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We present a model of equal spin $s_1$ dimer single molecule magnets. The spins within each dimer interact via the Heisenberg and the most general set of four quadratic anisotropic spin interactions with respective strengths $J$ and…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Dmitri V. Efremov , Richard A. Klemm

Exact analytical diagonalization is used to study the bipartite entanglement of the antiferromagnetic mixed spin-(1/2,$S$) Heisenberg dimer (MSHD) with the help of negativity. Under the assumption of uniaxial single-ion anisotropy affecting…

Quantum Physics · Physics 2021-12-08 Hana Vargová , Jozef Strečka , Natália Tomašovičová

The concept of negativity is adapted in order to explore the quantum and thermal entanglement of the mixed spin-(1/2,$S$) Heisenberg dimers in presence of an external magnetic field. The mutual interplay between the spin size $S$, XXZ…

Statistical Mechanics · Physics 2021-08-17 Hana Vargová , Jozef Strečka

We calculate the static and dynamic properties of single crystal, single molecule magnets consisting of equal spin $S=1/2$ or 5/2 dimers. The spins in each dimer interact with each other via the Heisenberg exchange interaction and with the…

Statistical Mechanics · Physics 2009-11-07 Dmitri V. Efremov , Richard A. Klemm

We study single-ion and exchange anisotropy effects in equal-spin $s_1$ tetramer single molecule magnets exhibiting $T_d$, $D_{4h}$, $D_{2d}$, $C_{4h}$, $C_{4v}$, or $S_4$ ionic point group symmetry. We first write the group-invariant…

Strongly Correlated Electrons · Physics 2009-11-13 Richard A. Klemm , Dmitri V. Efremov

For equal-spin $s_1$ tetramer single molecule magnets with ionic point groups $g=T_d, D_{4h}, D_{2d}, C_{4h}, C_{4v}$, and $S_4$, we write the group-invariant single-ion, Dzaloshinskii-Moriya, and symmetric anisotropic near-neighbor and…

Mesoscale and Nanoscale Physics · Physics 2008-05-13 Richard A. Klemm , Dmitri V. Efremov

We present a microscopic theory of single molecule magnets. From our exact single-ion spin matrix elements for four arbitrary spins, we study the single-ion anisotropy of equal spins exhibiting $T_d$, $D_{2d}$, or $C_{4v}$ molecular group…

Mesoscale and Nanoscale Physics · Physics 2013-05-29 Richard A. Klemm , Dmitri V. Efremov

The effect of dipolar interaction and local uniaxial anisotropy on the magnetic response of small spin clusters where spins are located on the vertices of icosahedron, cuboctahedron, tetrahedron and square geometry have been investigated.…

Atomic and Molecular Clusters · Physics 2012-01-11 Alfred Hucht , Sanjubala Sahoo , Shreekantha Sil , Peter Entel

The influence of uniaxial single-ion anisotropy -DSz^2 on the magnetic and thermal properties of Heisenberg antiferromagnets (AFMs) is investigated. The uniaxial anisotropy is treated exactly and the Heisenberg interactions are treated…

Strongly Correlated Electrons · Physics 2017-05-15 David C. Johnston

Detailed magnetization, specific heat, and $^7$Li nuclear magnetic resonance (NMR) measurements on single crystals of the hyperhoneycomb Kitaev magnet $\beta$-Li$_2$IrO$_3$ are reported. At high temperatures, {\cred anisotropy of the…

Strongly Correlated Electrons · Physics 2019-07-30 M. Majumder , F. Freund , T. Dey , M. Prinz-Zwick , N. Büttgen , Y. Skourski , A. Jesche , A. A. Tsirlin , P. Gegenwart

We use Green's function method to study the Heisenberg model of LaFeAsO with the striped antiferromagnetic collinear spin structure. In addition to the intra-layer spin couplings $J_{1a},J_{1b},J_2$ and the inter-layer coupling $J_c$, we…

Superconductivity · Physics 2010-01-05 Ren Gui Zhu

We present a finite-temperature theory of the anisotropic spin-spin correlations in magnetic metallic monolayers, deposited on a suitable substrate. The `spins' are the local moments set up by the itinerant electrons, and the key concept is…

Mesoscale and Nanoscale Physics · Physics 2013-05-29 M. dos Santos Dias , J. B. Staunton , A. Deak , L. Szunyogh

Single molecule magnets (SMMs) with single-ion anisotropies $\mathbf d$, comparable to exchange interactions J, between spins have recently been synthesized. In this paper, we provide theoretical insights into the magnetism of such systems.…

Strongly Correlated Electrons · Physics 2017-11-22 Sumit Haldar , Rajamani Raghunathan , Jean-Pascal Sutter , S. Ramasesha

The effect of uniaxial single-ion anisotropy on quantum entanglement is rigorously quantified using negativity in a mixed spin-($1$,$1/2$,$1$) Heisenberg trimer, accounting for different exchange coupling constants between identical and…

Quantum Physics · Physics 2025-09-03 Hana Vargová , Jozef Strečka

We discuss low-temperature properties of magnets with integer spin and large single-ion easy-plane anisotropy $D$ in transverse magnetic field $h$. Considering the exchange interaction between spins as a perturbation and using the diagram…

Strongly Correlated Electrons · Physics 2011-12-30 A. V. Sizanov , A. V. Syromyatnikov

We present an experimental study of macroscopic and microscopic magnetic anisotropy of a spin tetramer system \cso using torque magnetometry and ESR spectroscopy. Large rotation of macroscopic magnetic axes with temperature observed from…

Strongly Correlated Electrons · Physics 2016-08-08 Mirta Herak , Dijana Žilić , Dubravka Matković Čalogović , Helmuth Berger

Magnetic behavior of a spin-1 Heisenberg dimer is analysed in dependence on both uniaxial single-ion anisotropy and XXZ exchange anisotropy in a zero- as well as non-zero longitudinal magnetic field. A complete set of eigenfunctions and…

Materials Science · Physics 2007-05-23 J. Strecka , M. Jascur , M. Hagiwara , Y. Narumi , J. Kuchar , S. Kimura , K. Kindo

Magnetism of the $S$ = 1 Heisenberg antiferromagnets on the spatially anisotropic square lattice has been scarcely explored. Here we report a study of the magnetism, specific heat, and thermal conductivity on Ni[SC(NH$_2$)$_2$]$_6$Br$_2$…

Materials Science · Physics 2019-03-15 X. Zhao , Z. Y. Zhao , L. M. Chen , X. Rao , H. L. Che , L. G. Chu , H. D. Zhou , L. S. Ling , J. F. Wang , X. F. Sun

In this work, we present the first magnetization measurements of DyCo$_5$ single crystals in magnetic fields up to 14 T, spanning a temperature range up to 600 K. Our investigation reveals several unique features, including a significant…

Both quantum and classical behavior of single atomic spins on surfaces is determined by the local anisotropy of adatoms and their coupling to the immediate electronic environment. Yet adatoms seldom reside on surfaces alone and it is…

Materials Science · Physics 2015-11-04 P. Ruiz-Díaz , O. V. Stepanyuk , V. S. Stepanyuk
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