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Related papers: Non-equilibrium Magnetization Dynamics in the Fe_8…

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We describe an experiment aimed at measuring the spin dynamics of the Fe8 single-molecule magnet in the presence of pulsed microwave radiation. In earlier work, heating was observed after a 0.2-ms pulse of intense radiation, indicating that…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 M. Bal , Jonathan R. Friedman , M. T. Tuominen , E. M. Rumberger , D. N. Hendrickson

Microwave radiation applied to single-molecule magnets can induce large magnetization changes when the radiation is resonant with transitions between spin levels. These changes are interpreted as due to resonant heating of the sample by the…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 M. Bal , Jonathan R. Friedman , E. M. Rumberger , S. Shah , D. N. Hendrickson , N. Avraham , Y. Myasoedov , H. Shtrikman , E. Zeldov

We use millimeter wave radiation to manipulate the populations of the energy levels of a single crystal molecular magnet Fe8. When a continuous wave radiation is in resonance with the transitions from the ground state to the first excited…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 M. Bal , Jonathan R. Friedman , Y. Suzuki , K. Mertes , E. M. Rumberger , D. N. Hendrickson , Y. Myasoedov , H. Shtrikman , N. Avraham , E. Zeldov

Magnetization measurements made in small fields as a function of temperature reveal an unusual equilibrium below 900 mK for the molecular nano-magnet Fe_8. Measurements of the relaxation of the magnetization demonstrate that the approach to…

Other Condensed Matter · Physics 2007-05-23 V. Villar , E. Lhotel , C. Sangregorio , C. Paulsen

We measure magnetization changes in a single crystal of the single-molecule magnet Fe8 when exposed to intense, short (<20 $\mu$s) pulses of microwave radiation resonant with the m = 10 to 9 transition. We find that radiation induces a…

Mesoscale and Nanoscale Physics · Physics 2008-03-14 M. Bal , Jonathan R. Friedman , W. Chen , M. T. Tuominen , C. C. Beedle , E. M. Rumberger , D. N. Hendrickson

We present measurements on the single molecule magnet Fe8 in the presence of pulsed microwave radiation at 118 GHz. The spin dynamics is studied via time resolved magnetization experiments using a Hall probe magnetometer. We investigate the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 K. Petukhov , S. Bahr , W. Wernsdorfer , A. -L. Barra , V. Mosser

We present pump-probe measurements on the single-molecule magnet Fe_8 with microwave pulses having a length of several nanoseconds. The microwave radiation in the experiments is located in the frequency range between 104 GHz and 118 GHz.…

Mesoscale and Nanoscale Physics · Physics 2008-02-05 S. Bahr , K. Petukhov , V. Mosser , W. Wernsdorfer

The magnetocaloric effect, that consists of adiabatic temperature changes in a varying external magnetic field, appears not only when the amplitude is changed, but in cases of anisotropic magnetic materials also when the direction is…

Strongly Correlated Electrons · Physics 2019-03-25 C. Beckmann , J. Ehrens , J. Schnack

The low temperature spin dynamics of a Fe8 Single-Molecule Magnet was studied under circularly polarized electromagnetic radiation allowing us to establish clearly photon-assisted tunneling. This effect, while linear at low power, becomes…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 L. Sorace , W. Wernsdorfer , C. Thirion , A. -L. Barra , M. Pacchioni , D. Mailly , B. Barbara

We have used inelastic neutron scattering and muon-spin rotation to compare the low energy magnetic excitations in single crystals of superconducting Fe1.01Se0.50Te0.50 and non-superconducting Fe1.10Se0.25Te0.75. We confirm the existence of…

We report the observation of strong coupling of a macroscopic ensemble of ~10^{16} Fe_8 molecular nanomagnets to the resonant mode of a microwave cavity. We use millimeter-wave spectroscopy to measure the splitting of the system's resonant…

Mesoscale and Nanoscale Physics · Physics 2014-06-11 A. W. Eddins , C. C. Beedle , D. N. Hendrickson , Jonathan R. Friedman

We report measurements on magnetization reversal in the Fe$_8$ molecular magnet using fast pulsed magnetic fields of 1.5 kT/s and in the temperature range of 0.6-4.1 K. We observe and analyze the temperature dependence of the reversal…

Mesoscale and Nanoscale Physics · Physics 2014-09-11 S. N. Jammalamadaka , J. Vanacken , V. V. Moshchalkov , Saül Vélez , J. Tejada , Ferran Macià

We present magnetization measurements on the single molecule magnet Fe8 in the presence of pulsed microwave radiation. A pump-probe technique is used with two microwave pulses with frequencies of 107 GHz and 118 GHz and pulse lengths of…

Mesoscale and Nanoscale Physics · Physics 2007-10-17 S. Bahr , K. Petukhov , V. Mosser , W. Wernsdorfer

The mechanism of rapid and selective heating of magnetic metal oxides under the magnetic field of microwaves which continues beyond the Curie temperature $ T_{c} $ is identified by using the Heisenberg model. Monte Carlo calculations based…

Materials Science · Physics 2009-02-13 Motohiko Tanaka , Hirohiko Kono , Koji Maruyama

Spin relaxation between the two lowest-lying spin-states has been studied in the S=4 single molecule magnet Ni$_4$ under steady state conditions of low amplitude and continuous microwave irradiation. The relaxation rate was determined as a…

Mesoscale and Nanoscale Physics · Physics 2008-07-22 G. de Loubens , D. A. Garanin , C. C. Beedle , D. N. Hendrickson , A. D. Kent

The low temperature relaxation of the magnetization in magnetic molecular solids such as Fe$_8$ is studied using Monte Carlo simulations. A set of rate equations is developed to understand the simulations, and the results are compared. The…

Statistical Mechanics · Physics 2015-10-14 Avinash Vijayaraghavan , Anupam Garg

The nonequilibrium responses of Ising metamagnet (layered antiferromagnet) to the propagating magnetic wave are studied by Monte Carlo simulation. Here, the spatio-temporal variations of magnetic field keeps the system away from…

Statistical Mechanics · Physics 2015-03-11 Muktish Acharyya

Presented are magnetization measurements on a crystal of Fe8 single-molecule magnets using a Hall probe magnetometer. Irradiation with microwaves at frequencies of 92 and 110-120 GHz leads to the observation of electron paramagnetic…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 K. Petukhov , W. Wernsdorfer , A. -L. Barra

Photons emitted by transition between the discrete levels of single molecular magnets might obay the elementary condition for Dicke's super-radiance. We investigate this possibility in the Fe8 molecule where magnetization jumps are known to…

Strongly Correlated Electrons · Physics 2009-05-13 Oren Shafir , Amit Keren

Tunneling of the spins in the Fe$_8$ molecular magnet from a metastable ground state to an excited state is accompanied by a decay of these spins to the global ground state, and an increase of the crystal temperature. We measured this…

Mesoscale and Nanoscale Physics · Physics 2019-10-29 Maayan Yaari , Amit Keren
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