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Alkali-doped fullerides exhibit a wealth of unusual phases that remain controversial by nature. Here we report a cryogenic scanning tunneling microscopy study of the sub-molecular structural and electronic properties of expanded fullerene…

Superconductivity · Physics 2020-02-26 Sha Han , Meng-Xue Guan , Can-Li Song , Yi-Lin Wang , Ming-Qiang Ren , Sheng Meng , Xu-Cun Ma , Qi-Kun Xue

Variations in the band structures of C60-polymers are studied, when conjugation conditions and the electron number are changed. We use a semiempirical model with the Su-Schrieffer-Heeger type electron-phonon interactions. In the neutral…

Materials Science · Physics 2016-08-31 Kikuo Harigaya

C60 fullerides are uniquely flexible molecular materials that exhibit a rich variety of behavior, including superconductivity and magnetism in bulk compounds, novel electronic and orientational phases in thin films, and quantum transport in…

Materials Science · Physics 2009-11-13 Yayu Wang , Ryan Yamachika , Andre Wachowiak , Michael Grobis , Michael F. Crommie

Using density functional methods we calculated structural and electronic properties of bulk chloroform and bromoform intercalated C60, C60 2CHX3 (X=Cl,Br). Both compounds are narrow band insulator materials with a gap between valence and…

Materials Science · Physics 2016-08-31 R. Windiks , A. Bill , B. Delley , V. Z. Kresin

Graphite is an example of a layered material that can be bent to form fullerenes which promise important applications in electronic nanodevices. The spheroidal geometry of a slightly elliptically deformed sphere was used as a possible…

Materials Science · Physics 2007-05-23 Richard Pincak , Michal Pudlak

The polarization-response spectrum of the fullerene C60 modeled as a homogeneous spherical plasma shell is calculated in the framework of the hydrodynamic approach allowing for the spatial dispersion caused by the Fermi-distributed valence…

Plasma Physics · Physics 2017-10-17 V. B. Gildenburg , I. A. Pavlichenko

We report temperature-dependent photoelectron spectra for a monolayer of C_60 adsorbed on HOPG, as well as C 1s x-ray absorption. This extends a previous report which showed the close similarity between the spectrum of the HOMO for the…

Strongly Correlated Electrons · Physics 2015-06-24 P. A. Bruhwiler , P. Baltzer , S. Andersson , D. Arvanitis , N. Martensson

Nanoclusters like fullerenes as the unit to build intriguing two-dimensional topological structures is of great challenge. Here we propose three bridged fullerene monolayers and comprehensively investigate the novel fullerene monolayer as…

Materials Science · Physics 2022-07-21 Linfeng Yu , Jinyuan Xu , Bo Peng , Guangzhao Qin , Gang Su

High resolution angle-resolved photoemission measurements have been carried out on (Sr,K)Fe$_2$As$_2$ superconductor (Tc=21 K). Three hole-like Fermi surface sheets are clearly resolved for the first time around the Gamma point. The overall…

Recent direct experimental observation of multiple highly-dispersive C$_{60}$ valence bands has allowed for a detailed analysis of the unique photoemission traits of these features through photon energy- and polarization-dependent…

Mesoscale and Nanoscale Physics · Physics 2023-01-18 Drew W. Latzke , Claudia Ojeda-Aristizabal , Jonathan D. Denlinger , Ryan Reno , Alex Zettl , Alessandra Lanzara

We use first principles density functional theory to calculate the electronic structure of the phenylthiolate (S-C$_6$H$_5$) self-assembled monolayer (SAM) on Cu(111) and Au(111) substrates. We find significant lateral dispersion of the SAM…

Materials Science · Physics 2009-11-10 Vasili Perebeinos , Marshall Newton

We study the electronic spectrum for doped electronic states in the orientationally disordered M3C60 fullerides. Momentum-resolved Green's functions are calculated within a cluster-Bethe-lattice model, and compared with results from…

Condensed Matter · Physics 2009-10-22 E. J. Mele , S. C. Erwin

The aim of the present study is to clarify the charge composition of fullerite C60 electron-beam dispersion (EBD) products and investigate the influence of fullerene ions and electrons on the structure of the deposited coatings by applying…

Materials Science · Physics 2012-08-06 Ihar Razanau , Tetsu Mieno , Victor Kazachenko

By the first-principles electronic structure calculations, we have studied electronic structures of FeSe monolayer and bilayer thin films on SrTiO$_3$ (001) with SrO-termination or TiO$_2$ termination. We find that both FeSe monolayer and…

Superconductivity · Physics 2012-06-18 Kai Liu , Zhong-Yi LU , Tao Xiang

Silver films were deposited at room temperature onto H-passivated Si(111) surfaces. Their electronic properties have been analyzed by angle-resolved photoelectron spectroscopy. Submonolayer films were semiconducting and the onset of…

Materials Science · Physics 2009-11-07 A. Arranz , J. F. Sanchez-Royo , J. Avila , V. Perez-Dieste , P. Dumas , M. C. Asensio

The first angle-resolved photoemission spectroscopy results from MgB$_2$ single crystals are reported. Close to the $\Gamma$K and $\Gamma$M directions, three distinct dispersions are observed approaching the Fermi energy, as can be assigned…

Superconductivity · Physics 2016-08-31 H. Uchiyama , K. M. Shen , S. Lee , A. Damascelli , D. H. Lu , D. L. Feng , Z. -X. Shen , S. Tajima

The orientation of luminescent molecules in organic light-emitting diodes (OLEDs) strongly influences device performance. However, our understanding of the factors controlling emitter orientation is limited as current measurements only…

The polymer phases of AC60 form distinct crystal structures characterized by the mutual orientations of the (C60-)n chains. We show that the direct electric quadrupole interaction between chains always favors the orthorhombic structure Pmnn…

Materials Science · Physics 2009-10-31 K. H. Michel , A. V. Nikolaev

We investigate the electronic reconstruction across the tetragonal-orthorhombic structural transition in FeSe by employing polarization-dependent angle-resolved photoemission spectroscopy (ARPES) on detwinned single crystals. Across the…

Starting from a model of rigid interacting C60 polymer chains on an orthorhombic lattice, we study the mutual orientation of the chains and the stability of the crystalline structures Pmnn and I2/m. We take into account i) van der Waals…

Materials Science · Physics 2012-08-17 B. Verberck , K. H. Michel , A. V. Nikolaev
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