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We present a joint implementation of dynamical-mean-field theory (DMFT) with the pseudopotential plane-wave approach, via Wannier functions, for the determination of the electronic properties of strongly correlated materials. The scheme…

Strongly Correlated Electrons · Physics 2018-08-08 G. Trimarchi , I. Leonov , N. Binggeli , Dm. Korotin , V. I. Anisimov

We have constructed maximally-localized Wannier functions for prototype structures of solid molecular hydrogen under pressure, starting from LDA and tight-binding Bloch wave functions. Each occupied Wannier function can be associated with…

Materials Science · Physics 2009-10-31 Ivo Souza , Richard M. Martin , Nicola Marzari , Xinyuan Zhao , David Vanderbilt

In designing and optimizing new-generation nanomaterials and related quantum devices, dissipation versus decoherence phenomena are often accounted for via local scattering models, such as relaxation-time and Boltzmann-like schemes. Here we…

Mesoscale and Nanoscale Physics · Physics 2017-09-14 Rita Claudia Iotti , Fabrizio Dolcini , Fausto Rossi

The ionization potential of molecular chains is well-known to be a tunable nano-scale property that exhibits clear quantum confinement effects. State-of-the-art methods can accurately predict the ionization potential in the small molecule…

Chemical Physics · Physics 2024-03-28 Guy Ohad , Michal Hartstein , Tim Gould , Jeffrey B. Neaton , Leeor Kronik

We investigate a recently developed approach [P. L. Silvestrelli, Phys. Rev. Lett. 100, 053002 (2008); J. Phys. Chem. A 113, 5224 (2009)] that uses maximally localized Wannier functions to evaluate the van der Waals contribution to the…

Materials Science · Physics 2012-06-12 Lampros Andrinopoulos , Nicholas D. M. Hine , Arash A. Mostofi

We introduce a Wannier-type formulation of periodic local vibrational mode theory that yields real-space-localized vibrational modes associated with individual internal coordinates in crystalline solids. These modes are constructed as…

Materials Science · Physics 2026-05-12 Mateusz Mojsak , Elfi Kraka , Adam A. L. Michalchuk

We present a mixed basis-set approach to obtain optical absorption spectra within a generalized Kohn-Sham time-dependent density functional theory framework. All occupied valence molecular orbitals (MOs) are expanded in a plane-wave (PW)…

Chemical Physics · Physics 2025-08-13 Kyle Chen , Barry Y. Li , Tucker Allen , Daniel Neuhauser

A new implementation is proposed for including van der Waals (vdW) interactions in Density Functional Theory (DFT) using the Maximally-Localized Wannier functions (MLWFs), which is free from empirical parameters. With respect to the…

Chemical Physics · Physics 2019-05-22 Pier Luigi Silvestrelli , Alberto Ambrosetti

Density functional theory (DFT) embedding provides a formally exact framework for interfacing correlated wave-function theory (WFT) methods with lower-level descriptions of electronic structure. Here, we report techniques to improve the…

Chemical Physics · Physics 2015-06-12 Jason D. Goodpaster , Taylor A. Barnes , Frederick R. Manby , Thomas F. Miller

The DFT/vdW-WF2s1 method based on the generation of localized Wannier functions, recently developed to include the van der Waals interactions in the Density Functional Theory and describe adsorption processes on metal surfaces by taking…

Chemical Physics · Physics 2016-04-06 Pier Luigi Silvestrelli , Alberto Ambrosetti

Tight-binding models for ultracold atoms in optical lattices can be properly defined by using the concept of maximally localized Wannier functions for composite bands. The basic principles of this approach are reviewed here, along with…

Quantum Gases · Physics 2016-03-30 Michele Modugno , Julen Ibañez-Azpiroz , Giulio Pettini

There has been a high demand in rectifying the band gap under-estimation problem in density functional theory (DFT), while keeping the computational load at the same level as local density approximation. DFT-1/2 and shell DFT-1/2 are useful…

Materials Science · Physics 2025-07-08 Shengxin Yang , Jiangzhen Shi , Kan-Hao Xue , Jun-Hui Yuan , Xiangshui Miao

When the first four spectral moments are considered, spectral features missing in standard Kohn-Sham (KS) density-functional theory (DFT), such as upper and lower Hubbard bands, as well as spectral satellite peaks, can be described, and the…

Strongly Correlated Electrons · Physics 2023-01-13 Frank Freimuth , Stefan Blügel , Yuriy Mokrousov

We introduce a method for the selective preparation and detection of quasiparticle wave packets, based on creation operators that generate dressed, localized excitations on top of interacting vacua of (quasi-)one-dimensional quantum lattice…

Quantum Physics · Physics 2026-04-20 Mattia Morgavi , Peter Majcen , Marco Rigobello , Simone Montangero , Pietro Silvi

We present an approach to parameterize DFT+$U$+$V$ from hybrid-functional calculations using Wannier-function projections. The method constructs a common localized Wannier basis for both semilocal DFT and hybrid-functional calculations,…

Strongly Correlated Electrons · Physics 2026-02-25 Dmitry M. Korotin , Anna A. Anisimova , Vladimir I. Anisimov

Maximally localized Wannier functions (MLWFs) based on Kohn-Sham band-structures provide a systematic way to construct realistic, materials specific tight-binding models for further theoretical analysis. Here, we construct MLWFs for the Mn…

Strongly Correlated Electrons · Physics 2013-05-29 Roman Kovacik , Claude Ederer

We report a theoretical scheme that enables the calculation of maximally localized Wannier functions in the formalism of projector-augmented-waves (PAW) which also includes the ultrasoft-pseudopotential (USPP) approach. We give a…

Soft Condensed Matter · Physics 2007-05-23 Andrea Ferretti , Arrigo Calzolari , Benedetta Bonferroni , Rosa Di Felice

In a tight-binding lattice model with $n$ orbitals (single-particle states) per site, Wannier functions are $n$-component vector functions of position that fall off rapidly away from some location, and such that a set of them in some sense…

Mesoscale and Nanoscale Physics · Physics 2017-03-29 N. Read

We shall revisit the conventional treatment of open quantum devices based on the Wigner-Function formalism. Our analysis will show that the artificial spatial separation between device active region and external reservoirs -properly defined…

Other Condensed Matter · Physics 2007-05-23 Luigi Genovese , David Taj , Fausto Rossi

This paper proposes a novel localized Fourier extension method for approximating non-periodic functions via domain segmentation. By partitioning the computational domain into subregions with uniform discretization scales, the method…

Numerical Analysis · Mathematics 2025-08-29 Zhenyu Zhao , Yanfei Wang
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