Related papers: Mesoscopic quantum coherence in antiferromagnetic …
We study macroscopic quantum coherence in antiferromagnetic molecular magnets in the presence of magnetic fields. Such fields generate artificial tunnel barriers with externally tunable strength. We give detailed semi-classical predictions…
The inelastic neutron scattering (INS) spectrum is studied for the antiferromagnetic molecular wheel CsFe8, in the temperature range 2 - 60 K, and for transfer energies up 3.6 meV. A qualitative analysis shows that the observed peaks…
The antiferromagnetic molecular wheel Fe18 of eighteen exchange-coupled Fe(III) ions has been studied by measurements of the magnetic torque, the magnetization, and the inelastic neutron scattering spectra. The combined data show that the…
Based on numerical calculations it is shown that the antiferromagnetic grid molecule Mn-[3 x 3] is a very promising candidate to experimentally detect the phenomenon of quantum tunneling of the Neel vector.
We study theoretically the spin dynamics of the ferric wheel, an antiferromagnetic molecular ring. For a single nuclear or impurity spin coupled to one of the electron spins of the ring, we calculate nuclear and electronic spin correlation…
We present detailed calculations of low-energy spin dynamics in the ``ferric wheel'' systems Na:Fe_6 and Cs:Fe_8 in a magnetic field. We compute by exact diagonalisation the low-energy spectra and matrix elements for total-spin and…
The macroscopic quantum coherence in a biaxial antiferromagnetic molecular magnet in the presence of magnetic field acting parallel to its hard anisotropy axis is studied within the two-sublattice model. On the basis of instanton technique…
We study theoretically the thermodynamic properties and spin dynamics of a class of magnetic rings closely related to ferric wheels, antiferromagnetic ring systems, in which one of the Fe (III) ions has been replaced by a dopant ion to…
Macroscopic quantum coherence oscillations in mesoscopic antiferromagnets may appear when the anisotropy potential creates a barrier between the antiferromagnetic states with opposite orientations of the Neel vector. This phenomenon is…
The detailed theoretical understanding of quantum spin dynamics in various molecular magnets is an important step on the roadway to technological applications of these systems. Quantum effects in both ferromagnetic and antiferromagnetic…
We study macroscopic quantum coherence (MQC) in small ferrimagnets. Through semi-classical calculations we show that even a small uncompensated moment has a drastic effect on MQC. In particular, there is a rapid crossover to a regime where…
The tunnel splitting in biaxial antiferromagnetic particles is studied with a magnetic field applied along the hard anisotropy axis. We observe the oscillation of tunnel splitting as a function of the magnetic field due to the quantum phase…
The magnetic behaviour of nanoparticles of antiferromagnetic ferritin, with a mean Fe loading of 410 atoms per core, has been investigated by 57Fe Mossbauer absorption spectroscopy down to very low temperature (34mK). In previous experi-…
Mesoscopic quantum phase coherence is important because it improves the prospects for handling quantum degrees of freedom in technology. Here we show that the development of such coherence can be monitored using magnetic neutron scattering…
We generalize the Landau-Zener theory of coherent tunneling transitions by taking thermal relaxation into account. The evaluation of a new generalized master equation containing a dynamic tunneling rate that includes the interaction between…
We show that the cold atom systems of simultaneously trapped Bose-Einstein condensates (BEC's) and quantum degenerate fermionic atoms provide promising laboratories for the study of macroscopic quantum tunneling. Our theoretical studies…
An effective Hamiltonian, describing quantum tunneling in ferrimagnetic nanoparticles which includes interactions between the electronic spins of nanoparticle and microscopic environmental spins (like nuclear spins or paramagnetic…
The role of $S$-mixing in the quantum tunneling of the magnetization in nanomagnets has been investigated. We show that the effect on the tunneling frequency is huge and that the discrepancy (more than 3 orders of magnitude in the tunneling…
The spin-phase interference effects are studied analytically in resonant quantum tunneling of the N\'{e}el vector between degenerate excited levels in nanometer-scale single-domain antiferromagnets in the absence of an external magnetic…
The Landau Zener method allows to measure very small tunnel splittings \Delta in molecular clusters Fe_8. The observed oscillations of \Delta as a function of the magnetic field applied along the hard anisotropy axis are explained in terms…