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Strong coupling phenomena, such as the like charged macroions attraction, opposite charged macroions repulsion, charge renormalization or charge inversion, are known to be mediated by multivalent counterions. Most theories treat the…

Soft Condensed Matter · Physics 2016-02-03 Sandipan Dutta , Y. S. Jho

The mechanisms of electrostatic interactions between two charged dielectric spheres inside a polarizable medium have been investigated, in terms of hypothetical effective dipoles that depict how the positive and negative charge in each…

Soft Condensed Matter · Physics 2025-02-06 Yanyu Duan , Zecheng Gan , Ho-Kei Chan

A theory is presented for the onset of shear thickening in colloidal suspensions of particles, stabilized by an electrostatic repulsion. Based on an activation model a critical shear stress can be derived for the onset of shear thickening…

Soft Condensed Matter · Physics 2011-07-26 Joachim Kaldasch , Bernhard Senge , Jozua Laven

Since the early observation of nematic phases of disc-like clay colloids by Langmuir in 1938, the phase behaviour of such systems has resisted theoretical understanding. The main reason is that there is no satisfactory generalization for…

Soft Condensed Matter · Physics 2009-11-07 E. Trizac , L. Bocquet , R. Agra , J-J. Weis , M. Aubouy

We predict the nature (attractive or repulsive) and range (exponentially screened or long-range power law) of the electrostatic interactions of oppositely charged and planar plates as a function of the salt concentration and surface charge…

Soft Condensed Matter · Physics 2012-01-31 Dan Ben-Yaakov , Yoram Burak , David Andelman , S. A. Safran

Physical properties of colloidal materials can be modified by addition of nanoparticles. Within a model of like-charged mixtures of particles governed by effective electrostatic interactions, we explore the influence of charged…

Soft Condensed Matter · Physics 2018-05-22 Braden M. Weight , Alan R. Denton

We study the problem of charge regulation and its effects on electrostatic interactions between dissociable charge groups immersed in a univalent electrolyte, within a family of one dimensional exactly solvable models. We consider the case…

Soft Condensed Matter · Physics 2015-06-23 A. C. Maggs , R. Podgornik

We review briefly the concept of colloidal dispersions, their general properties and some of their most important applications, as well as the basic molecular interactions that give rise to their properties in equilibrium. Similarly, we…

Soft Condensed Matter · Physics 2015-09-28 R. Lopez-Esparza , M. A. Balderas Altamirano , E. Pérez , A. Gama Goicochea

Using computer simulations of two charged colloidal spheres with their counterions in a hard sphere solvent, we show that the granular nature of the solvent significantly influences the effective colloidal interaction. For divalent…

Chemical Physics · Physics 2016-08-15 E. Allahyarov , H. Löwen

We perform extensive molecular dynamics simulations of a highly charged flexible polyelectrolyte (PE) chain in a poor solvent for the case when the chain is in a collapsed state and the electrostatic interactions, characterized by the…

Soft Condensed Matter · Physics 2016-09-22 Anvy Moly Tom , Satyavani Vemparala , R Rajesh , Nikolai Brilliantov

The electrostatic complexation between DOTAP-DOPC unilamellar liposomes and an oppositely charged polyelectrolyte (NaPA) has been investigated in a wide range of the liposome surface charge density. We systematically characterized the…

Soft Condensed Matter · Physics 2015-03-11 Simona Sennato , Laura Carlini , Domenico Truzzolillo , Federico Bordi

A survey is presented of various aspects of the interaction of charged particles with solids. In the framework of many-body perturbation theory, we study the nonlinear interaction of charged particles with a free gas of interacting…

Materials Science · Physics 2015-06-24 J. M. Pitarke , I. G. Gurtubay , V. U. Nazarov

The solid-liquid phase-diagram of charge-stabilized colloidal suspensions is calculated using a technique that combines a continuous Poisson-Boltzmann description for the microscopic electrolyte ions with a molecular-dynamics simulation for…

Soft Condensed Matter · Physics 2009-11-07 J. Dobnikar , R. Rzehak , H. H. von Gruenberg

Recent experiments have shown that trivalent ion, spermidine$^{3+}$, can provoke lateral microphase segregation in DNA brushes. Using molecular simulations and simple theoretical arguments, we explore the effects of trivalent counterions on…

Soft Condensed Matter · Physics 2017-03-03 Lei Liu , Philip A. Pincus , Changbong Hyeon

We study electrostatic mechanisms of destabilization of highly asymmetric electrolytes. For this purpose, we perform primitive model Monte Carlo simulations of charged macroions immersed in multivalent salt solution. At low salt…

Soft Condensed Matter · Physics 2007-06-20 Vladimir Lobaskin , Khawla Qamhieh

Responsive poly-N-isopropylacrylamide-based microgels are commonly used as model colloids with soft repulsive interactions. It has been shown that the microgel-microgel interaction in solution can be easily adjusted by varying the…

Soft Condensed Matter · Physics 2021-09-06 Steffen Bochenek , Cathy E. McNamee , Michael Kappl , Hans Juergen Butt , Walter Richtering

Electric double layers (EDL) with counterions only, say electrons with the elementary charge $-e$, in thermal equilibrium at the inverse temperature $\beta$ are considered. In particular, we study the effect of the surface charge modulation…

Statistical Mechanics · Physics 2022-07-26 Ladislav Šamaj

We investigate the interaction between highly charged lipid bilayers in the presence of monovalent counterions. Neutron and X-ray reflectivity experiments show that the water layer between like-charged bilayers is thinner than for…

Constant temperature molecular dynamics simulations were used to study solutions of flexible polyelectrolyte chains at nonzero concentrations with explicit counterions and unscreened coulombic interactions. Counterion condensation, measured…

Statistical Mechanics · Physics 2009-10-31 J. C. Chu , C. H. Mak

We calculate the elastic field mediated interaction between macroscopic particles in a columnar hexagonal phase. The interaction is found to be long-ranged and non-central, with both attractive and repulsive parts. We show how the…

Soft Condensed Matter · Physics 2009-11-07 Ronojoy Adhikari