibits strongly asymmetric line shape, which is well…

Strongly Correlated Electrons · Physics 2007-05-23 Muneaki Hase , Jure Demsar , Masahiro Kitajima

The strength of the electron-phonon coupling parameter and its evolution throughout a solid's phase diagram often determines phenomena such as superconductivity, charge- and spin-density waves. Its experimental determination relies on the…

Ultrafast dynamics of graphite is investigated by time-resolved photoemission spectroscopy. We observe spectral features of direct photoexcitations, non-thermal electron distributions, and recovery dynamics occurring with two time scales…

Materials Science · Physics 2011-08-24 Y. Ishida , T. Togashi , K. Yamamoto , M. Tanaka , T. Taniuchi , T. Kiss , M. Nakajima , T. Suemoto , S. Shin

Radio-frequency compressed ultrafast electron diffraction has been used to probe the coherent and incoherent coupling of impulsive electronic excitation at 1.55 eV (800 nm) to optical and acoustic phonon modes directly from the perspective…

Materials Science · Physics 2015-06-23 Robert P. Chatelain , Vance R. Morrison , Bart L. M. Klarenaar , Bradley J. Siwick

Multi-temperature models are nowadays often used to quantify the ultrafast electron-phonon (boson) relaxations and coupling strengths in advanced quantum solids. To test their applicability we study the time evolution of the electron…

Materials Science · Physics 2020-01-29 Manuel Obergfell , Jure Demsar

The rate of energy transfer between electrons and phonons is investigated by a first principles framework for electron temperatures up to $T_e=50000$ K while considering the lattice at ground state. Two typical but differently complex…

Other Condensed Matter · Physics 2022-03-08 Jia Zhang , Rui Qin , Wenjun Zhu , Jan Vorberger

The electron-phonon coupling in ultrafast heating systems is studied within the framework of Boltzmann transport equation (BTE) with coupled electron and phonon transport. A discrete unified gas kinetic scheme is developed to solve the BTE,…

Mesoscale and Nanoscale Physics · Physics 2023-08-25 Chuang Zhang , Rulei Guo , Meng Lian , Junichiro Shiomi

Ultrafast optical pump-probe spectroscopy is used to track carrier dynamics in the large magnetoresistance material WTe$_{2}$. Our experiments reveal a fast relaxation process occurring on a sub-picosecond time scale that is caused by…

We use ultrafast optical spectroscopy to investigate the electronic and lattice dynamics of the charge-density wave (CDW) material 1$T$-TiSe$_2$ across various temperatures and pump fluences. We reveal a close relationship between the…

Strongly Correlated Electrons · Physics 2026-04-28 Xue-Qing Ye , Hao Liu , Qi-Yi Wu , Chen Zhang , Xiao-Fang Tang , Bo Chen , Chuan-Cun Shu , Hai-Yun Liu , Yu-Xia Duan , Peter M. Oppeneer , Jian-Qiao Meng

We report temperature evolution of coherently excited acoustic and optical phonon dynamics in superconducting iron pnictide single crystal Ca(Fe_0.944Co_0.056)_2As_2 across the spin density wave transition at T_SDW ~ 85 K and…

Strongly Correlated Electrons · Physics 2012-12-14 Sunil Kumar , L. Harnagea , S. Wurmehl , B. Buchner , A. K. Sood
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