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The structure of spherical micelles of the diblock poly(styrene-block-acrylic acid) [PS-b-PA] copolymer in water was investigated up to concentrations where the polyelectrolyte coronal layers have to shrink and/or interpenetrate in order to…

Soft Condensed Matter · Physics 2009-11-10 A. V. Korobko , W. Jesse , A. Lapp , S. U. Egelhaaf , J. R. C. van der Maarel

We investigate by scattering techniques the structure of water-based soft composite materials comprising a crystal made of Pluronic block-copolymer micelles arranged in a face-centered cubic lattice and a small amount (at most 2% by volume)…

Soft Condensed Matter · Physics 2012-06-07 Elisa Tamborini , Neda Ghofraniha , Julian Oberdisse , Luca Cipelletti , Laurence Ramos

Triblock terpolymers exhibit a rich self-organization behavior including the formation of fascinating cylindrical core-shell structures with a phase separated corona. After crystallization-induced self-assembly of…

Soft Condensed Matter · Physics 2017-08-23 S. Rosenfeldt , F. Luedel , C. Schulreich , T. Hellweg , A. Radulescu , J. Schmelz , H. Schmalz , L. Harnau

We report on the complexation between charged-neutral block copolymers and oppositely charged surfactants studied by small-angle neutron scattering. Two block copolymers/surfactant systems are investigated, poly(acrylic…

Soft Condensed Matter · Physics 2007-05-23 Jean-Francois Berret

When polyelectrolyte-neutral block copolymers are mixed in solutions to oppositely charged species (e.g. surfactant micelles, macromolecules, proteins etc), there is the formation of stable supermicellar aggregates combining both…

Soft Condensed Matter · Physics 2007-05-23 J. -F. Berret , K. Yokota , M. Morvan

We present a self-consistent field theory (SCFT) study of spherical micelle formation in a blend of poly(styrene-butadiene) diblocks and homopolystyrene. The micelle core radii, corona thicknesses and critical micelle concentrations are…

Soft Condensed Matter · Physics 2011-06-28 M. J. Greenall , D. M. A. Buzza , T. C. B. McLeish

Polypeptide-based diblock copolymers forming either well-defined self-assembled micelles or vesicles after direct dissolution in water or in dichloromethane, have been studied combining light and neutron scattering with electron microscopy…

Complexation of a long flexible polyelectrolyte (PE) molecule with oppositely charged spherical particles such as colloids, micelles, or globular proteins in a salty water solution is studied. PE binds spheres winding around them, while…

Soft Condensed Matter · Physics 2009-10-31 Toan T. Nguyen , Boris I. Shklovskii

We report on the formation of colloidal complexes resulting from the electrostatic self-assembly of polyelectrolyte-neutral block copolymers and oppositely charged surfactants. The copolymers investigated are asymmetric and characterized by…

Soft Condensed Matter · Physics 2007-05-23 Jean-Francois Berret , Pascal Herve , Isabelle Grillo

The interaction of amphiphilic polymers with small colloids, capable to reversibly stick onto the chains, is studied. Adhesive small colloids in solution are able to dynamically bind two polymer segments. This association leads to…

Soft Condensed Matter · Physics 2010-11-10 Vladimir A. Baulin , Albert Johner , Josep Bonet Avalos

We study the effective interaction between differently charged polyelectrolyte-colloid complexes in electrolyte solutions via Monte Carlo simulations. These complexes are formed when short and flexible polyelectrolyte chains adsorb onto…

Soft Condensed Matter · Physics 2010-05-05 D. Truzzolillo , F. Bordi , F. Sciortino , S. Sennato

We report the formation of colloidal complexes resulting from the electrostatic co-assembly between anionic surfactants and cationic polyelectrolytes or block copolymers. Combining light and x-ray scattering experiments with cryogenic…

Soft Condensed Matter · Physics 2009-04-01 J. -F. Berret

We consider conformations and intra-molecular conformational transitions in amphiphilic starlike polymers formed by diblock copolymer arms with inner hydrophobic and outer polyelectrolyte blocks. A combination of an analytical mean-field…

Soft Condensed Matter · Physics 2012-05-15 Alexey A. Polotsky , Tatiana M. Birshtein , Mohamed Daoud , Oleg V. Borisov

Using a simplified microstructural picture we show that interactions between thermosenstive microgel particles can be described by a polymer brush like corona decorating the dense core. The softness of the potential is set by the relative…

Soft Condensed Matter · Physics 2010-03-29 Frank Scheffold , Pedro Diaz-Leyva , Mathias Reufer , Nasser Ben Braham , Iseult Lynch , James L. Harden

We investigated the formation of cocontinuous structures in polymer blends. These polymeric bijels (bicontinuous interfacially jammed emulsion gels) were composed of polystyrene oligomer, polybutene and fluorescent hydrophobic silica…

Soft Condensed Matter · Physics 2015-02-03 Lian Bai , John Fruehwirth , Xiang Cheng , Christopher W. Macosko

We study the ionic equilibria and interactions of neutral semi-permeable spherical shells immersed in electrolyte solutions, including polyions. Although the shells are uncharged, only one type of ions of the electrolyte can permeate them,…

Soft Condensed Matter · Physics 2012-07-24 Vladimir Lobaskin , Artem N. Bogdanov , Olga I. Vinogradova

Blockage of pores by particles is found in many processes, including filtration and oil extraction. We present filtration experiments through a linear array of ten channels with one dimension which is sub-micron, through which a dilute…

Fluid Dynamics · Physics 2018-02-26 Olivier Liot , Akash Singh , Patrice Bacchin , Paul Duru , Jeffrey F. Morris , Pierre Joseph

This study utilizes self-consistent field theory to characterize various features of cononsolvency-driven spherical micelles formed by double hydrophilic block copolymers (DHBCs). Micelles are observed only at an intermediate cosolvent…

Soft Condensed Matter · Physics 2025-04-07 Xiangyu Zhang , Jing Zong , Dong Meng

We theoretically study the reentrant condensation of a polyelectrolyte in the presence of an oppositely-charged surfactant,a phenomenon whose phase-transition mechanism remains under discussion. We focus on the adsorption and attraction…

Soft Condensed Matter · Physics 2024-11-12 Huaisong Yong

The behavior of polyelectrolytes between charged surfaces immersed in semi-dilute solutions is investigated theoretically. A continuum mean field approach is used for calculating numerically concentration profiles between two electrodes…

Soft Condensed Matter · Physics 2007-05-23 I. Borukhov , D. Andelman , H. Orland
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