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The temperature dependent ac and dc magnetization and heat capacity data of Ca$_3$CoIrO$_6$, a spin-chain compound crystallizing in a K$_4$CdCl$_6$-derived rhombohedral structure, show the features due to magnetic ordering of a…

Strongly Correlated Electrons · Physics 2009-11-10 S. Rayaprol , Kausik Sengupta , E. V. Sampathkumaran

A quasi one-dimensional compound, Ca3CuRuO6, has been synthesized by solid-state reaction method and studied using magnetization (M) and heat capacity (C) measurements. This compound undergoes magnetic ordering (T_o) around 40 K, as…

Strongly Correlated Electrons · Physics 2016-08-31 S. Rayaprol , E. V. Sampathkumaran

The results of x-ray diffraction, and ac and dc magnetization as a function of temperature are reported for a new class of spin-chain oxides, Ca3Co1+xIr1-xO6. While the x= 0.0, 0.3, 0.5 and 1.0 are found to form in the K4CdCl6-derived…

Materials Science · Physics 2007-05-23 S. Rayaprol , Kausik Sengupta , E. V. Sampathkumaran

The results of ac and dc magnetization and heat capacity measurements as a function of temperature (T = 1.8 to 300 K) are reported for a quasi-one-dimensional compound, Ca$_3$CuMnO$_6$, crystallizing in a triclinically distorted…

Strongly Correlated Electrons · Physics 2009-11-10 Kausik Sengupta , S. Rayaprol , K. K. Iyer , E. V. Sampathkumaran

We report the results of ac and dc magnetic susceptibility (chi), heat-capacity (C), isothermal magnetization and isothermal remanent magnetization measurements on the compound, Sr3CuRhO6, crystallizing in a K4CdCl6-derived monoclinic…

Strongly Correlated Electrons · Physics 2007-05-23 E. V. Sampathkumaran , Niharika Mohapatra , Sudhindra Rayaprol , Kartik K Iyer

The dielectric behavior of the single crystals of the spin-chain system Ca3Co2O6, undergoing geometrically frustrated antiferromagnetic ordering below 25 K, has been investigated as a function of temperature and magnetic field (H) and…

Materials Science · Physics 2016-03-17 Tathamay Basu , Kartik K. Iyer , P. L. Paulose , E. V. Sampathkumaran

The results of ac and dc magnetization and heat capacity measurements on the oxides, Ca$_3$Co$_{1+x}$Mn$_{1-x}$O$_6$, forming in a K$_4$CdCl$_6$-derived rhombohedral quasi-one-dimensional crystal structure, are reported. As far as…

Strongly Correlated Electrons · Physics 2009-11-10 S. Rayaprol , Kausik Sengupta , E. V. Sampathkumaran

We have investigated the magnetic, dielectric and magnetodielectric (MDE) behavior of a geometrically frustrated spin-chain system, Ca3Co1.4Rh0.6O6, in the single crystalline form for different orientations. The results bring out that the…

Strongly Correlated Electrons · Physics 2015-06-22 Tathamay Basu , Kartik K. Iyer , Kiran Singh , K. Mukherjee , P. L. Paulose , E. V. Sampathkumaran

We report that the major features in the temperature dependence of dc and ac magnetization of a well-known spin-chain compound, Ca3Co2O6, which has been known to exhibit two complex magnetic transitions due to geometrical frustration (one…

Strongly Correlated Electrons · Physics 2015-05-13 Niharika Mohapatra , Kartik K Iyer , Sitikantha D Das , B. A. Chalke , S. C. Purandare , E. V. Sampathkumaran

The magnetic behavior of a solid solution, Ca3-xYxCo2O6, based on an exotic spin-chain compound, Ca3Co2O6, crystallizing in K4CdCl6-derived rhombohedral structure is investigated. Among the compositions investigated (x= 0.0, 0.3, 0.5, 0.75…

Strongly Correlated Electrons · Physics 2009-11-11 S. Rayaprol , E. V. Sampathkumaran

To study the relationship between the properties of low-dimensional spin systems with weakly coupled Cu-triangles and their crystal structure, single crystals of $Cs_3Cu_3Cl_8OH$ (1) and the new $Cs_3Cu_3Cl_{7.6}Br_{0.4}OH$ (2) were grown.…

We present a detailed powder and single crystal neutron diffraction study of the spin chain compound Ca3Co2O6. Below 25 K, the system orders magnetically with a modulated partially disordered antiferromagnetic structure. We give a…

Strongly Correlated Electrons · Physics 2008-09-17 S. Agrestini , L. C. Chapon , A. Daoud-Aladine , J. Schefer , A. Gukasov , C. Mazzoli , M. R. Lees , O. A. Petrenko

The magnetic behavior of the Ca3Co2O6 spin chain compound is characterized by a large Ising-like character of its ferromagnetic chains, set on triangular lattice, that are antiferromagnetically coupled. At low temperature, T < 7K, the 3D…

Strongly Correlated Electrons · Physics 2007-05-23 A. Maignan , V. Hardy , S. Hebert , M. Drillon , M. R. Lees , O. Petrenko , D. Mc K. Paul , D. Khomskii

We report the results of ac and dc magnetization (M) and heat-capacity (C) measurements on the solid solution, Sr$_3$Cu$_{1-x}$Zn$_x$IrO$_6$. While the Zn end member is known to form in a rhombohedral pseudo one-dimensional K$_4$CdCl$_6$…

Strongly Correlated Electrons · Physics 2009-11-07 Asad Niazi , E. V. Sampathkumaran , P. L. Paulose , D. Eckert , A. Handstein , K. -H. Müller

We report temperature (T) dependence of dc magnetization, electrical resistivity (rho(T)), and heat-capacity of rare-earth (R) compounds, Gd3RuSn6 and Tb3RuSn6, which are found to crystallize in the Yb3CoSn6-type orthorhombic structure…

Strongly Correlated Electrons · Physics 2017-06-28 Sanjay K Upadhyay , Kartik K Iyer , E. V. Sampathkumaran

Heat-capacity (C) and ac susceptibility measurements have been performed on the spin-chain compounds, Sr3ZnRhO6 and Ca3NiMnO6, to establish their magnetic behavior and to explore whether there are magnetic frustration effects due to…

Strongly Correlated Electrons · Physics 2009-11-10 S. Rayaprol , Kausik Sengupta , E. V. Sampathkumaran , Y. Matsushita

We have investigated the magnetic behavior of the nano crystals, synthesized by high-energy ball-milling, for a well-known geometrically frustrated spin-chain system, Ca3CoRhO6, and compared its magnetic characteristics with those of the…

Strongly Correlated Electrons · Physics 2015-05-13 Niharika Mohapatra , Kartik K Iyer , B. A. Chalke , E. V. Sampathkumaran

Specific heat measurements were carried out on the closely related spin-chain oxides Ca3Co2O6 and Ca3CoRhO6. Both compounds consist of Ising magnetic chains that are arranged on a triangular lattice. The spin coupling along and between the…

Strongly Correlated Electrons · Physics 2009-11-10 V. Hardy , M. R. Lees , A. Maignan , S. Hebert , D. Flahaut , C. Martin , D. McK. Paul

We present electronic structure calculations for the one-dimensional magnetic chain compounds Ca_3CoRhO_6 and Ca_3FeRhO_6. The calculations are based on density functional theory and the local density approximation. We use the augmented…

Strongly Correlated Electrons · Physics 2008-01-26 V. Eyert , U. Schwingenschloegl , C. Hackenberger , T. Kopp , R. Fresard , U. Eckern

Materials based on a crown ether complex together with magnetic ions, especially Cu(II), can be used to synthesize new low dimesional quantum spin systems. We have prepared the new crown ether complex…

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