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Metal-insulator transitions involve a mix of charge, spin, and structural degrees of freedom, and when strongly-correlated, can underlay the emergence of exotic quantum states. Mott insulators induced by the opening of a Coulomb gap are an…

Strongly Correlated Electrons · Physics 2021-05-14 Yejun Feng , Yishu Wang , D. M. Silevitch , S. E. Cooper , D. Mandrus , Patrick A. Lee , T. F. Rosenbaum

The popular dual electronic (Mott) and structural (Peierls) transitions in VO2 are explored using x-ray absorption spectromicroscopy with high spatial and spectral resolutions. It is found that during both heating and cooling, the…

Strongly Correlated Electrons · Physics 2015-11-20 Suhas Kumar , John Paul Strachan , Matthew D. Pickett , Alexander Bratkovsky , Yoshio Nishi , R. Stanley Williams

The Mott insulator $\beta'$-EtMe$_3$Sb[Pd(dmit)$_2$]$_2$ belongs to a class of charge transfer solids with highly-frustrated triangular lattice of $S=1/2$ molecular dimers and a quantum-spin-liquid ground state. Our experimental and ab…

Strongly Correlated Electrons · Physics 2018-06-27 P. Lazić , M. Pinterić , D. Rivas Góngora , A. Pustogow , K. Treptow , T. Ivek , O. Milat , B. Gumhalter , N. Došlić , M. Dressel , S. Tomić

Strong correlation effects, such as a dramatic increase in the effective mass of the carriers of electricity, recently observed in the low density electron gas have provided spectacular support for the existence of a sharp metal-insulator…

Strongly Correlated Electrons · Physics 2009-11-13 A. Camjayi , K. Haule , V. Dobrosavljevic , G. Kotliar

In order to study the origin of metallization of VO$_2$ induced by electron injection, we deposit K atoms onto the surface of VO$_2$ films grown on TiO$_2$ (001) substrates, and we investigate the change in the electronic and crystal…

Strongly Correlated Electrons · Physics 2019-03-27 Daisuke Shiga , Makoto Minohara , Miho Kitamura , Ryu Yukawa , Koji Horiba , Hiroshi Kumigashira

Although vanadium dioxide (VO2) exhibits the most abrupt metal to insulator transition (MIT) properties near room-temperature, the present regulation of their MIT functionalities is insufficient owing to the high complexity and susception…

Materials Science · Physics 2023-01-03 Xuanchi Zhou , Yuchen Cui , Yanlong Shang , Haifan Li , Jiaou Wang , Ye Meng , Xiaoguang Xu , Yong Jiang , Nuofu Chen , Jikun Chen

Recently the memristive electrical transport properties in NbO$_2$ have attracted much attention for their promising application to the neuromorphic computation. At the center of debates is whether the metal-to-insulator transition (MIT)…

Mesoscale and Nanoscale Physics · Physics 2022-10-20 Samuel W. Olin , S. Abdel Razek , L. F. J. Piper , Wei-Cheng Lee

VO2, of interest for decades due to both its phenomenology and its potential applications, has a monoclinic distortion of the rutile crystal structure at ambient temperature that is coupled to its metal-insulator transition (MIT). In…

Materials Science · Physics 2022-07-14 Xin Gui , Robert J. Cava

Metal-oxide-metal devices based on amorphous VOx are shown to exhibit one of two distinct negative differential resistance (NDR) characteristics depending on the maximum current employed for electroforming. For low compliance currents they…

Applied Physics · Physics 2021-02-03 Sanjoy Kumar Nandi , Sujan Kumar Das , Caleb Estherby , Angus Gentle , Robert G. Elliman

The metal-insulator transition (MIT) of V6O11 is studied by means of electronic structure calculations using the augmented spherical wave method. The calculations are based on density functional theory and the local density approximation.…

Strongly Correlated Electrons · Physics 2009-11-07 U. Schwingenschloegl , V. Eyert , U. Eckern

The metal insulator transition of nano-scaled $VO_2$ devices is drastically different from the smooth transport curves generally reported. The temperature driven transition occurs through a series of resistance jumps ranging over 2 decades…

Mesoscale and Nanoscale Physics · Physics 2008-10-31 Amos Sharoni , Juan Gabriel Ramírez , Ivan K. Schuller

We report structural, magnetization, electrical resistivity and nuclear- and electron spin resonance data of the complex transition metal oxide In_2VO_5 in which structurally well-defined V-O chains are realized. An itinerant character of…

Strongly Correlated Electrons · Physics 2009-11-13 A. Moller , T. Taetz , N. Hollmann , J. A. Mydosh , V. Kataev , M. Yehia , E. Vavilova , B. Buchner

The spin Seebeck effect (SSE) is sensitive to thermally driven magnetic excitations in magnetic insulators. Vanadium dioxide in its insulating low temperature phase is expected to lack magnetic degrees of freedom, as vanadium atoms are…

The competition between kinetic energy and Coulomb interactions in electronic systems can lead to complex many-body ground states with competing superconducting, charge density wave, and magnetic orders. Here we study the low temperature…

Light-manipulation of correlated electronic phases in solids offers the tantalizing prospect of realizing electronic devices operating at the ultrafast time-scale. In this context, the experimental realization of non-equilibrium transitions…

Strongly Correlated Electrons · Physics 2021-04-09 Francesco Grandi , Martin Eckstein

Phase transitions are key in determining and controlling the quantum properties of correlated materials. Here, by using the powerful combination of precise material synthesis and angle resolved photoelectron spectroscopy, we show evidence…

We present an ab initio quantum theory of the metal-insulator transition in Ti$_2$O$_3$. The recently developed cluster LDA+DMFT scheme is applied to describe the many-body features of this compound. The conventional single site DMFT cannot…

Strongly Correlated Electrons · Physics 2009-11-10 A. I. Poteryaev , A. I. Lichtenstein , G. Kotliar

Theoretical studies of the metamagnetism and anomalous phase of Sr3Ru2O7 have focused on the role of van Hove singularities, although much experimental evidence points towards quantum criticality having a large effect. We investigate the…

Strongly Correlated Electrons · Physics 2015-05-19 A. M. Berridge

We study the interplay of the structural phase transition, flat electronic band dispersion, and metal-to-insulator transition (MIT) in the parent compounds of the Ru-pnictide superconductors by using first-principles calculations. Our…

Materials Science · Physics 2024-01-30 Niraj Aryal , Emil S. Bozin , Weiguo Yin

The low temperature monoclinic, insulating phase of vanadium dioxide is ordinarily considered nonmagnetic, with dimerized vanadium atoms forming spin singlets, though paramagnetic response is seen at low temperatures. We find a nonlocal…

Strongly Correlated Electrons · Physics 2022-09-19 Renjie Luo , Xuanhan Zhao , Liyang Chen , Tanner J. Legvold , Henry Navarro , Ivan K. Schuller , Douglas Natelson