English
Related papers

Related papers: Magnetism in Exact Exchange Density Functional The…

200 papers

Among the quasi-2D van der Waals magnetic systems, Fe4GeTe2 imprints a profound impact due to its near-room temperature ferromagnetic behaviour and the complex magnetothermal phase diagram exhibiting multiple phase transformations, as…

The dimeric form of the single-molecule magnet [Mn$_4$O$_3$Cl$_4$(O$_2$CEt)$_3$(py)$_3$]$_2$ recently revealed interesting phenomena: no quantum tunneling at zero field and tunneling before magnetic field reversal. This is attributed to…

In this paper we present an accurate numerical scheme for extracting inter-atomic exchange parameters ($J_{ij}$) of strongly correlated systems, based on first-principles full-potential electronic structure theory. The electronic structure…

Strongly Correlated Electrons · Physics 2015-03-11 Y. O. Kvashnin , O. Grånäs , I. Di Marco , M. I. Katsnelson , A. I. Lichtenstein , O. Eriksson

We have explored, computationally and experimentally, the magnetic properties of \fecob{} alloys. Calculations provide a good agreement with experiment in terms of the saturation magnetization and the magnetocrystalline anisotropy energy…

Within the same failure mode, iron has the lowest ideal tensile strength among the transition metals crystallizing in the body-centered cubic structure. Here, we demonstrate that this anomalously low strength of Fe originates partly from…

Materials Science · Physics 2014-07-02 Xiaoqing Li , Stephan Schönecker , Jijun Zhao , Börje Johansson , Levente Vitos

In spin-density-functional theory (SDFT) for noncollinear magnetic materials, the Kohn-Sham system features exchange-correlation (xc) scalar potentials and magnetic fields. The significance of the xc magnetic fields is not very well…

Strongly Correlated Electrons · Physics 2023-03-29 Daniel Hill , Justin Shotton , Carsten A. Ullrich

Me$_{3+\delta}$Ge, being a Weyl semimetal, shows a large anomalous Hall effect (AHE), which decreases slowly with an increase in $\delta$ from 0.1 to 0.4. However, AHE in this compound remains significantly large in the whole range of…

Strongly Correlated Electrons · Physics 2023-05-17 Venus Rai , Anne Stunault , Wolfgang Schmidt , Subhadip Jana , Jörg Perßon , Thomas Brückel , Shibabrata Nandi

Magnetism in transition metal compounds is usually considered starting from a description of isolated ions, as exact as possible, and treating their (exchange) interaction at a later stage. We show that this standard approach may break down…

Strongly Correlated Electrons · Physics 2016-10-24 S. V. Streltsov , D. I. Khomskii

By expanding the wave function in plane waves, we use the pseudopotential method of density functional theory within the generalized gradient approximation to calculate the effective magnetic coupling energies of the S=5/2 spins in the Fe2…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Sergey Stolbov , Richard A. Klemm , Talat S. Rahman

Fast spin manipulation in magnetic heterostructures, where magnetic interactions between different materials often define the functionality of devices, is a key issue in the development of ultrafast spintronics. Although recently developed…

Materials Science · Physics 2022-03-04 X. Liu , H. C. Yuan , P. Liu , J. Y. Shi , H. L. Wang , S. H. Nie , F. Jin , Z. Zheng , X. Z. Yu , J. H. Zhao , H. B. Zhao , G. Lüpke

We calculate magnetic anisotropy energy of Fe and Ni by taking into account the effects of strong electronic correlations, spin-orbit coupling, and non-collinearity of intra-atomic magnetization. The LDA+U method is used and its equivalence…

Strongly Correlated Electrons · Physics 2009-10-31 Imseok Yang , Sergej Y. Savrasov , Gabriel Kotliar

In this report we review the method of explicit calculations of interatomic exchange interactions of magnetic materials. This involves exchange mechanisms normally referred to as Heisenberg exchange, Dzyaloshinskii-Moriya interaction and…

Starting from exact expression for the dynamical spin susceptibility in the time-dependent density functional theory a controversial issue about exchange interaction parameters and spin-wave excitation spectra of itinerant electron…

Materials Science · Physics 2009-11-10 M. I. Katsnelson , A. I. Lichtenstein

Exchange interactions are a manifestation of the quantum mechanical nature of the electrons and play a key role in predicting the properties of materials from first principles. In density functional theory (DFT), a widely used approximation…

Materials Science · Physics 2020-03-27 Marco Bernardi

The Fe$_{n}$GeTe$_{2}$ systems are newly discovered two-dimensional van-der-Waals materials, exhibiting magnetism at room temperature. The sub-systems belonging to Fe$_{n}$GeTe$_{2}$ class are special because they show site-dependent…

Materials Science · Physics 2022-12-19 Sukanya Ghosh , Soheil Ershadrad , Vladislav Borisov , Biplab Sanyal

Using an accurate semi-analytic wavefunction for two electron atoms, we construct the external potential for varying strength of electron-electron (e-e) interaction. Using this potential we explicitly calculate the energy of their positive…

Atomic and Molecular Clusters · Physics 2016-02-18 Rabeet Singh Chauhan , Manoj K. Harbola

The magnetic ground state of FeRh is highly sensitive towards the lattice constant. This, in addition to partially filled d-shells of Fe and Rh, posed a significant challenge for Density Functional Theory (DFT) calculations in the past.…

Materials Science · Physics 2024-01-24 Shishir Kumar Pandey , Saikat Debnath , Zhanghao Zhouyina , Qiangqiang Gu

Half-metallicity, low magnetic damping and high curie temperature (TC) are crucial for application in spintronics and full Heusler alloys in this regard exhibit remarkable properties. Herein, we have considered Co2FeAl (CFA) and Fe2CoAl…

Computational Physics · Physics 2018-06-08 Lalrinkima , Gennady M. Mikhailov , D. P. Rai

The compound FeMnP$_{0.50}$Si$_{0.50}$ has been studied by magnetic measurements, M\"ossbauer spectroscopy and electronic structure and total energy calculations. An unexpected high magnetic hyperfine field for Fe atoms located at the…

Magnetisation dynamics in exchange spring magnets have been studied using simulations of the FePt/Fe bilayer system. The FePt hard layer exhibits strong perpendicular magnetocrystalline anisotropy, while the soft (Fe) layer has negligible…

Mesoscale and Nanoscale Physics · Physics 2010-06-29 Pedro M. S. Monteiro , D. S. Schmool