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Magnetic hyperfine field at Cu isotopes as impurities in Fe were recently measured at low temperature. A model to explain these experimental results is proposed. The diluted Cu impurities in the ferromagnetic Fe host are described by an…

Nuclear Experiment · Physics 2012-07-19 A. L. de Oliveira , C. M. Chaves , N. A. de Oliveira , A. Troper

The full potential all electron linearized augmented plane wave plus local orbitals (FP-LAPW + lo) method, as implemented in the suite of software WIEN2K, has been used to systematically investigate the structural, electronic, and magnetic…

Strongly Correlated Electrons · Physics 2015-05-14 Raymond Atta-Fynn , Asok K. Ray

The local magnetic moments and hyperfine magnetic fields (HFF) in the ordered alloys Fe_{15}Sn and Fe_{15}Si are calculated with the first-principles full-potential linear augmented plane wave (FP LAPW) method. The results are compared with…

Materials Science · Physics 2009-10-31 A. K. Arzhnikov , L. V. Dobysheva

The Fe-Cu intersite charge transfer and Fe charge disproportionation are interesting phenomena observed in some LnCu3Fe4O12 (Ln: Lanthanides) compounds containing light and heavy Ln atoms, respectively. We show that a change in the spin…

Strongly Correlated Electrons · Physics 2014-04-07 N. Rezaei , P. Hansmann , M. S. Bahramy , R. Arita

The magnetic and electronic structures of $3d$ impurity atoms from Sc to Zn in ferromagnetic body-centered cubic iron are investigated using the all-electron full-potential linearized augmented plane-wave method based on the generalized…

Materials Science · Physics 2010-05-25 Gul Rahman , In Gee Kim , H. K. D. H. Bhadeshia , Arthur J. Freeman

Carbon atom vacancies in graphene give rise to a local magnetic moment of $\sigma+\pi$ origin, whose magnitude is yet uncertain and debated. Partial quenching of $\pi$ magnetism has been ubiquitously reported in periodic $first-principles$…

Materials Science · Physics 2023-02-27 Mirko Leccese , Rocco Martinazzo

Rare-earth (RE) atoms on top of 2D materials represent an interesting platform with the prospect of tailoring the magnetic anisotropy for practical applications. Here, we investigate the ground state and magnetic properties of selected…

Mesoscale and Nanoscale Physics · Physics 2024-07-25 Johanna P. Carbone , Juba Bouaziz , Gustav Bihlmayer , Stefan Blügel

The simultaneous influence of electronic correlations and magnetic ordering on the theoretical estimation of phonons and related properties of Ni is investigated. The work includes a comparative DFT and DFT+U study, where on-site Coulomb…

Strongly Correlated Electrons · Physics 2023-07-13 Shivani Bhardwaj , Sudhir K. Pandey

We consider the effects of local impurities in highly frustrated diamond lattice antiferromagnets, which exhibit large but non-extensive ground state degeneracies. Such models are appropriate to many A-site magnetic spinels. We argue very…

Strongly Correlated Electrons · Physics 2011-08-30 Lucile Savary , Emanuel Gull , Simon Trebst , Jason Alicea , Doron Bergman , Leon Balents

The archetypal $3d$ Mott insulator hematite, Fe$_2$O$_3$, is one of the basic oxide components playing an important role in mineralogy of Earth's lower mantle. Its high pressure-temperature behavior, such as the electronic properties,…

Strongly Correlated Electrons · Physics 2019-10-07 I. Leonov , G. Kh. Rozenberg , I. A. Abrikosov

The electronic structures of the actinide elements U, Np, Pu, Am, Cm and Bk are investigated within the self-interaction corrected local spin density approximation. This method allows to describe a dual character of the 5f electrons, some…

Strongly Correlated Electrons · Physics 2009-11-11 A. Svane , L. Petit , Z. Szotek , W. M. Temmerman

Lanthanides in the trivalent oxidation state are typically described using an ionic picture that leads to localized magnetic moments. The hierarchical energy scales associated with trivalent lanthanides produce desirable properties for…

Many-body perturbation theory in the GW approach is applied to lanthanide oxides, using the local-density approximation plus a Hubbard U correction (LDA+U) as the starting point. Good agreement between the G0W0 density of states and…

Materials Science · Physics 2009-11-13 Hong Jiang , Ricardo I. Gomez-Abal , Patrick Rinke , Matthias Scheffler

High-resolution photoemission spectroscopy and realistic ab-initio calculations have been employed to analyze the onset and progression of d-sp hybridization in Fe impurities deposited on alkali metal films. The interplay between…

We perform systematic density functional theory (DFT) calculations to assess the performance of various exchange-correlation potentials $V_{xc}$ in describing the chalcogenide GaM$_4$Q$_8$ lacunar spinels (M=Mo, V, Nb, Ta; Q=S, Se). We…

Materials Science · Physics 2019-09-25 Yiqun Wang , Danilo Puggioni , James M. Rondinelli

Anderson models, based on quantum chemical studies of the molecule of U(C_8H_8)_2, are applied to investigate the problem of an U impurity in a metal. The special point here is that the U 5f-orbitals are divided into two subsets: an almost…

Strongly Correlated Electrons · Physics 2009-10-30 Mikito Koga , Wenjian Liu , Michael Dolg , Peter Fulde

We study the property of a magnetic impurity on a single-layer graphene within an Anderson impurity model. Due to the vanishing local density of states at the Fermi level in graphene, the impurity spin cannot be effectively screened out.…

Strongly Correlated Electrons · Physics 2011-06-30 Chunhua Li , Jian-Xin Zhu , C. S. Ting

Combining density-functional theory calculations and microscopic tight-binding models, we investigate theoretically the electronic and magnetic properties of individual substitutional transition-metal impurities (Mn and Fe) positioned in…

Materials Science · Physics 2014-04-18 M. R. Mahani , M. Fhokrul Islam , A. Pertsova , C. M. Canali

Electronic correlations and spin-orbit interactions in plutonium create variations in the bonding behavior of each of its allotropes. In $\delta$-Pu, the 5f electrons lie at the tipping point between itinerant and localized behavior which…

Materials Science · Physics 2024-05-16 Alexander R. Muñoz , Travis E. Jones

To resolve the microscopic origin of magnetism in the Fe2O3/FeTiO3-system, we have performed density functional theory calculations taking into account on-site Coulomb repulsion. By varying systematically the concentration, distribution and…

Materials Science · Physics 2009-09-23 Rossitza Pentcheva , Hasan Sadat Nabi