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Magnetization and neutron elastic scattering measurements under a hydrostatic pressure were performed on KCuCl3, which is a three-dimensionally coupled spin dimer system with a gapped ground state. It was found that an intradimer…

Under the hydrostatic pressure $P=1.48$ GPa, polarized neutron elastic scattering experiments have been carried out on the coupled spin dimer system TlCuCl$_3$ with the gapped ground state at ambient pressure. Pressure-induced magnetic…

Strongly Correlated Electrons · Physics 2009-11-10 A. Oosawa , K. Kakurai , T. Osakabe , M. Nakamura , M. Takeda , H. Tanaka

KCuCl$_3$ is a three dimensionally coupled spin dimer system, which undergoes a pressure-induced quantum phase transition from a gapped ground state to an antiferromagnetic state at a critical pressure of $P_{\rm c} \simeq 8.2$ kbar.…

Strongly Correlated Electrons · Physics 2009-11-13 K. Goto , T. Osakabe , K. Kakurai , Y. Uwatoko , A. Oosawa , J. Kawakami , H. Tanaka

We have performed magnetization measurements of the gapped quantum magnet CsFeCl$_3$ at temperatures ($T$) down to 0.5\,K at ambient pressure and down to 1.8\,K at hydrostatic pressures ($P$) of up to 1.5\,GPa. The lower-field ($H$) phase…

Strongly Correlated Electrons · Physics 2016-09-28 Nobuyuki Kurita , Hidekazu Tanaka

We carried out zero-field muon-spin-rotation (ZF-$\mu$SR) measurements in hydrostatic pressures in impurity-doped quantum spin gap system Tl(Cu$_{0.985}$Mg$_{0.015}$)Cl$_3$ to investigate microscopic magnetic properties of the…

Strongly Correlated Electrons · Physics 2015-05-18 Takao Suzuki , Isao Watanabe , Fumiko Yamada , Motoki Yamada , Yasuyuki Ishii , Takayuki Kawamata , Takayuki Goto , Hidekazu Tanaka

Magnetic phase transition under hydrostatic pressure in TlCu$_{0.988}$Mg$_{0.012}$Cl$_3$ was investigated by magnetization measurements. The parent compound TlCuCl$_3$ is a coupled spin dimer system, which undergoes a pressure-induced…

Strongly Correlated Electrons · Physics 2009-11-11 H. Imamura , T. Ono , K. Goto , H. Tanaka

We present thermal expansion alpha, magnetostriction and specific heat C measurements of \tal, which shows a quantum phase transition from a spin-gap phase to a Neel-ordered ground state as a function of magnetic field around H_{C0}->4.8T.…

Strongly Correlated Electrons · Physics 2009-11-11 T. Lorenz , S. Stark , O. Heyer , N. Hollmann , A. Vasiliev , A. Oosawa , H. Tanaka

Magnetization measurements under a hydrostatic pressure of P = 1.4 GPa were performed on the coupled spin dimer system TlCuCl_3, which exhibits a pressure-induced quantum phase transition from a gapped singlet state to an antiferromagnetic…

Strongly Correlated Electrons · Physics 2009-11-13 Fumiko Yamada , Yasuyuki Ishii , Takao Suzuki , Teiichiro Matsuzaki , Hidekazu Tanaka

Magnetic phase transitions under hydrostatic pressures in spin gap systems TlCu$_{0.988}$Mg$_{0.012}$Cl$_3$ and KCu$_{0.973}$Mg$_{0.027}$Cl$_3$ were investigated by magnetization measurements. The present doped systems exhibit…

Strongly Correlated Electrons · Physics 2015-06-25 T. Ono , H. Imamura , J. Kawakami , K. Goto , H. Tanaka

We present a thermal expansion and magnetostriction study of TlCuCl_3, which shows a magnetic-field induced transition from a spin gap phase to a Neel ordered phase. Using Ehrenfest relations we derive huge and strongly anisotropic uniaxial…

Strongly Correlated Electrons · Physics 2009-11-11 N. Johannsen , A. Oosawa , H. Tanaka , A. Vasiliev , T. Lorenz

Thallium copper chloride is a quantum spin liquid of S = 1/2 Cu^2+ dimers. Interdimer superexchange interactions give a three-dimensional magnon dispersion and a spin gap significantly smaller than the dimer coupling. This gap is closed by…

Strongly Correlated Electrons · Physics 2009-11-10 M. Matsumoto , B. Normand , T. M. Rice , M. Sigrist

Magnetization measurements were performed on TlCuCl$_3$ with gapped ground state. The critical density and the magnetic phase diagram were obtained. The interacting constant was obtained as $U/k_{\rm B} = 313$ K. The experimental phase…

Strongly Correlated Electrons · Physics 2015-06-25 F. Yamada , T. Ono , M. Fujisawa , H. Tanaka , T. Sakakibara

We present high-resolution measurements of the thermal expansion and the magnetostriction of TlCuCl$_{3}$ which shows field-induced antiferromagnetic order. We find pronounced anomalies in the field and temperature dependence of different…

Strongly Correlated Electrons · Physics 2009-11-10 N. Johannsen , A. Vasiliev , A. Oosawa , H. Tanaka , T. Lorenz

We report high-pressure magnetization and $^{35}$Cl NMR studies on $\alpha$-RuCl$_3$ with pressure up to 1.5~GPa. At low pressures, the magnetic ordering is identified by both the magnetization data and the NMR data, where the $T_N$ shows a…

Strongly Correlated Electrons · Physics 2017-12-06 Y. Cui , J. Zheng , K. Ran , Jinsheng Wen , Zhengxin Liu , B. Liu , Wenan Guo , Weiqiang Yu

Neutron elastic scattering measurements have been performed under the hydrostatic pressure in order to investigate the spin structure of the pressure-induced magnetic ordering in the spin gap system TlCuCl$_3$. Below the ordering…

Strongly Correlated Electrons · Physics 2009-11-10 A. Oosawa , M. Fujisawa , T. Osakabe , K. Kakurai , H. Tanaka

The magnetization measurements have been performed on the doped spin gap system TlCu_{1-x}Mg_xCl_3 with x <= 0.025. The parent compound TlCuCl_3 is a three-dimensional coupled spin dimer system with the excitation gap Delta/k_B = 7.7 K. The…

Strongly Correlated Electrons · Physics 2009-11-07 A. Oosawa , T. Ono , H. Tanaka

KCuCl$_3$ is a three-dimensional coupled spin-dimer system and has a singlet ground state with an excitation gap ${\Delta}/k_{\rm B}=31$ K. High-field magnetization measurements for KCuCl$_3$ have been performed in static magnetic fields of…

Strongly Correlated Electrons · Physics 2009-11-07 A. Oosawa , T. Takamasu , K. Tatani , H. Abe , N. Tsujii , O. Suzuki , H. Tanaka , G. Kido , K. Kindo

Using dc and ac magnetometry, the pressure dependence of the magnetization of the three-dimensional antiferromagnetic coordination polymer Mn(N(CN)$_{2}$)$_{2}$ was studied up to 12 kbar and down to 8K. The magnetic transition temperature,…

Materials Science · Physics 2015-02-03 P. A. Quintero , D. Rajan , M. K. Peprah , T. V. Brinzari , R. S. Fishman , D. R. Talham , M. W. Meisel

TlCuCl3 shows a quantum phase transition from a spin-gap phase to a Neel-ordered ground state as a function of magnetic field around H_{C0}~4.8T. From measurements of the specific heat c and the linear thermal expansion alpha_i we calculate…

Strongly Correlated Electrons · Physics 2015-06-25 S. Stark , O. Heyer , A. Vasiliev , A. Oosawa , H. Tanaka , T. Lorenz

Specific heat measurements have been performed in the coupled dimer system TlCuCl$_3$, which has a singlet ground state with the excitation gap $\Delta \simeq 7.5$K. The cusplike anomaly indicative of the 3D magnetic ordering was clearly…

Strongly Correlated Electrons · Physics 2009-10-31 A. Oosawa , H. Aruga Katori , H. Tanaka
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