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A progress report on two recent theoretical approaches proposed to understand the physics of irreversible fractal aggregates showing up a structural transition from a rather dense to a more multibranched growth is presented. In the first…

Condensed Matter · Physics 2008-08-31 E. Canessa

We develop an algorithm for bosonic path integral molecular dynamics (PIMD) simulations with periodic boundary conditions (PBC) that scales quadratically with the number of particles. Path integral methods are a powerful tool to simulate…

Chemical Physics · Physics 2025-09-16 Jacob Higer , Yotam M. Y. Feldman , Barak Hirshberg

Ebert et al. [Phys. Rev. Lett. 77, 3827 (1996)] have fractured icosahedral Al-Mn-Pd single crystals in ultrahigh vacuum and have investigated the cleavage planes in-situ by scanning tunneling microscopy (STM). Globular patterns in the…

Materials Science · Physics 2007-10-10 F. Rösch , Ch. Rudhart , J. Roth , H. -R. Trebin , P. Gumbsch

We present a force-biased Monte Carlo (FMC) method for structural modeling of transition metal clusters of Fe, Ni, and Cu with 5 to 60 atoms. By employing the Finnis-Sinclair potential for Fe and the Sutton-Chen potential for Ni and Cu, the…

Materials Science · Physics 2017-12-06 Dil K. Limbu , Parthapratim Biswas

Packing transitions in the lowest energy structures of Li clusters as a function of size have been identified via simulated annealing. For N>21, the large $p$ character of Li leads to unexpected ionic structures. At N~25, a packing pattern…

chem-ph · Physics 2009-10-22 Ming Wen Sung , Ryoichi Kawai , John H. Weare

The diffusionless Burgers-Bain phase transition from a hcp arrangement to a cuboidal lattice (fcc and bcc) is analysed in great detail for Lennard-Jones solids. From the lattice vectors of an underlying bi-lattice smoothly connecting these…

The low-energy level structure and electromagnetic transitions of $^{48,50}$Cr nuclei have been studied by using interacting boson model with isospin (IBM-3). A sequence of isospin excitation bands with isospin $(T= T_{z}$, $T_{z}+1$ and $…

Nuclear Theory · Physics 2007-05-23 F. H. Al-Khudair , G. L. Long

In recent years, methods have been developed that allow first-principles electronic-structure calculations to be carried out under conditions of fixed electric field. For some purposes, however, it is more convenient to work at fixed…

Materials Science · Physics 2011-09-19 Jiawang Hong , David Vanderbilt

In this work we undertake a comprehensive numerical study of the ground state structures and optical absorption spectra of isomers of B$_{12}$ cluster. Geometry optimization was performed at the coupled-cluster-singles-doubles (CCSD) level…

Atomic and Molecular Clusters · Physics 2019-05-22 Pritam Bhattacharyya , Ihsan Boustani , Alok Shukla

Molecular dynamics simulation is employed to understand the thermodynamic behavior of cuboctahedron (cub) and icosahedron (ico) nanoparticles with 2-20 number of shells (55-28741 atoms). The embedded atom method was used to describe the…

Materials Science · Physics 2019-08-13 Maryam Azadeh , Movaffaq Kateb , Pirooz Marashi

Using molecular dynamics simulation technique, we have studied the melting behaviours of free, icosahedral PtN clusters in the size range of N=12-14. Voter and Chen version of an embedded-atom model, derived by fitting to experimental data…

Atomic and Molecular Clusters · Physics 2009-11-10 Ali Sebetci , Ziya B. Guvenc

We study a large number of physically-plausible arrangements of chromophores, generated via a computational method involving stochastic real-space transformations of a naturally occurring `reference' structure, illustrating our methodology…

Chemical Physics · Physics 2017-05-23 George C. Knee , Patrick Rowe , Luke D. Smith , Alessandro Troisi , Animesh Datta

Shapes and energies of icosahedral fullerenes are studied on an atomically detailed level. The numerical results based on the effective binary carbon-carbon potential are related to the theory of elasticity of crystalline membranes with…

Other Condensed Matter · Physics 2007-05-23 A. Siber

Isoscalar (IS) monopole and dipole excitations in $^{16}$O were investigated by the method of shifted basis antisymmetrized molecular dynamics combined with the generator coordinate method. Significant strengths of the IS monopole and…

Nuclear Theory · Physics 2019-07-10 Yoshiko Kanada-En'yo , Yuki Shikata

We systematically study the design of simple patchy sphere models that reversibly self-assemble into monodisperse icosahedral clusters. We find that the optimal patch width is a compromise between structural specificity (the patches must be…

Soft Condensed Matter · Physics 2007-09-03 Alex W. Wilber , Jonathan P. K. Doye , Ard A. Louis , Eva G. Noya , Mark A. Miller , Pauline Wong

The free energy of a 600-atom Lennard-Jones cluster is calculated as a function of surface and bulk crystallinity in order to study the structural transformations that occur in the core of medium sized clusters. Within the order parameter…

Statistical Mechanics · Physics 2010-05-27 Ivan Saika-Voivod , Louis Poon , Richard K. Bowles

In this work, phase diagrams of a modified two-mode phase-field crystal (PFC) that show two-dimensional (2D) and three-dimensional (3D) crystallographic structures were determined by utilizing a free energy minimization method. In this…

Materials Science · Physics 2017-06-06 Arezoo Emdadi , Mohsen Asle Zaeem , Ebrahim Asadi

We use ab initio pseudopotential total energy calculations with a plane wave basis set to investigate the structural energetics of various phases of polymorphic NbN. Particular attention is given to its recently discovered superconducting…

mtrl-th · Physics 2015-06-26 S. Ogut , K. M. Rabe

A global search for possible LiF cluster structures is performed, up to (LiF)8. The method is based on simulated annealing, where all the energies are evaluated on the ab initio level. In addition, the threshold algorithm is employed to…

Materials Science · Physics 2010-07-21 K. Doll , J. C. Schoen , M. Jansen

Using pair potentials fitted to an ab--initio database, combined with replica--exchange simulated annealing, we show the complex, quasicrystal-related Al$_{11}$Ir$_4$ compound contains a new version of the "pseudo-Mackay" icosahedral…

Materials Science · Physics 2012-06-26 Marek Mihalkovič , C. L. Henley