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The structure of liquid water at ambient conditions is studied in ab initio molecular dynamics simulations using van der Waals (vdW) density-functional theory, i.e. using the new exchange-correlation functionals optPBE-vdW and vdW-DF2.…

The central topic of this letter is to show that light-matter hybridization not only gives rise to novel dynamic responses but can also modify intermolecular interactions and induce new structural order. Using the van der Waals (vdW) system…

Quantum Physics · Physics 2023-10-20 Jianshu Cao , Eli Pollak

We present results for a density functional theory study of small water clusters and hexagonal ice Ih, using the van der Waals density functional (vdW-DF). In particular, we examine energetic, structural, and vibrational properties of these…

Soft Condensed Matter · Physics 2011-07-20 Brian Kolb , T. Thonhauser

We investigate the van der Waals interactions in solid molecular hydrogen structures. We calculate enthalpy and the Gibbs free energy to obtain zero and finite temperature phase diagrams, respectively. We employ density functional theory…

Materials Science · Physics 2019-05-10 Sam Azadi , Graeme J. Ackland

Diffusion processes govern fundamental phenomena such as phase transformations, doping, and intercalation in van der Waals (vdW) bonded materials. Here, we quantify the diffusion dynamics of W atoms by visualizing the motion of individual…

A thermal model of kinetic friction is assigned to a classical loaded particle moving on a fluctuating smooth surface. A sinusoidal wave resembles surface fluctuations with a relaxation time. The Hamiltonian is approximated to the mean…

Mesoscale and Nanoscale Physics · Physics 2023-05-08 Rasoul Kheiri

We present a new scheme to include the van der Waals (vdW) interactions in approximated Density Functional Theory (DFT) by combining the Quantum Harmonic Oscillator model with the Maximally Localized Wannier Function technique. With respect…

Materials Science · Physics 2015-06-16 Pier Luigi Silvestrelli

In principle, density functional theory yields the correct ground-state densities and energies of electronic systems under the action of a static external potential. However, traditional approximations fail to include Van der Waals energies…

Condensed Matter · Physics 2016-08-31 Walter Kohn , Yigal Meir , Dmitrii E. Makarov

Repulsive short-range and attractive long-range van der Waals (vdW) forces have an appreciable role in the behavior of extended molecular systems. When using empirical force fields - the most popular computational methods applied to such…

Chemical Physics · Physics 2023-09-27 Almaz Khabibrakhmanov , Dmitry V. Fedorov , Alexandre Tkatchenko

Fluctuations exist in any material object $A$. If $A$ has non-zero temperature $T$, one speaks about thermal fluctuations. If $A$ is at very low $T$, the fluctuations are of quantum origin. Interesting effects appear if two bodies $A$ and…

Statistical Mechanics · Physics 2025-09-30 Daniel Dantchev , Nicholay Tonchev

The characteristic function for the joint measurement of the changes of two commuting observables upon an external forcing of a quantum system is derived. In particular, the statistics of the internal energy, the exchanged heat and the work…

Statistical Mechanics · Physics 2009-02-18 Peter Talkner , Michele Campisi , Peter Hänggi

Noncovalent van der Waals (vdW) interactions are responsible for a wide range of phenomena in matter. Popular density-functional methods that treat vdW interactions use disparate physical models for these intricate forces, and as a result…

Materials Science · Physics 2020-04-15 Jan Hermann , Alexandre Tkatchenko

We consider the the van der Waals force involving excited atoms in general environments, constituted by magnetodielectric bodies. We develop a dynamical approach studying the dynamics of the atoms and the field, mutually coupled. When only…

Quantum Physics · Physics 2017-02-24 Pablo Barcellona , Roberto Passante , Lucia Rizzuto , Stefan Yoshi Buhmann

It is known that ab initio molecular dynamics (AIMD) simulations of liquid water, based on the generalized gradient approximation (GGA) to density functional theory (DFT), yield structural and diffusive properties in reasonable agreement…

Materials Science · Physics 2015-05-19 Jue Wang , G. Roman-Perez , Jose M. Soler , Emilio Artacho , M. -V. Fernandez-Serra

We consider a single slight protuberance in a perfectly conducting plane, and investigate the van der Waals (vdW) interaction between this surface and a neutral polarizable particle. When the protuberance is sufficiently smooth, so that the…

Quantum Physics · Physics 2022-07-13 Edson C. M. Nogueira , Lucas Queiroz , Danilo T. Alves

It is shown that if kinetics of quantum transitions takes account of energy uncertainty of intermediate states, then it creates non-decaying correlations and non-averagable (flicker) fluctuations in the energy as well as in rates of…

Statistical Mechanics · Physics 2018-12-21 Yuriy E. Kuzovlev

The study of van der Waals (vdW) materials has seen increased interest in recent years, due to the wide range of uses for these materials because of their unique mechanical, electronic, and optical properties. This area has recently…

Mesoscale and Nanoscale Physics · Physics 2023-11-02 Sivakumar Vishnuvardhan Mambakkam , Stephanie Law

We examine whether fluctuation-induced forces can lead to stable levitation. First, we analyze a collection of classical objects at finite temperature that contain fixed and mobile charges, and show that any arrangement in space is unstable…

Quantum Physics · Physics 2014-11-20 Sahand Jamal Rahi , Mehran Kardar , Thorsten Emig

The theoretical description of sparse matter attracts much interest, in particular for those ground-state properties that can be described by density functional theory (DFT). One proposed approach, the van der Waals density functional…

We derive the fluctuation theorem for quantum-state statistics that can be obtained when we initially measure the total energy of a quantum system at thermal equilibrium, let the system evolve unitarily, and record the quantum-state data…

Statistical Mechanics · Physics 2018-08-01 Naoto Tsuji , Masahito Ueda
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