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The results of ac and dc magnetization and heat capacity measurements on the oxides, Ca$_3$Co$_{1+x}$Mn$_{1-x}$O$_6$, forming in a K$_4$CdCl$_6$-derived rhombohedral quasi-one-dimensional crystal structure, are reported. As far as…

Strongly Correlated Electrons · Physics 2009-11-10 S. Rayaprol , Kausik Sengupta , E. V. Sampathkumaran

A positive muon spin rotation and relaxation ($\mu^+$SR) experiment on [Ca$_2$CoO$_3$]$_{0.62}$[CoO$_2$], ({\sl i.e.}, Ca$_3$Co$_4$O$_9$, a layered thermoelectric cobaltite) indicates the existence of two magnetic transitions at $\sim$ 100…

Strongly Correlated Electrons · Physics 2009-11-10 J. Sugiyama , J. H. Brewer , E. J. Ansaldo , H. Itahara , K. Dohmae , Y. Seno , C. Xia , T. Tani

The results of ac and dc magnetization and heat capacity measurements as a function of temperature (T = 1.8 to 300 K) are reported for a quasi-one-dimensional compound, Ca$_3$CuMnO$_6$, crystallizing in a triclinically distorted…

Strongly Correlated Electrons · Physics 2009-11-10 Kausik Sengupta , S. Rayaprol , K. K. Iyer , E. V. Sampathkumaran

We report a comprehensive experimental and theoretical study of the quasi-one-dimensional quantum magnet CuNCN. Based on magnetization measurements above room temperature as well as muon spin rotation and electron spin resonance…

We report a neutron diffraction and muon spin relaxation muSR study of static and dynamical magnetic properties of BaCo2V2O8, a quasi-one-dimensional spin-chain system. A proposed model for the antiferromagnetic structure includes: a…

The title compound belongs to a wide group of quasi-one-dimensional (Q1D) antiferromagnets (AF) and its Co2+ ions form Q1D screw-chains along the c-axis. We here present the first investigation of the microscopic magnetic nature of a single…

Strongly Correlated Electrons · Physics 2013-07-30 M. Mansson , K. Prsa , J. Sugiyama , H. Nozaki , A. Amato , K. Omura , S. Kimura , M. Hagiwara

A detailed zero and transverse field (ZF&TF) muon spin rotation (muSR) investigation of magnetism and the magneto-electric coupling in Cu2OSeO3 is reported. An internal magnetic field B_int(T=0) = 85.37(25) mT was found, in agreement with a…

Strongly Correlated Electrons · Physics 2015-05-28 A. Maisuradze , Z. Guguchia , B. Graneli , H. M. Ronnow , H. Berger , H. Keller

Magnetism of layered cobaltites Na$_x$CoO$_2$ with $x$ = 0.6 and 0.9 has been investigated by a positive muon spin rotation and relaxation ($\mu^+$SR) spectroscopy together with magnetic susceptibility and specific heat measurements, using…

Strongly Correlated Electrons · Physics 2009-11-10 J. Sugiyama , J. H. Brewer , E. J. Ansaldo , B. Hitti , M. Mikami , Y. Mori , T. Sasaki

Heat-capacity behavior in the presence of externally applied magnetic field (H) up to 140 kOe is investigated (2-35 K) for the quasi-1-dimensional compound, Ca3Co2O6, believed to order magnetically with the so-called partially disordered…

Strongly Correlated Electrons · Physics 2009-11-10 E. V. Sampathkumaran , Z. Hiroi , S. Rayaprol , Y. Uwatoko

We present the results of a muon-spin relaxation (muSR) investigation into magnetic ordering in several families of layered quasi-two-dimensional molecular antiferromagnets based on transition metal ions such as S=1/2 Cu2+ bridged with…

The magnetic response of CaK(Fe$_{0.949}$Ni$_{0.051}$)$_4$As$_4$ was investigated by means of the muon-spin rotation/relaxation. The long-range commensurate magnetic order sets in below the N\'{e}el temperature $T_{\rm N}= 50.0(5)$~K. The…

The interplay of crystal electric field, temperature, and spin-orbit coupling can yield a Kramers ion and thus an effective S = 1/2 ground state for Co2+ ions (3d7), which is often the case for low dimensional materials. This is because a…

Materials Science · Physics 2025-04-01 Lun Jin , Robert J. Cava

A combination of variable-temperature neutron scattering, reverse Monte Carlo analysis and direct Monte Carlo simulation is used to characterise the emergence of magnetic order in the metal--organic framework (MOF) Tb(HCOO)$_3$ over the…

Disordered Systems and Neural Networks · Physics 2016-12-21 Daniel R. Harcombe , Philip G. Welch , Pascal Manuel , Paul J. Saines , Andrew L. Goodwin

Sr_4Cr_3O_9 is the n = 2 member of a family of quasi-one-dimensional compounds A_{n+2}T_{n+1}O_{3n+3} (A = Ca, Sr, or Ba, T = transition metal, and n = 1 to \infty) having a crystal structure which consists of chains of n TO_6 octahedra…

Strongly Correlated Electrons · Physics 2008-08-26 Yogesh Singh , D. C. johnston

Dielectric and magnetic properties have been studied for poly-crystalline samples of quasi-one-dimensional frustrated spin-1/2 system Rb$_{2}$(Cu$_{1-x}$M$_{x}$)$_{2}$Mo$_{3}$O$_{12}$(M=Ni and Zn) which does not exhibit a three-dimensional…

Strongly Correlated Electrons · Physics 2015-06-12 Yukio Yasui , Yudai Yanagisawa , Ryuji Okazaki , Ichiro Terasaki

We have performed field-swept 59Co NMR measurements on the 'exotic' spin-chain material, Ca3Co2O6, crystallizing in K4CdCl6-type rhombohedral structure, believed to exhibit two magnetic transition temperatures (around 24 and 12 K). This is…

Strongly Correlated Electrons · Physics 2009-11-10 E. V. Sampathkumaran , N. Fujiwara , S. Rayaprol , P. K. Madhu , Y. Uwatoko

Using muon spin rotation (muSR) we investigated the magnetic and superconducting properties of a series of Ba(Fe1-xCox)2As2 single crystals with 0 =< x =< 0.15. Our study details how the antiferromagnetic order is suppressed upon Co…

We report on a 59Co NMR investigation of the trigonal cobaltate Ca3Co2O6 carried out on a single crystal, providing precise determinations of the electric field gradient and chemical shift tensors, and of the internal magnetic fields at the…

Strongly Correlated Electrons · Physics 2015-05-20 G. Allodi , R. De Renzi , S. Agrestini , C. Mazzoli , M. R. Lees

We present the first evidence of magnetic order in the quasi-one-dimensional spin 1/2 molecular chain compound, copper pyrazine dinitrate Cu(C4H4N2)(NO3)2}. Zero field muon-spin relaxation measurements made at dilution refrigerator…

Strongly Correlated Electrons · Physics 2007-11-14 T. Lancaster , S. J. Blundell , M. L. Brooks , P. J. Baker , F. L. Pratt , J. L. Manson , C. P. Landee , C. Baines

Magnetic properties of a one-dimensional frustrated quantum spin system Rb2Cu2Mo3O12 is investigated by the muon spin relaxation (muSR) technique. Although this system shows an incommensurate spin correlation in neutron scattering, it has…

Strongly Correlated Electrons · Physics 2018-04-04 Seiko Ohira-Kawamura , Keisuke Tomiyasu , Akihiro Koda , Dita P. Sari , Retno Asih , Sungwon Yoon , Isao Watanabe , Kenji Nakajima
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