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We theoretically investigate the ground state spin of a polynuclear transition-metal complex as a function of the number of added electrons taking into account strong electron correlations. Our phenomenological model of the so-called…

Strongly Correlated Electrons · Physics 2007-05-23 C. Romeike , M. R. Wegewijs , M. Ruben , W. Wenzel , H. Schoeller

We present a new mechanism for a spin blockade effect associated with a change in the type of magnetic anisotropy over oxidation state in a single molecule transistor, by taking an example of an individual Eu$_{2}$(C$_{8}$H$_{8}$)$_{3}$…

Mesoscale and Nanoscale Physics · Physics 2016-11-23 Guangpu Luo , Kyungwha Park

The total spin of correlated electrons in a quantum dot changes with magnetic field and this effect is generally linked to the change in the total angular momentum from one magic number to another, which can be understood in terms of an…

Mesoscale and Nanoscale Physics · Physics 2009-10-30 Hiroshi Imamura , Hideo Aoki , Peter A. Maksym

Molecular nanomagnets show clear signatures of coherent behavior and have a wide variety of effective low-energy spin Hamiltonians suitable for encoding qubits and implementing spin-based quantum information processing. At the nanoscale,…

Mesoscale and Nanoscale Physics · Physics 2013-05-29 Mircea Trif , Filippo Troiani , Dimitrije Stepanenko , Daniel Loss

We present measurements on spin blockade in a laterally integrated quantum dot. The dot is tuned into the regime of strong Coulomb blockade, confining ~ 50 electrons. At certain electronic states we find an additional mechanism suppressing…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 A. K. Huettel , H. Qin , A. W. Holleitner , R. H. Blick , K. Neumaier , D. Weinmann , K. Eberl , J. P. Kotthaus

We theoretically investigate inelastic transport through anisotropic magnetic molecules weakly coupled to one ferromagnetic and one nonmagnetic lead. We find that the current is suppressed over wide voltage ranges due to spin blockade. In…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Florian Elste , Carsten Timm

Motivated by the experimental evidence of the Nagaoka ferromagnetism in quantum dot systems by Dehollain et al [1], we search for possible confirmation of such kind of ferromagnetism by analyzing the spin-resolved transport properties of a…

Mesoscale and Nanoscale Physics · Physics 2024-10-04 Piotr Trocha , Emil Siuda , Ireneusz Weymann

Inspired by the Nagaoka ferromagnetism, we propose an itinerant model to study the transition between the Mott singlet state and a ferromagnetic state by emulating a doping process in finite lattices. In the Nagaoka ferromagnetism, the…

Strongly Correlated Electrons · Physics 2015-01-14 Hiroaki Onishi , Seiji Miyashita

The ability to make electrical contact to single molecules creates opportunities to examine fundamental processes governing electron flow on the smallest possible length scales. We report experiments in which we controllably stretch…

It is known that the quantum-mechanical ground state of a nano-scale junction has a significant impact on its electrical transport properties. This becomes particularly important in transistors consisting of a single molecule. Due to strong…

Single-electronics and spintronics are among the most intensively investigated potential complements or alternatives to CMOS electronics. Single-electronics, which is based on the discrete charge of the electron, is the ultimate in…

We present an analysis of electron transport through two weakly coupled precision placed phosphorus donors in silicon. In particular, we examine the (1,1) to (0,2) charge transition where we predict a new type of current blockade driven…

Quantum Physics · Physics 2015-09-21 Samuel K. Gorman , Matthew A. Broome , William J. Baker , Michelle Y. Simmons

We study electronic transport through a magnetic molecule with an intrinsic spin $S$ coupled to two magnetic electrodes, in the incoherent regime. The molecule is modeled as a single resonant level with large Coulomb repulsion (no double…

Mesoscale and Nanoscale Physics · Physics 2010-11-19 Thibaut Jonckheere , Ken-Ichiro Imura , Thierry Martin

Controlling electronic transport through a single-molecule junction is crucial for molecular electronics or spintronics. In magnetic molecular devices, the spin degree-of-freedom can be used to this end since the magnetic properties of the…

We report on the observation of Kondo and split Kondo peaks in single-molecule transistors containing a single spin transition molecule with a Fe2+ ion. Coulomb blockade characteristics reveal a double quantum dot behavior in a parallel…

Mesoscale and Nanoscale Physics · Physics 2010-04-27 A. Bernand-Mantel , J. S. Seldenthuis , A. Beukman , H. S. J. van der Zant , V. Meded , R. Chandrasekhar , K. Fink , M. Ruben , F. Evers

Embedding a magnetic electroactive molecule in a three-terminal junction allows for the fast and local electric field control of magnetic properties desirable in spintronic devices and quantum gates. Here, we provide an example of this…

Magnetic switching of a single-molecule magnet (SMM) due to spin-polarized current is investigated theoretically. The charge transfer between the electrodes takes place via the lowest unoccupied molecular orbital (LUMO) of the SMM.…

Mesoscale and Nanoscale Physics · Physics 2007-08-29 Maciej Misiorny , Józef Barnas

The quantum mechanical screening of a spin via conduction electrons depends sensitively on the environment seen by the magnetic impurity. A high degree of responsiveness can be obtained with metal complexes, as the embedding of a metal ion…

Strongly Correlated Electrons · Physics 2018-11-29 Jens Kügel , Michael Karolak , Andreas Krönlein , David Serrate , Matthias Bode , Giorgio Sangiovanni

We investigate a silicon single-electron transistor (SET) in a metal-oxide-semiconductor (MOS) structure by applying a magnetic field perpendicular to the sample surface. The quantum dot is defined electrostatically in a point contact…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 Binhui Hu , C. H. Yang

We present a complete theory of the spin torque phenomena in a ultrasmall nanomagnet coupled to non-collinear ferromagnetic electrodes through tunnelling junctions. This model system can be described by a simple microscopic model which…

Mesoscale and Nanoscale Physics · Physics 2008-02-22 O. Parcollet , X. Waintal
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