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An extensive series of neutron diffraction experiments and molecular dynamics simulations has shown that mixtures of methanol and water exhibit extended structures in solution despite the components being fully miscible in all proportions.…

Soft Condensed Matter · Physics 2009-11-10 L. Dougan , S. P. Bates , R. Hargreaves , J. P. Fox , J. Crain , J. L. Finney , V. Reat , A. K. Soper

Methanol-water liquid mixtures have been investigated by high-energy synchrotron X-ray and neutron diffraction at low temperatures. We are thus able to report the first complete sets of both X-ray and neutron weighted total scattering…

Binary mixtures of water with lower alcohols display non-linear phase behaviour upon mixing which are attributed to potential cluster formation at molecular level. Unravelling such elusive structures requires the investigation of…

Soft Condensed Matter · Physics 2023-10-09 Riccardo Morbidini , Robert M. Edkins , Mark Devonport , Gøran Nilsen , Tilo Seydel , Katharina Edkins

The hydrogen-bonded structure of methanol-water mixtures is investigated over the entire alcohol concentration range (from $x_{\mathrm{Methanol}}=$ 0.1 to 1.0) at several temperatures, from 300 K down to the freezing point of the given…

Chemical Physics · Physics 2023-07-07 Ildikó Pethes , László Pusztai , László Temleitner

Results of systematic molecular dynamics studies of ethanol-water mixtures, over the entire concentration range, were reported previously to agree with experimental X-ray diffraction data. These simulated systems are analyzed in this work…

Soft Condensed Matter · Physics 2017-09-14 Orsolya Gereben , László Pusztai

We have investigated the hydrogen-bonded structures in liquid methanol and a 7:3 mole fraction aqueous solution using classical Molecular Dynamics simulations at 298K and ambient pressure. We find that, in contrast to recent predictions…

Soft Condensed Matter · Physics 2009-11-10 Susan K. Allison , Joseph P. Fox , Rowan Hargreaves , Simon P. Bates

Extensive molecular dynamics computer simulations have been conducted for ethanol-water liquid mixtures in the water-rich side of the composition range, with 10, 20 and 30 mol % of the alcohol, at temperatures between room temperature and…

Chemical Physics · Physics 2019-06-12 Szilvia Pothoczki , László Pusztai , Imre Bakó

Discrete element method simulations of confined bidisperse granular shear flows elucidate the balance between diffusion and segregation that can lead to either mixed or segregated states, depending on confining pressure. Results indicate…

Soft Condensed Matter · Physics 2018-09-24 Alexander M. Fry , Paul B. Umbanhowar , Julio M. Ottino , Richard M. Lueptow

New X-ray and neutron diffraction experiments have been performed on ethanol-water mixtures as a function of decreasing temperature, so that such diffraction data are now available over the entire composition range. Extensive molecular…

Soft Condensed Matter · Physics 2021-08-05 Szilvia Pothoczki , Ildikó Pethes , László Pusztai , László Temleitner , Koji Ohara , Imre Bakó

In this study some properties of the methanol-water mixture such as diffusivity, density, viscosity, and hydrogen bonding were calculated at different temperatures and atmospheric pressure using molecular dynamics simulations (MDS). The…

Atomic and Molecular Clusters · Physics 2017-08-08 Palazzo Mancini , Mara Cantoni

Since the structural transformations observed in water-ethanol binary mixtures are apparently driven by relatively weak intermolecular forces (like hydrophobicity and hydrogen bonding) that often cooperate to form self assembled structures,…

Soft Condensed Matter · Physics 2016-05-03 Rikhia Ghosh , Biman Bagchi

Efficient and sustainable techniques for separating water-methanol mixtures are in high demand in the industry. Recent studies have revealed that membranes and 2D materials could achieve such separation. In our research, we explore the…

Soft Condensed Matter · Physics 2023-06-28 Roger Bellido-Peralta , Fabio Leoni , Carles Calero , Giancarlo Franzese

We have investigated thermodynamic and dynamic properties as well as the dielectric constant of water-metha\-nol model mixtures in the entire range of composition by using constant pressure molecular dynamics simulations at ambient…

Soft Condensed Matter · Physics 2015-12-25 E. Galicia-Andrés , H. Dominguez , L. Pusztai , O. Pizio

We present a density-functional theory based molecular-dynamics study of the structural, dynamical, and electronic properties of liquid methanol under ambient conditions. The calculated radial distribution functions involving the oxygen and…

Chemical Physics · Physics 2009-11-07 Jan-Willem Handgraaf , Titus S. van Erp , Evert Jan Meijer

We report the temperature, pressure and composition dependence of some basic properties of model liquid water-methanol mixtures. For this purpose the isobaric-isothermal molecular dynamics computer simulations are employed. Our principal…

Soft Condensed Matter · Physics 2025-04-01 M. Cruz Sanchez , V. Trejos Montoya , O. Pizio

We investigate the segregation of a dense binary mixture of granular particles that only differ in their restitution coefficient. The mixture is vertically vibrated in the presence of gravity. We find a partial segregation of the species,…

Statistical Mechanics · Physics 2009-11-13 R. Brito , H. Enríquez , S. Godoy , R. Soto

We explored the composition dependence of a rather comprehensive set of properties of liquid water-ethanol mixtures by using the isobaric-isothermal molecular dynamics computer simulations. The united atom non-polarizable model from the…

Soft Condensed Matter · Physics 2024-07-02 D. Benavides Bautista , M. Aguilar , O. Pizio

We explore the effects of composition and temperature on the apparent molar volumes of species of water-methanol mixtures. Isothermal-isobaric molecular dynamics simulations are used with this purpose. Several combinations of models for…

Soft Condensed Matter · Physics 2021-01-20 M. Cruz Sanchez , M. Aguilar , O. Pizio

Aqueous solutions of LiCl are probably the most studied electrolyte solutions related to the complexity of liquid water at low temperatures. Despite the large amount of available experimental data hardly any computational studies were…

Soft Condensed Matter · Physics 2020-04-29 Philip H. Handle

Granular media are examined with the focus on polydisperse mixtures in the presence of two localized heat-baths. If the two driving energies are similar, the large particles prefer to stay in the `cold' regions of the system -- as far away…

Statistical Mechanics · Physics 2007-05-23 S. Luding , O. Strauss , S. McNamara
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