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We study the effective interaction mediated by strongly coupled Coulomb fluids between dielectric surfaces carrying quenched, random monopolar charges with equal mean and variance, both when the Coulomb fluid consists only of mobile…

Soft Condensed Matter · Physics 2020-10-01 Malihe Ghodrat , Ali Naji , Haniyeh Komaie-Moghaddam , Rudolf Podgornik

Interplay between counterion-mediated interaction and stiffness inherent to polymer chain can bring substantial complexity to the morphology and dynamics of polyelectrolyte brush condensates. Trivalent counterions induce collapse of…

Soft Condensed Matter · Physics 2018-07-24 Lei Liu , Changbong Hyeon

By a combination of Monte Carlo simulations and analytical calculations, we investigate the effective interactions between highly charged planar interfaces, neutralized by mobile counterions (salt-free system). While most previous analysis…

Soft Condensed Matter · Physics 2020-11-20 Ladislav Samaj , Martin Trulsson , Emmanuel Trizac

A simple model is presented for the appearance of attraction between two like charged polyions inside a polyelectrolyte solution. The polyions are modeled as rigid cylinders in a continuum dielectric solvent. The strong electrostatic…

Soft Condensed Matter · Physics 2009-10-31 Alexandre Diehl , Humberto A. Carmona , Yan Levin

The behavior of polyelectrolytes between charged surfaces immersed in semi-dilute solutions is investigated theoretically. A continuum mean field approach is used for calculating numerically concentration profiles between two electrodes…

Soft Condensed Matter · Physics 2007-05-23 I. Borukhov , D. Andelman , H. Orland

The electrophoretic behaviour of flexible polyelectrolyte chains ranging from single monomers up to long fragments of hundred repeat units is studied by a mesoscopic simulation approach. Abstracting from the atomistic details of the…

Soft Condensed Matter · Physics 2015-05-13 Kai Grass , Christian Holm

Using a simplified microstructural picture we show that interactions between thermosenstive microgel particles can be described by a polymer brush like corona decorating the dense core. The softness of the potential is set by the relative…

Soft Condensed Matter · Physics 2010-03-29 Frank Scheffold , Pedro Diaz-Leyva , Mathias Reufer , Nasser Ben Braham , Iseult Lynch , James L. Harden

Forces between charged silica particles in solutions of multivalent coions are measured with colloidal probe technique based on atomic force microscopy. The concentration of 1:z electrolytes is systematically varied to understand the…

Soft Condensed Matter · Physics 2019-08-08 Biljana Uzelac , Valentina Valmacco , Gregor Trefalt

Within a general framework we study the effective, deformation-induced interaction between two colloids trapped at a fluid interface. As an application, we consider the interface deformation owing to the electrostatic field of charged…

Soft Condensed Matter · Physics 2007-05-23 Alvaro Dominguez , Martin Oettel , Siegfried Dietrich

Polyelectrolyte brushes consist of a set of charged linear macromolecules each tethered at one end to a surface. An example is the glycocalyx which refers to hair-like negatively charged sugar molecules that coat the outside membrane of all…

Biological Physics · Physics 2024-07-16 William J Ceely , Marina Chugunova , Ali Nadim , James D Sterling

We study the electrophoretic mobility of spherical particles and the electrical conductivity in salt-free concentrated suspensions including finite ion size effects. An ideal salt-free suspension is composed of just charged colloidal…

Soft Condensed Matter · Physics 2017-09-13 Rafael Roa , Félix Carrique , Emilio Ruiz-Reina

We compare weak and strong coupling theory of counterion-mediated electrostatic interactions between two asymmetrically charged plates with extensive Monte-Carlo simulations. Analytical results in both weak and strong coupling limits…

Soft Condensed Matter · Physics 2009-05-26 M. Kanduc , M. Trulsson , A. Naji , Y. Burak , J. Forsman , R. Podgornik

We reformulate the theory of strong electrostatic coupling in order to describe an asymmetric electrolyte solution of monovalent salt ions and polyvalent counterions using field-theoretical techniques and Monte-Carlo simulations. The theory…

Soft Condensed Matter · Physics 2015-05-14 Matej Kanduc , Ali Naji , Jan Forsman , Rudolf Podgornik

We theoretically and experimentally investigate colloid-oil-water-interface interactions of charged, sterically stabilized, poly(methyl-methacrylate) colloidal particles dispersed in a low-polar oil (dielectric constant $\epsilon=5-10$)…

Theoretical calculations for colloidal charge-stabilized and hard sphere suspensions show that hydrodynamic interactions yield a qualitatively different particle concentration dependence of the short-time self-diffusion coefficient. The…

Soft Condensed Matter · Physics 2009-10-31 E. Overbeck , Ch. Sinn , M. Watzlawek

We study the melting behavior of charged colloidal crystals, using a simulation technique that combines a continuous mean-field Poisson-Boltzmann description for the microscopic electrolyte ions with a Brownian-dynamics simulation for the…

Soft Condensed Matter · Physics 2009-11-13 J. Dobnikar , Y. Chen , R. Rzehak , H. H. von Grünberg

In this dissertation we analyzed the double-layer force interaction between two dielectric charged colloidal spheres of different radii immersed in a solution of ions in water and in thermal equilibrium. In the limit of low electrostatic…

Soft Condensed Matter · Physics 2016-03-01 Daniel Martínez Tibaduiza

The behaviour and stability of soft and biological matter depend significantly on electrostatic interactions, as particles such as proteins and colloids acquire a charge when dispersed in an electrolytic solution. A typical simplification…

Soft Condensed Matter · Physics 2025-05-09 Andraž Gnidovec , Emanuele Locatelli , Simon Čopar , Anže Božič , Emanuela Bianchi

In the present work, we study the equilibrium conformations of linear polyelectrolytes tethered onto a spherical, oppositely charged core in equilibrium with an ionic reservoir of fixed concentration. Particular focus is placed on the…

Soft Condensed Matter · Physics 2021-12-21 Amin Bakhshandeh , Maximiliano Segala , Thiago Colla

We investigate theoretically the phase diagram of an insoluble charged surfactant monolayer in contact with a semi-dilute polyelectrolyte solution (of opposite charge). The polyelectrolytes are assumed to have long-range and attractive…

Soft Condensed Matter · Physics 2012-07-19 Adi Shafir , David Andelman
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