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In many quantum magnets especially the rare-earth ones, the low-lying crystal field states are not well separated from the excited ones and thus are insufficient to describe the low-temperature magnetic properties. Inspired by this simple…

Strongly Correlated Electrons · Physics 2019-06-12 Changle Liu , Fei Ye Li , Gang Chen

Processes occurring in the strong-field regime of QED are characterized by background electromagnetic fields of the order of the critical field $F_{cr}=m^2c^3/\hbar|e|$ in the rest frame of participating charges. It has been conjectured…

High Energy Physics - Phenomenology · Physics 2020-02-05 A. Di Piazza , T. N. Wistisen , M. Tamburini , U. I. Uggerh\{o}j

We apply the first-principles density functional theory + dynamical mean field theory framework to evaluate the crystal field splitting on rare earth sites in hard magnetic intermetallics. An atomic (Hubbard-I) approximation is employed for…

Strongly Correlated Electrons · Physics 2017-11-15 Pascal Delange , Silke Biermann , Takashi Miyake , Leonid Pourovskii

Neutron time-of-flight spectroscopy has been employed to study the crystal-field splitting of Pr$^{3+}$ in the pyrochlore stannate Pr$_{2}$Sn$_{2}$O$_{7}$. The crystal field has been parameterized from a profile fit to the observed neutron…

Strongly Correlated Electrons · Physics 2013-10-28 A. J. Princep , D. Prabhakaran , A. T. Boothroyd , D. T. Adroja

In a recent study of the magnetic properties of rare-earth systems the two extreme situations have been considered in which the crystalline electrostatic field is large or small with respect to the spin-orbit interaction. In the first case…

Strongly Correlated Electrons · Physics 2010-08-17 Keisuke Hatada , Kuniko Hayakawa , Fabrizio Palumbo

We present a crystal field theory of transition metal impurities in semiconductors in a trigonally distorted tetrahedral coordination. We develop a perturbative scheme to treat covalency effects within the weak ligand field case (Coulomb…

Strongly Correlated Electrons · Physics 2009-11-11 R. O. Kuzian , A. M. Daré , P. Sati , R. Hayn

It has been shown that the crystal-field interactions can produce a non- magnetic singlet ground state for the highly-correlated d6 system situated in the quasi-octahedral crystal field (CEF) surrounding provided the spin-orbit interactions…

Strongly Correlated Electrons · Physics 2009-10-31 R. J. Radwanski , Z. Ropka

We introduce a phase-field crystal model that creates an array of complex three- and two-dimensional crystal structures via a numerically tractable three-point correlation function. The three-point correlation function is designed in order…

Materials Science · Physics 2017-11-15 Eli Alster , David Montiel , Katsuyo Thornton , Peter W. Voorhees

The existence of CEF states and the magnetism in conducting compounds NdAl2, UPd2Al3 and YbRh2Si2 is discussed. We point out that in metallic compounds localized crystal-field states coexist with conduction electrons. These compounds are…

Strongly Correlated Electrons · Physics 2008-10-08 R. J. Radwanski Z. Ropka

Evidence is summarized attesting that the standard exchange field theory of ferromagnetism by Heisenberg has not been successful. It is replaced by the crystal field and a simple assumption that spin orientation is inexorably associated…

General Physics · Physics 2011-06-21 Yuri Mnyukh

Rare-earth (RE) based compounds and alloys are of great interest both for their fundamental physical properties and for applications. In order to tailor the required compounds for a specific task, one must be able to predict the energy…

Condensed Matter · Physics 2007-05-23 Nicola Magnani

In a recent class of phase field crystal (PFC) models, the density order parameter is coupled to powers of its mean field. This effectively introduces a phenomenology of higher-order direct correlation functions acting on long wavelengths,…

Materials Science · Physics 2024-08-21 Daniel L. Coelho , Duncan Burns , Emily Wilson , Nikolas Provatas

On the basis of the point charge model, we formulate the crystalline electronic field (CEF) Hamiltonian $H_{\rm CEF}$ in the rare-earth based quasicrystal (QC) and approximant crystal (AC) with ligand ions located at pseudo 5-fold…

Strongly Correlated Electrons · Physics 2022-03-22 Shinji Watanabe , Mina Kawamoto

In materials science the phase field crystal approach has become popular to model crystallization processes. Phase field crystal models are in essence Landau-Ginzburg-type models, which should be derivable from the underlying microscopic…

Soft Condensed Matter · Physics 2013-05-30 M. Oettel , S. Dorosz , M. Berghoff , B. Nestler , T. Schilling

As a possible mechanism of the $\gamma-\alpha$ phase transition in pristine cerium a change of the electronic density from a disordered state with symmetry Fm-3m to an ordered state Pa-3 has been proposed. Here we include on-site and inter-…

Strongly Correlated Electrons · Physics 2009-11-07 A. V. Nikolaev , K. H. Michel

The choice that a solid system "makes" when adopting a crystal structure (stable or metastable) is ultimately governed by the interactions between electrons forming chemical bonds. By analyzing 6 prototypical binary transition-metal…

Strongly Correlated Electrons · Physics 2019-10-29 Nicola Lanatà , Tsung-Han Lee , Yong-Xin Yao , Vladan Stevanović , Vladimir Dobrosavljević

These are introductory lectures to some aspects of the physics of strongly correlated electron systems. I first explain the main reasons for strong correlations in several classes of materials. The basic principles of dynamical mean-field…

Strongly Correlated Electrons · Physics 2009-09-29 Antoine Georges

The ground state spin of the negatively charged nitrogen-vacancy center in diamond has been the platform for the recent rapid expansion of new frontiers in quantum metrology and solid state quantum information processing. In ambient…

Materials Science · Physics 2012-06-05 M. W. Doherty , F. Dolde , H. Fedder , F. Jelezko , J. Wrachtrup , N. B. Manson , L. C. L. Hollenberg

Metal-insulator transitions driven by magnetic fields have been extensively studied in 2D, but a 3D theory is still lacking. Motivated by recent experiments, we develop a scaling theory for the metal-insulator transitions in the…

Mesoscale and Nanoscale Physics · Physics 2021-07-29 Peng-Lu Zhao , Hai-Zhou Lu , X. C. Xie

Exploring new parameter regimes to realize and control novel phases of matter has been a main theme in modern condensed matter physics research. The recent discovery of 2D magnetism in nearly freestanding monolayer atomic crystals has…