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We introduce the Korringa-Kohn-Rostocker non-local coherent potential approximation (KKR-NLCPA) for describing the electronic structure of disordered systems. The KKR-NLCPA systematically provides a hierarchy of improvements upon the widely…

Materials Science · Physics 2009-11-07 D. A. Rowlands , J. B. Staunton , B. L. Gyorffy

The single-site Korringa-Kohn-Rostoker Coherent Potential Approximation (KKR-CPA) ignores short range ordering present in disordered metallic systems. In this paper, we establish a new technique to fix this shortcoming by embedding an…

Materials Science · Physics 2020-08-26 Vishnu Raghuraman , Yang Wang , Michael Widom

We present an ab-initio formalism for the calculation of transport properties in compositionally disordered systems within the framework of the Korringa-Kohn-Rostoker non-local coherent potential approximation. Our formalism is based upon…

Materials Science · Physics 2009-11-13 P. R. Tulip , J. B. Staunton , S. Lowitzer , D. Ködderitzsch , H. Ebert

We investigate the effect of short-range order (SRO) on the electronic structure in alloys from the theoretical point of view using density of states (DOS) data. In particular, the interaction between the atoms at different lattice sites is…

We extend the single-site coherent potential approximation (CPA) to include the effects of non-local disorder correlations (alloy short-range order) on the electronic structure of random alloy systems. This is achieved by mapping the…

Strongly Correlated Electrons · Physics 2009-11-10 M. S. Laad , L. Craco

The method of electronic structure calculations for strongly correlated disordered materials is developed employing the basic idea of coherent potential approximation (CPA). Evolution of electronic structure and spin magnetic moment value…

Strongly Correlated Electrons · Physics 2014-02-28 M. A. Korotin , Z. V. Pchelkina , N. A. Skorikov , E. Z. Kurmaev , V. I. Anisimov

We apply variational principles from statistical physics and the Landau theory of phase transitions to multicomponent alloys using the multiple-scattering theory of Korringa-Kohn-Rostoker (KKR) and the coherent potential approximation…

Materials Science · Physics 2016-02-24 Suffian N. Khan , J. B. Staunton , G. M. Stocks

We present first principles charge- and spin-selfconsistent electronic structure computations on the Heusler-type disordered alloys Fe$_{3-x}$V$_{x}$X for three different metalloids X=(Si, Ga and Al). In these calculations we use the…

Materials Science · Physics 2009-10-31 A. Bansil , S. Kaprzyk , P. E. Mijnarends , J. Toboła

A scheme to calculate the electronic structure of systems having a spiral magnetic structure is presented. The approach is based on the KKR (Korringa-Kohn-Rostoker) Green's function formalism which allows in combination with CPA (Coherent…

Strongly Correlated Electrons · Physics 2013-08-08 S. Mankovsky , G. H. Fecher , H. Ebert

Chemical short-range order (SRO) affects the distribution of elements throughout the solid-solution phase of metallic alloys, thereby modifying the background against which microstructural evolution occurs. Investigating such…

Materials Science · Physics 2024-07-10 Yifan Cao , Killian Sheriff , Rodrigo Freitas

Recently the nonlocal coherent-potential approximation (NLCPA) has been introduced by Jarrell and Krishnamurthy for describing the electronic structure of substitutionally disordered systems. The NLCPA provides systematic corrections to the…

Materials Science · Physics 2009-11-11 D. A. Rowlands

Electronic-structure methods based on density-functional theory (DFT) were used to directly quantify the effect of chemical short-range order (SRO) on thermodynamic, structural, and electronic properties of archetypal face-centered-cubic…

Materials Science · Physics 2023-05-16 Will Morris , Duane D. Johnson , Prashant Singh

We here study electronic structure and magnetic properties of disordered CoPd and CoPt alloys using Augmented Space Recursion technique coupled with the tight-binding linearized muffin tin orbital (TB-LMTO) method. Effect of short range…

Materials Science · Physics 2019-08-17 Subhradip Ghosh , Chhanda Basu Chaudhuri , Biplab Sanyal , Abhijit Mookerjee

The equilibrium short-range order (SRO) in Cu-Pd alloys is studied theoretically. The evolution of the Fermi surface-related splitting of the (110) diffuse intensity peak with changing temperature is examined. The results are compared with…

Statistical Mechanics · Physics 2009-10-31 I. Tsatskis , E. K. H. Salje

A general method is proposed for calculating a fully k-dependent, continuous, and causal spectral function A(k,E) within the recently introduced nonlocal version of the coherent-potential approximation (NLCPA). The method involves the…

Materials Science · Physics 2009-11-11 G. M. Batt , D. A. Rowlands

An idealized high entropy oxide is characterized by perfect chemical disorder and perfect positional order. In this work, we investigate the extent to which short-range order (SRO) and local structural distortions impede that idealized…

The electronic, magnetic and transport properties of Fe intercalated 2H-TaS$_2$ have been investigated by means of the Korringa-Kohn-Rostoker (KKR) method. The non-stoichiometry and disorder in the system has been accounted for using the…

Mesoscale and Nanoscale Physics · Physics 2015-10-21 S. Mankovsky , K. Chadova , D. Ködderitzsch , W. Bensch , H. Ebert

The random phase approximation (RPA) for the correlation energy functional of density functional theory has recently attracted renewed interest. Formulated in terms of the Kohn-Sham (KS) orbitals and eigenvalues, it promises to resolve some…

Other Condensed Matter · Physics 2009-11-13 Hong Jiang , Eberhard Engel

The theoretical description of modern nanoelectronic devices requires a quantum mechanical treatment and often involves disorder, e.g. form alloys. Therefore, the ab initio theory of transport using non-equilibrium Green's functions is…

Mesoscale and Nanoscale Physics · Physics 2014-02-07 Christian Franz , Michael Czerner , Christian Heiliger

Traditional metallic alloys are mixtures of elements where the atoms of minority species tend to distribute randomly if they are below their solubility limit, or lead to the formation of secondary phases if they are above it. Recently, the…

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