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Starting from the quantum Liouville equation for the density operator and applying the Weyl quantization, Wigner equations for the longitudinal and transversal optical and acoustic phonons are deduced. The equations are valid for any solid,…

Mathematical Physics · Physics 2023-01-03 Vito Dario Camiola , Giorgia Vitanza , Vittorio Romano

We present a fast and stable numerical technique to obtain the self-energy terms of electrodes for first-principles electron-transport calculations. Although first-principles calculations based on the real-space finite-difference method are…

Mesoscale and Nanoscale Physics · Physics 2016-01-27 Tomoya Ono , Shigeru Tsukamoto

Nanoscale electronic transport is of intense technological interest, with applications ranging from semiconducting devices and molecular junctions to charge migration in biological systems. Most explicit theoretical approaches treat…

Mesoscale and Nanoscale Physics · Physics 2014-08-08 Justin E. Elenewski , Hanning Chen

Density functional theory calculations of electronic transport based on local exchange and correlation functionals contain self-interaction errors. These originate from the interaction of an electron with the potential generated by itself…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 C. Toher , S. Sanvito

We have presented a consistent electronic transport framework for the two-dimensional extended Holstein's organic molecular-crystal based upon complete quantum-mechanical treatment through the non-equilibrium Green's function (NEGF)…

Mesoscale and Nanoscale Physics · Physics 2022-08-04 Bhupesh Bishnoi

Inelastic effects in electron transport through nano-sized devices are addressed with a method based on nonequilibrium Green's functions (NEGF) and perturbation theory to infinite order in the electron-vibration coupling. We discuss the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Thomas Frederiksen , Mads Brandbyge , Nicolas Lorente , Antti-Pekka Jauho

When a molecule dissociates, the exact Kohn-Sham (KS) and Pauli potentials may form step structures. Reproducing these steps correctly is central for the description of dissociation and charge-transfer processes in density functional theory…

Chemical Physics · Physics 2021-03-23 Jakub Kocák , Eli Kraisler , Axel Schild

We present a cluster-based density-functional approach to model charge transport through molecular and atomic contacts. The electronic structure of the contacts is determined in the framework of density functional theory, and the parameters…

Mesoscale and Nanoscale Physics · Physics 2008-12-04 F. Pauly , J. K. Viljas , U. Huniar , M. Hafner , S. Wohlthat , M. Burkle , J. C. Cuevas , G. Schon

We propose to correlate transmittance maps and spectral-density maps of planar junctions, in order to analyze quantitatively and in detail spin-dependent transport calculations. Since spectral-density maps can be resolved with respect to…

Mesoscale and Nanoscale Physics · Physics 2013-05-29 P. Bose , P. Zahn , I. Mertig , J. Henk

In this contribution we demonstrate structural control over a transport resonance in HS(CH$_{2}$)$_{n}$[1,4 - C$_{6}$H$_{4}$](CH$_{2}$)$_{n}$SH (n = 1, 3, 4, 6) metal - molecule - metal junctions, fabricated and tested using the scanning…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Carly Brooke , Andrea Vezzoli , Simon J. Higgins , Linda A. Zotti , J. J. Palacios , Richard J. Nichols

We use the effective-mass approximation and the density-functional theory with the local-density approximation for modeling two-dimensional nano-structures connected phase-coherently to two infinite leads. Using the non-equilibrium Green's…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Paula Havu , Ville Havu , Martti Puska , Risto Nieminen

Using self-energy-corrected density functional theory (DFT) and a coherent scattering-state approach, we explain current-voltage (IV) measurements of four pyridine-Au and amine-Au linked molecular junctions with quantitative accuracy.…

Mesoscale and Nanoscale Physics · Physics 2012-12-04 Pierre Darancet , Jonathan R. Widawsky , Hyoung Joon Choi , Latha Venkataraman , Jeffrey B. Neaton

Electron transport characteristics through molecular wires are studied by using the Green's function formalism. Parametric calculations are performed based on the tight-binding model to investigate the transport properties through the…

Mesoscale and Nanoscale Physics · Physics 2009-11-06 Santanu K. Maiti

Building on the many existing algorithms for calculating the DC transport properties of quantum tight-binding models, we develop a systematic approach that expresses finite frequency observables in terms of the stationary Green's function…

Mesoscale and Nanoscale Physics · Physics 2013-02-15 Oleksii Shevtsov , Xavier Waintal

We introduce a scheme for constructing partly occupied, maximally localized Wannier functions (WFs) for both molecular and periodic systems. Compared to the traditional occupied WFs the partly occupied WFs posses improved symmetry and…

Materials Science · Physics 2009-11-10 K. S. Thygesen , L. B. Hansen , K. W. Jacobsen

We combine the linearized Boltzmann Transport Equation (LBTE) and quantum transport by means of the Non-equilibrium Green's Functions (NEGF) to simulate single-layer MoS2 and WS2 ultra-scaled transistors with carrier mobilities extracted…

Mesoscale and Nanoscale Physics · Physics 2020-10-13 Youseung Lee , Sara Fiore , Mathieu Luisier

Electron transport through a diatomic molecular tunnel junction shows wave like interference phenomenon. By using Keldysh non-equilibrium Green's function (NEGF) theory, we have explicitly presented current and differential conductance…

Mesoscale and Nanoscale Physics · Physics 2012-12-18 Muhammad Imran

This paper presents an ab initio methodology to account for electron-phonon interactions in 2D materials, focusing on transition metal dichalcogenides (TMDCs). It combines density functional theory and maximally localized Wannier functions…

Mesoscale and Nanoscale Physics · Physics 2023-12-04 Jonathan Backman , Youseung Lee , Mathieu Luisier

We report findings from several ab-initio, self-consistent calculations of electronic and transport properties of wurtzite aluminum nitride. Our calculations utilized a local density approximation (LDA) potential and the linear combination…

We theoretically study the electronic transport in the monolayer of dithiolated phenylene vinylene oligomeres coupled to the (111) surfaces of gold electrodes. We use non-equilibrium Green functions (NEGF) and density functional theory(DFT)…

Materials Science · Physics 2009-11-10 Z. Crljen , A. Grigoriev , G. Wendin , K. Stokbro
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