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Halide perovskites have emerged as one of the most interesting materials for optoelectronic applications due to their favorable properties, such as defect-tolerance and long charge carrier lifetimes, which are attributed to their dynamic…

Materials Science · Physics 2023-11-20 Julia Wiktor , Erik Fransson , Dominik Kubicki , Paul Erhart

Investigation of elementary excitations has advanced our understanding of many-body physics governing most physical properties of matter. Recently spin-orbit excitons have drawn much attention, whose condensates near phase transitions…

Strongly Correlated Electrons · Physics 2019-07-24 A. Nag , S. Bhowal , M. Moretti Sala , A. Efimenko , I. Dasgupta , S. Ray

The effective Hamiltonian for perovskite titanates is derived by taking into account the three-fold degeneracy of $t_{2g}$ orbitals and the strong electron-electron interactions. The magnetic and orbital ordered phases are studied in the…

Strongly Correlated Electrons · Physics 2009-11-07 S. Ishihara , T. Hatakeyama , S. Maekawa

Through a combination of neutron diffraction and Landau theory we describe the spin ordering in the ground state of the quadruple perovskite manganite CaMn7O12 - a magnetic multiferroic supporting an incommensurate orbital density wave that…

Strongly Correlated Electrons · Physics 2016-05-25 R. D. Johnson , D. D. Khalyavin , P. Manuel , A. Bombardi , C. Martin , L. C. Chapon , P. G. Radaelli

The concept of spin-orbital entanglement on superexchange bonds in transition metal oxides is introduced and explained on several examples. It is shown that spin-orbital entanglement in superexchange models destabilizes the long-range (spin…

Strongly Correlated Electrons · Physics 2012-07-13 Andrzej M. Oleś

We describe a variational theory of multi-band two-dimensional electron gases that captures the interplay between electrostatic confining potentials, orbital-dependent interlayer electronic hopping and electron-electron interactions, and…

Strongly Correlated Electrons · Physics 2017-05-10 John R. Tolsma , Marco Polini , Allan H. MacDonald

The lead halide perovskites demonstrate huge potential for optoelectronic applications, high energy radiation detectors, light emitting devices and solar energy harvesting. Those materials exhibit strong spin-orbit coupling enabling…

We present elastic and quasielastic neutron scattering measurements characterizing peculiar short-range charge-orbital and spin order in the layered perovskite material La1.5Sr0.5CoO4. We find that below Tc~750 K holes introduced by Sr…

Strongly Correlated Electrons · Physics 2009-10-31 I. A. Zaliznyak , J. P. Hill , J. M. Tranquada , R. Erwin , Y. Moritomo

We report a site-separated $^{17}$O-NMR study of the layered perovskite ruthenate Sr$_3$Ru$_2$O$_7$, which exhibits nearly two-dimensional transport properties and itinerant metamagnetism at low temperatures. The local hole occupancies and…

Strongly Correlated Electrons · Physics 2007-05-23 K. Kitagawa , K. Ishida , R. S. Perry , H. Murakawa , K. Yoshimura , Y. Maeno

The crystallographic and magnetic phase diagram of the n=2 layered manganite La2-2xSr1+2xMn2O7 in the region x=>0.5 has been studied using temperature dependent neutron powder diffraction. The magnetic phase diagram reveals a progression of…

Materials Science · Physics 2009-10-31 C. D. Ling , J. E. Millburn , J. F. Mitchell , D. N. Argyriou J. Linton , H. N. Bordallo

We argue that in lightly hole doped perovskite-type Mn oxides the holes (Mn$^{4+}$ sites) are surrounded by nearest neighbor Mn$^{3+}$ sites in which the occupied $3d$ orbitals have their lobes directed towards the central hole (Mn$^{4+}$)…

Strongly Correlated Electrons · Physics 2009-10-31 T. Mizokawa , D. I. Khomskii , G. A. Sawatzky

The coherent spin dynamics of electrons and holes are studied in a FA0.9Cs0.1PbI2.8Br0.2 perovskite bulk crystal, using time-resolved Kerr ellipticity in a two-color pump-probe scheme. The probe photon energy is tuned to the exciton…

We have theoretically studied successive transitions in vanadium spinel oxides with (t_2g)^2 electron configuration. These compounds show a structural transition at ~ 50K and an antiferromagnetic transition at ~ 40K. Since threefold t_2g…

Strongly Correlated Electrons · Physics 2009-11-11 Yukitoshi Motome , Hirokazu Tsunetsugu

We study magnetic excitations in vanadium spinel oxides AV$_2$O$_4$ (A=Zn, Mg, Cd) using two models: first one is a superexchange model for vanadium S=1 spins, second one includes in addition spin-orbit coupling, and crystal anisotropy. We…

Strongly Correlated Electrons · Physics 2014-09-03 N. B. Perkins , O. Sikora

A model of localized classical electrons coupled to lattice degrees of freedom and, via the Coulomb interaction, to each other, has been studied to gain insight into the charge and orbital ordering observed in lightly doped manganese…

Strongly Correlated Electrons · Physics 2009-10-31 K. H. Ahn , A. J. Millis

We present our theoretical and numerical results on thermodynamic properties and the microscopic mechanism of two successive transitions in vanadium spinel oxides $A$V$_2$O$_4$ ($A$=Zn, Mg, or Cd) obtained by Monte Carlo calculations of an…

Strongly Correlated Electrons · Physics 2007-05-23 Yukitoshi Motome , Hirokazu Tsunetsugu

Vortons are of interest in high-energy physics as possible dark matter candidates and as probes of Grand Unified Theories. Using the recently derived weak-field metric for a chiral vorton, we study the dynamics of test particles by…

General Relativity and Quantum Cosmology · Physics 2025-12-12 S. M. Holme , H. S. Ramadhan , I. Nurul Huda , Leonardus B. Putra

Motivated by recent experiments on vanadium spinels, $A$V$_2$O$_4$, that show an increasing degree of electronic delocalization for smaller cation sizes, we study the evolution of orbital ordering (OO) between the strong and…

Strongly Correlated Electrons · Physics 2012-08-13 Yasuyuki Kato , Gia-Wei Chern , K. A. Al-Hassanieh , Natalia B. Perkins , C. D. Batista

Recently, the effects of spin-orbit coupling (SOC) in correlated materials have become one of the most actively studied subjects in condensed matter physics, as correlations and SOC together can lead to the discovery of new phases. Among…

Strongly Correlated Electrons · Physics 2016-03-17 Jeffrey G. Rau , Eric Kin-Ho Lee , Hae-Young Kee

We have investigated the orbital states of the orbital-glassy (short-range orbital ordered) spinel vanadate Co$_{1.21}$V$_{1.79}$O$_{4}$ using x-ray absorption spectroscopy (XAS), x-ray magnetic circular dichroism (XMCD), and subsequent…