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Strong electron correlations drive Mott insulator transitions. Yet, there exists no framework to classify Mott insulators by their degree of correlation. Cuprate superconductors, with their tunable doping and rich phase diagrams, offer a…

We report a neutron and Raman scattering study of a single-crystal of La(2)CuO(4.05) prepared by high temperature electrochemical oxidation. Elastic neutron scattering measurements show the presence of two phases, corresponding to the two…

We report on Raman scattering measurements of single crystalline La$_{1-x}$Sr$_x$MnO$_3$ ($x$=0, 0.06, 0.09 and 0.125), focusing on the high frequency regime. We observe multi-phonon scattering processes up to fourth-order which show…

The Raman response of the metallic glass Ni$_{67}$Zr$_{33}$ is measured as a function of polarization and temperature and analyzed theoretically. Unexpectedly, the intensity in the range up to 300\wn increases upon cooling, which is…

Disordered Systems and Neural Networks · Physics 2015-05-20 B. Muschler , I. Tüttő , A. Zawadowski , J. Balogh , R. Hackl

Low energy excitations in the multiferroic material TbMnO3 have been investigated by Raman spectroscopy. Our observations reveal the existence of two peaks at 30 cm-1 and 60 cm-1. They are observed in the cycloidal phase below the Curie…

Strongly Correlated Electrons · Physics 2010-10-12 P. Rovillain , M. Cazayous , Y. Gallais , A. Sacuto , M-A. Measson , H. Sakata

Resonant behavior of the Raman process is predicted when the laser frequency is close to the orbital excitation energy of LaMnO3 at 2 eV. The incident photon creates a vibrationally excited self-trapped ``orbiton'' state from the…

Strongly Correlated Electrons · Physics 2009-10-31 Vasili Perebeinos , Philip B. Allen

We investigate the collective behavior of orbital angular momentum in the spin ferromagnetic state of a Mott insulator with $t_{2g}$ orbital degeneracy. The frustrated nature of the interactions leads to an infinite degeneracy of classical…

Strongly Correlated Electrons · Physics 2009-11-07 Giniyat Khaliullin , Satoshi Okamoto

Recent optical conductivity measurements reveal the presence of Hubbard excitons in certain Mott insulators. In light of these results, it is important to revisit the dynamics of these materials to account for excitonic correlations. We…

Strongly Correlated Electrons · Physics 2020-09-23 D. J. Lovinger , M. Brahlek , P. Kissin , D. M. Kennes , A. J. Millis , R. Engel-Herbert , R. D. Averitt

The Mott transistor is a paradigm for a new class of electronic devices---often referred to by the term Mottronics---, which are based on charge correlations between the electrons. Since correlation-induced insulating phases of most oxide…

The elementary excitations of a model Hamiltonian that captures the low energy behavior of a simple two-fold degenerate Hubbard Hamiltonian with Hund's rule coupling, is studied. The phase diagram in the mean-field limit and in a two-site…

Strongly Correlated Electrons · Physics 2007-05-23 J. van den Brink , W. Stekelenburg , D. I. Khomskii , G. A. Sawatzky , K. I. Kugel

Magnetic excitations in the optimally doped high-$T_\mathrm{c}$ superconductor Bi$_{1.5}$Pb$_{0.55}$Sr$_{1.6}$La$_{0.4}$CuO$_{6+\delta}$ (OP-Bi2201, $T_\mathrm{c}\simeq 34$ K) are investigated by Cu $L_3$ edge resonant inelastic x-ray…

The doping and temperature dependent optical conductivity spectra of the quasi-two-dimensional Ca_{2-x}Sr_xRuO_4 (0.0=<x=<2.0) system were investigated. In the Mott insulating state, two electron correlation-induced peaks were observed…

Strongly Correlated Electrons · Physics 2009-11-07 J. S. Lee , Y. S. Lee , T. W. Noh , S. -J. Oh , Jaejun Yu , S. Nakatsuji , H. Fukazawa , Y. Maeno

We study the model high-temperature superconductor HgBa2CuO4+d with electronic Raman scattering and optical ellipsometry over a wide doping range. The resonant Raman condition which enhances the scattering cross section of "two-magnon"…

Superconductivity · Physics 2015-06-16 Yuan Li , M. Le Tacon , Y. Matiks , A. V. Boris , T. Loew , C. T. Lin , Lu Chen , M. K. Chan , C. Dorow , L. Ji , N. Barisic , X. Zhao , M. Greven , B. Keimer

We use polarized magneto-Raman scattering to study purely electronic excitations and the electron-phonon coupling in bulk graphite. At a temperature of 4.2 K and in magnetic fields up to 28 T we observe $K$-point electronic excitations…

Mesoscale and Nanoscale Physics · Physics 2015-05-30 P. Kossacki , C. Faugeras , M. Kühne , M. Orlita , A. A. L. Nicolet , J. M. Schneider , D. M. Basko , Y. I. Latyshev , M. Potemski

We present a Raman scattering study of Ca$_2$RuO$_4$, in which we investigate the temperature-dependence of the lattice dynamics and the electron-phonon interaction below the metal-insulator transition temperature ({\it T}$_{\rm MI}$).…

Strongly Correlated Electrons · Physics 2009-11-11 H. Rho , S. L. Cooper , S. Nakatsuji , H. Fukazawa , Y. Maeno

We have measured the doping and temperature dependence of lattice vibrations and magnetic excitations in the prototypical doped spin-orbit Mott insulator Sr$_{2-x}$La$_x$IrO$_4$ (x=0, 0.015, and 0.10). Our findings show that the…

Strongly Correlated Electrons · Physics 2017-09-27 H. Gretarsson , J. Sauceda , N. H. Sung , M. Höppner , M. Minola , B. J. Kim , B. Keimer , M. Le Tacon

The superconducting critical temperature $T_{\mathrm{c}}$ of intercalated iron-selenide superconductor (Li,Fe)OHFeSe (FeSe11111) can be increased to 42 K from 8 K of bulk FeSe. It shows remarkably similar electronic properties as the…

Vanadium dioxide is of broad interest as a spin-1/2 electron system that realizes a metal-insulator transition near room temperature, due to a combination of strongly correlated and itinerant electron physics. Here, resonant inelastic X-ray…

A detailed inelastic neutron scattering study of the high temperature superconductor $\rm YBa_2Cu_3O_{6.85}$ provides evidence of new resonant magnetic features, in addition to the well known resonant mode at 41 meV: (i) a commensurate…

Superconductivity · Physics 2007-05-23 S. Pailhes , Y. Sidis , P. Bourges , V. Hinkov , A. Ivanov , C. Ulrich , L. P. Regnault , B. Keimer

Two magnon excitations and the nodal spin density wave (SDW) gap were observed in BaFe2As2 by Raman scattering. Below the SDW transition temperature (TSDW) nodal SDW gap opens together with new excitations in reconstructed electronic…

Superconductivity · Physics 2010-11-01 S. Sugai , Y. Mizuno , R. Watanabe , T. Kawaguchi , K. Takenaka , H. Ikuta , Y. Takayanagi , N. Hayamizu , Y. Sone