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We compute the electronic structure of acceptor clusters in silicon by using three methods to include electron correlations: the full configuration interaction, the Heitler-London approximation, and the unrestricted Hartree-Fock method. We…

Mesoscale and Nanoscale Physics · Physics 2021-09-15 Jianhua Zhu , Wei Wu , Andrew J. Fisher

This review presents a concise, yet comprehensive discussion on the evolution of theoretical methods employed to determine the ground and excited states of molecules in weak and strong magnetic fields. The weak-field cases have been studied…

Atomic and Molecular Clusters · Physics 2021-05-31 Mihir Date , R. W. A Havenith

We study the collective states formed by two-dimensional electrons in Landau levels of index $n\ge 2$ near half-filling. By numerically solving the self-consistent Hartree-Fock (HF) equations for a set of oblique two-dimensional lattices,…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 A. M. Ettouhami , C. B. Doiron , F. D. Klironomos , R. Côté , Alan T. Dorsey

We explore the existence and behaviour of holomorphic restricted Hartree-Fock (h-RHF) solutions for two-electron problems. Through algebraic geometry, the exact number of solutions with $n$ basis functions is rigorously identified as…

Chemical Physics · Physics 2018-01-15 Hugh G. A. Burton , Mark Gross , Alex J. W. Thom

The few-body problem for $N=4$ fermionic charge carriers in a double-well moir\'{e} quantum dot (MQD), representing the first step in a bottom-up strategy to investigate formation of molecular supercrystals in transition metal…

Strongly Correlated Electrons · Physics 2024-03-20 Constantine Yannouleas , Uzi Landman

Exact-diagonalization calculations for N=3 electrons in anisotropic quantum dots, covering a broad range of confinement anisotropies and strength of inter-electron repulsion, are presented for zero and low magnetic fields. The excitation…

Mesoscale and Nanoscale Physics · Physics 2008-01-03 Yuesong Li , Constantine Yannouleas , Uzi Landman

Strong repelling interactions between a few fermions or bosons confined in two-dimensional circular traps lead to particle localization and formation of quantum Wigner molecules (QWMs) possessing definite point-group space symmetries. These…

Mesoscale and Nanoscale Physics · Physics 2016-04-18 Constantine Yannouleas , Uzi Landman

We present a group theoretical study of the symmetry-broken unrestricted Hartree-Fock orbitals and electron densities in the case of a two-dimensional N-electron single quantum dot (with and without an external magnetic field). The breaking…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Constantine Yannouleas , Uzi Landman

We have obtained the exact ground state wave functions of the Anderson-Hubbard model for different electron fillings on a 4x4 lattice with periodic boundary conditions - for 1/2 filling such ground states have roughly 166 million states.…

Strongly Correlated Electrons · Physics 2007-11-17 X. Chen , P. W. Leung , R. J. Gooding

Fully numerical mesh solutions of 2D quantum equations of Schroedinger and Hartree-Fock type allow us to work with wavefunctions which possess a very flexible geometry. This flexibility is especially important for calculations of atoms and…

Atomic Physics · Physics 2015-06-26 Mikhail V. Ivanov , Peter Schmelcher

We study the behavior of Hartree-Fock (HF) solutions in the vicinity of conical intersections. These are here understood as regions of a molecular potential energy surface characterized by degenerate or nearly-degenerate eigenfunctions with…

Chemical Physics · Physics 2018-04-10 Lena C. Jake , Thomas M. Henderson , Gustavo E. Scuseria

A method for constructing semianalytical strongly correlated wave functions for single and molecular quantum dots is presented. It employs a two-step approach of symmetry breaking at the Hartree-Fock level and of subsequent restoration of…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Constantine Yannouleas , Uzi Landman

Energy spectra and spin configurations of a system of N=4 electrons in lateral double quantum dots (quantum dot Helium molecules) are investigated using exact diagonalization (EXD), as a function of interdot separation, applied magnetic…

Mesoscale and Nanoscale Physics · Physics 2009-08-03 Ying Li , Constantine Yannouleas , Uzi Landman

We present unrestricted Hartree Fock method coupled with configuration interaction (CI) method (URHF-CI) suitable for the calculation of ground and excited states of large number of electrons localized by complex gate potentials in…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Ramin M. Abolfath , Pawel Hawrylak

The transport properties of quantum dots with up to N=7 electrons ranging from the weak to the strong interacting regime are investigated via the projected Hartree-Fock technique. As interactions increase radial order develops in the dot,…

Mesoscale and Nanoscale Physics · Physics 2011-10-10 F. Cavaliere , U. De Giovannini , M. Sassetti , B. Kramer

We calculate the ground state phase diagram of the homogeneous electron gas in three dimensions within the Hartree-Fock approximation and show that broken symmetry states are energetically favored at any density against the homogeneous…

Strongly Correlated Electrons · Physics 2014-03-04 Lucas Baguet , François Delyon , Bernard Bernu , Markus Holzmann

The multiconfiguration time-dependent Hartree-Fock (MCTDHF) method is formulated for treating the coupled electronic and nuclear dynamics of diatomic molecules without the Born- Oppenheimer approximation. The method treats the full…

Computational Physics · Physics 2015-05-27 Daniel J. Haxton , Keith V. Lawler , C. William McCurdy

Energy spectra, spin configurations, and entanglement characteristics of a system of four electrons in lateral double quantum dots are investigated using exact diagonalization (EXD), as a function of interdot separation, applied magnetic…

Mesoscale and Nanoscale Physics · Physics 2009-02-12 Ying Li , Constantine Yannouleas , Uzi Landman

The energy levels of the first few low-lying states of helium and lithium atoms in intense magnetic fields up to $\approx 10^8-10^9$~T are calculated in this study. A pseudospectral method is employed for the computational procedure. The…

Quantum Physics · Physics 2014-06-11 Anand Thirumalai , Jeremy S. Heyl

A simple and commonly employed approximate technique with which one can examine spatially disordered systems when strong electronic correlations are present is based on the use of real-space unrestricted self-consistent Hartree-Fock wave…

Strongly Correlated Electrons · Physics 2009-11-13 X. Chen , A. Farhoodfar , T. McIntosh , R. J. Gooding , P. W. Leung