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Related papers: Current-induced nonequilibrium vibrations in singl…

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The realization of molecular-based electronic devices depends to a large extent on the ability to mechanically stabilize the involved molecular bonds, while making use of efficient resonant charge transport through the device. Resonant…

Mesoscale and Nanoscale Physics · Physics 2018-09-11 David Gelbwaser-Klimovsky , Alán Aspuru-Guzik , Michael Thoss , Uri Peskin

Quantum interference effects and decoherence mechanisms in single-molecule junctions are analyzed employing a nonequilibrium Green's function approach. Electrons tunneling through quasi-degenerate states of a nanoscale molecular junction…

Mesoscale and Nanoscale Physics · Physics 2011-07-25 R. Härtle , M. Butzin , O. Rubio-Pons , M. Thoss

Comprehending nonequilibrium electron-phonon dynamics at the microscopic level and at the short time scales is one of the main goals in condensed matter physics. Effective temperature models and time-dependent Boltzmann equations are…

Materials Science · Physics 2023-08-07 Nina Girotto , Fabio Caruso , Dino Novko

Based on quantum theory, we investigate the distribution of the electrons scattered in nonlinear Compton effect by an electromagnetic plane wave. Deviations of the final electron momentum from its initial value are solely due to quantum…

Atomic Physics · Physics 2015-06-05 Madalina Boca , Victor Dinu , Viorica Florescu

Interactions between mesoscopic devices induced by interface acoustic phonons propagating in the plane of a two-dimensional electron system (2DES) are investigated by phonon-spectroscopy. In our experiments ballistic electrons injected from…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 G. J. Schinner , H. P. Tranitz , W. Wegscheider , J. P. Kotthaus , S. Ludwig

Current-induced bond rupture is a fundamental process in nanoelectronic architectures such as molecular junctions and in scanning tunneling microscopy measurements of molecules at surfaces. The understanding of the underlying mechanisms is…

Mesoscale and Nanoscale Physics · Physics 2023-07-26 Yaling Ke , Jan Dvořák , Martin Čížek , Raffaele Borrelli , Michael Thoss

Electron transport in a self-consistent potential along a ballistic two-terminal conductor has been investigated. We have derived general formulas which describe the nonlinear current-voltage characteristics, differential conductance, and…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 O. M. Bulashenko , J. M. Rubi

Current-voltage characteristics of a single-electron transistor with a vibrating quantum dot were calculated assuming vibrons to be in a coherent (non-equilibrium) state. For a large amplitude of quantum dot oscillations we predict strong…

Mesoscale and Nanoscale Physics · Physics 2021-12-01 O. M. Bahrova , S. I. Kulinich , I. V. Krive

We reformulate and extend porous electrode theory for non-ideal active materials, including those capable of phase transformations. Using principles of non-equilibrium thermodynamics, we relate the cell voltage, ionic fluxes, and Faradaic…

Chemical Physics · Physics 2012-08-24 Todd R. Ferguson , Martin Z. Bazant

We calculate the phonons in a graphene nanoconstriction(GNC) in the presence of a high current density. The Joule-heating, current-induced forces, and coupling to electrode phonons is evaluated using first principles nonequilibrium DFT-NEGF…

Mesoscale and Nanoscale Physics · Physics 2014-03-18 Tue Gunst , Jing-Tao Lü , Per Hedegård , Mads Brandbyge

We consider the excitation of single-electron wave packets by means of a time dependent voltage applied to the ballistic edge channels of the integer quantum Hall effect at filling factor $\nu=2$. Due to electron-electron interactions,…

Mesoscale and Nanoscale Physics · Physics 2018-07-23 Matteo Acciai , Matteo Carrega , Jérôme Rech , Thibaut Jonckheere , Thierry Martin , Maura Sassetti

We investigate the transient effects occurring in a molecular quantum dot described by an Anderson-Holstein Hamiltonian which is instantly coupled to two fermionic leads biased by a finite voltage. In the limit of weak electron-phonon…

Mesoscale and Nanoscale Physics · Physics 2010-03-30 R. -P. Riwar , T. L. Schmidt

We investigate the electron transport properties of a model magnetic molecule formed by two magnetic centers whose exchange coupling can be altered with a longitudinal electric field. In general we find a negative differential conductance…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 Sujeet K. Shukla , Stefano Sanvito

The effect of non-equilibrium constraints and dephasing on the circulating currents in molecular junctions are analyzed. Circulating currents are manifestations of quantum effects and can be induced either by externally applied bias or an…

Mesoscale and Nanoscale Physics · Physics 2016-09-28 Hari Kumar Yadalam , Upendra Harbola

We present a combined treatment of the non-equilibrium dynamics and transport of electrons and phonons by carrying out \textit{ab initio} calculations of the fully coupled electron and phonon Boltzmann transport equations. We find that the…

Materials Science · Physics 2020-12-30 Nakib H. Protik , Boris Kozinsky

We propose a mechanism which allows one to control the transmission of single electrons through a molecular junction. The principle utilizes the emergence of transmission sidebands when molecular vibrational modes are coupled to the…

Mesoscale and Nanoscale Physics · Physics 2010-03-26 Thomas Olsen , Jakob Schiøtz

Effects related with deviations from thermodynamic equilibrium take a special place in the modern physics. Among those, non-equilibrium phenomena in quantum systems attract the highest interest. To date, the experimental technique of spin…

Mesoscale and Nanoscale Physics · Physics 2016-06-22 M. M. Glazov

The thermal, mechanical, and electronic performance of atomically thin semiconductors is governed by their low-energy phonons, yet the impact of atomic-scale disorder on these modes remains poorly understood. Here, we report the first…

Materials Science · Physics 2026-01-22 Aleksandar Radic , Boyao Liu , Akshay Rao , Sam Lambrick

Together with their fingerprint modes, molecules carry coherent vibrations of all their atoms (phonons). Phonon spectra extend from $\sim$20 to more than $10^{4}\,\mu$m, depending on molecular size. These spectra are discrete but large…

Astrophysics of Galaxies · Physics 2015-05-20 Renaud Papoular

We investigate on the same footing the time-dependent electronic transport properties and vibrational dynamics of a molecular junction. We show that fluctuations of both the molecular vibron displacement and the electronic current across…

Mesoscale and Nanoscale Physics · Physics 2019-03-27 Rémi Avriller , R Souto , A. Martin-Rodero , A Yeyati