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The expression for the short-range effective interaction potential of "quasinulei"\, is derived based on the model of the "pure"\, Coulomb interaction. This model represents the equilibrium Coulomb system (CS) of interacting electrons and…

General Physics · Physics 2019-07-24 S. A. Trigger

The determination of the effective Coulomb interactions to be used in low-energy Hamiltonians for materials with strong electronic correlations remains one of the bottlenecks for parameter-free electronic structure calculations. We propose…

Strongly Correlated Electrons · Physics 2017-08-09 Priyanka Seth , Philipp Hansmann , Ambroise van Roekeghem , Loig Vaugier , Silke Biermann

In his Comment (cond-mat/0104060) to [Phys. Rev. E 60, 6530 (1999)], Mateescu shows that while the effective interactions remain repulsive when the specific size of the micro-ions is taken into account via a Modified Poisson-Boltzmann…

Statistical Mechanics · Physics 2009-11-07 E. Trizac , J-L Raimbault

The electrostatic interaction between pairs of spherical or macroscopically long, parallel cylindrical colloids trapped at fluid interfaces is studied theoretically for the case of small inter-particle separations. Starting from the…

Soft Condensed Matter · Physics 2018-11-30 Arghya Majee , Markus Bier , S. Dietrich

In aqueous solutions, dissolved ions interact strongly with the surrounding water, thereby modifying the solution properties in an ion-specific manner. These ion-hydration interactions can be accounted for theoretically on a mean-field…

Soft Condensed Matter · Physics 2014-04-22 Dan Ben-Yaakov , David Andelman , Rudi Podgornik , Daniel Harries

The equilibrium electric double layer (EDL) that surrounds the colloidal particles is determinant for the response of a suspension under a variety of static or alternating external fields. An ideal salt-free suspension is composed by the…

Soft Condensed Matter · Physics 2017-09-13 R. Roa , F. Carrique , E. Ruiz-Reina

The ion-induced long-range orientational order between water molecules recently observed in second harmonic scattering experiments and illustrated with large scale molecular dynamics simulations is quantitatively explained using the…

Chemical Physics · Physics 2018-03-29 Luc Belloni , Daniel Borgis , Maximilien Levesque

We study suspensions of hydrophobic charged colloidal spheres dispersed in a demixed oil-water mixture by means of a modified Poisson-Boltzmann theory, taking into account image charge effects and partitioning of the monovalent ions. We…

Soft Condensed Matter · Physics 2016-08-14 Jos Zwanikken , René van Roij

We present a new approximation to ionic conductivity well suited to dynamical atomic-scale simulations, based on the Nernst-Einstein equation. In our approximation, ionic aggregates constitute the elementary charge carriers, and are…

Chemical Physics · Physics 2019-04-10 Arthur France-Lanord , Jeffrey C. Grossman

We study sedimentation equilibrium of low-salt suspensions of binary mixtures of charged colloids, both by Monte Carlo simulations of an effective colloids-only system and by Poisson-Boltzmann theory of a colloid-ion mixture. We show that…

Soft Condensed Matter · Physics 2009-11-11 M. Dijkstra , J. Zwanikken , R. van Roij

We describe arrangements of ions capable of producing short-range attractive interactions between pairs of charged colloidal spheres in the low temperature strongly correlated limit. For particles of radius $R$ with bare charge $Z$ and…

Strongly Correlated Electrons · Physics 2007-05-23 Francisco J. Solis , Monica Olvera de la Cruz

The interaction between charged bodies in an ionic solution is a general problem in colloid physics and becomes a central topic in the study of biological systems where the electrostatic interaction between proteins, nucleic acids,…

Soft Condensed Matter · Physics 2015-05-13 Fabien Paillusson , Maria Barbi , Jean-Marc Victor

We investigate, within a local density functional theory formalism, the interactions between like-charged polyions immersed in a confined electrolyte. We obtain a simple condition for a repulsive effective pair potential, that can be…

Soft Condensed Matter · Physics 2009-10-31 E. Trizac

The past two decades have seen a remarkable progress in the development of synthetic colloidal agents which are capable of creating directed motion in an unbiased environment at the microscale. These self-propelling particles are often…

Soft Condensed Matter · Physics 2023-02-10 Benno Liebchen , Aritra K. Mukhopadhyay

Criticality in a fluid of dielectric constant D that exhibits Ising-type behavior is studied as additional electrostatic (i.e., ionic) interactions are turned on. An exploratory perturbative calculation is performed for small ionicity as…

Soft Condensed Matter · Physics 2009-10-31 A. G. Moreira , M. M. Telo da Gama , M. E. Fisher

While the density functional theory with integral equations techniques are very efficient tools in numerical analysis of complex fluids, an analytical insight into the phenomenon of effective interactions is still limited. In this paper we…

Soft Condensed Matter · Physics 2014-09-24 M. Majka , P. F. Góra

Interaction non-additivity in the chemical context means that binding of certain atom to a reference atom cannot be fully predicted from the interactions of these two atoms with other atoms. This constitutes one of key phenomena determining…

Chemical Physics · Physics 2015-02-24 Vitaly V. Chaban , Oleg V. Prezhdo

Thermodynamic properties of charge-stabilised colloidal suspensions depend sensitively on the effective charge of the macroions, which can be substantially lower than the bare charge in the case of strong counterion-macroion association. A…

Soft Condensed Matter · Physics 2011-06-28 Alan R. Denton

Effective interactions inherently encompass many-body effects that appear unified. Analyzing these in reverse, that is, separating them into contributions from pairs, triples, or larger groups, is typically intricate and seldom pursued.…

A new computational method is presented for study suspensions of charged soft particles undergoing fluctuating hydrodynamic and electrostatic interactions. The proposed model is appropriate for polymers, proteins and porous particles…

Soft Condensed Matter · Physics 2015-04-14 Juan P. Hernandez-Ortiz , Juan J. de Pablo
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