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Transport and non-equilibrium magnetization in monolayers of magnetic molecules subject to a bias voltage are considered. We apply a master-equation approach going beyond the sequential-tunneling approximation to study the Coulomb-blockade…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Florian Elste , Carsten Timm

Photoemission and tunneling spectroscopies measure the energies at which single electrons can be added to or removed from an electronic system. Features observed in such spectra have revealed electrons coupling to vibrational modes of ions…

Strongly Correlated Electrons · Physics 2017-05-09 Joonho Jang , Benjamin Hunt , Loren N. Pfeiffer , Kenneth W. West , Raymond C. Ashoori

We study electron transport through a small metallic island in the perturbative regime. Using a recently developed diagrammatic technique, we calculate the occupation of the island as well as the conductance through the transistor in forth…

Mesoscale and Nanoscale Physics · Physics 2009-10-30 Jürgen König , Herbert Schoeller , Gerd Schön

We study electron transport through a small metallic island in the perturbative regime. Using a diagrammatic real-time technique, we calculate the occupation of the island as well as the conductance through the transistor at arbitrary…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Jürgen König , Herbert Schoeller , Gerd Schön

The tunneling spectra of small metallic grains shows an unusual structure of the differential conductance peaks. Namely, resonance peaks appear in clusters, or develop substructure as the the gate voltage is changed. These features are…

Condensed Matter · Physics 2007-05-23 Oded Agam

We discuss the electronic transport through molecules in the Kondo regime. We concentrate here on the influence of molecular vibrations. Two types of vibrations are investigated: (i) the breathing internal molecular modes, where the…

Mesoscale and Nanoscale Physics · Physics 2009-12-21 J. Mravlje , A. Ramsak

We investigate the interplay of quantum interference effects and electronic-vibrational coupling in electron transport through single-molecule junctions, employing a nonequilibrium Green's function approach. Our findings show that inelastic…

Mesoscale and Nanoscale Physics · Physics 2013-02-18 R. Härtle , M. Butzin , M. Thoss

We measure electron tunneling via discrete energy levels in ferromagnetic cobalt particles less than 4 nm in diameter, using non-magnetic electrodes. Due to magnetic anisotropy, the energy of each tunneling resonance shifts as an applied…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 S. Gueron , Mandar M. Deshmukh , E. B. Myers , D. C. Ralph

Detection of a single nuclear spin constitutes an outstanding problem in different fields of physics such as quantum computing or magnetic imaging. Here we show that the energy levels of a single nuclear spin can be measured by means of…

Mesoscale and Nanoscale Physics · Physics 2011-12-16 F. Delgado , J. Fernández-Rossier

We report transport measurements on a semiconductor quantum dot with a small number of confined electrons. In the Coulomb blockade regime, conduction is dominated by cotunneling processes. These can be either elastic or inelastic, depending…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 S. De Franceschi , S. Sasaki , J. M. Elzerman , W. G. van der Wiel , S. Tarucha , L. P. Kouwenhoven

Experiments studying vibrational effects on electronic transport through single molecules have observed several seemingly inconsistent behaviors, ranging from up to 30 harmonics of a vibrational frequency in one experiment, to an absence of…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Vivek Aji , J. E. Moore , C. M. Varma

We investigate electron transport through a mixed-valence molecular complex in which an excess electron can tunnel between hetero-valent transition metal ions, each having a fixed localized spin. We show that in this class of molecules the…

Mesoscale and Nanoscale Physics · Physics 2009-03-11 F. Reckermann , M. Leijnse , M. R. Wegewijs

It is demonstrated that non-equilibrium vibrational effects are enhanced in molecular devices for which the effective potential for vibrations is sensitive to the charge state of the device. We calculate the electron tunneling current…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Maarten R. Wegewijs , Katja C. Nowack

We carry out experiments on single-molecule junctions at low temperatures, using the mechanically controlled break junction technique. Analyzing the results received with more than ten different molecules the nature of the first peak in the…

Mesoscale and Nanoscale Physics · Physics 2012-03-21 Daniel Secker , Stefan Wagner , Stefan Ballmann , Rainer Härtle , Michael Thoss , Heiko B. Weber

The inelastic portion of the tunnel current through an individual magnetic atom grants unique access to read out and change the atom's spin state, but it also provides a path for spontaneous relaxation and decoherence. Controlled closure of…

Mesoscale and Nanoscale Physics · Physics 2016-01-05 B. Bryant , R. Toskovic , A. Ferrón , J. L. Lado , A. Spinelli , J. Fernández-Rossier , A. F. Otte

We report inelastic electron tunneling spectroscopy (IETS) of multilayer molecular junctions with and without incorporated metal nano-particles. The incorporation of metal nanoparticles into our devices leads to enhanced IET intensity and a…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Lam H. Yu , Christopher D. Zangmeister , James G. Kushmerick

We report finite-bias characteristics of electrical transport through phosphorus donors in silicon nanoscale transistors, in which we observe inelastic-cotunneling current in the Coulomb blockade region. The cotunneling current appears like…

Mesoscale and Nanoscale Physics · Physics 2023-01-25 Pooja Yadav , Soumya Chakraborty , Daniel Moraru , Arup Samanta

Molecular electronics offers unique scientific and technological possibilities, resulting from both the nanometre scale of the devices and their reproducible chemical complexity. Two fundamental yet different effects, with no classical…

Mesoscale and Nanoscale Physics · Physics 2017-05-12 Andrew K. Mitchell , Kim G. L. Pedersen , Per Hedegaard , Jens Paaske

We present explicit kinetic equations for quantum transport through a general molecular quantum-dot, accounting for all contributions up to 4th order perturbation theory in the tunneling Hamiltonian and the complete molecular density…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 M. Leijnse , M. R. Wegewijs

Tunneling is measured via the quantum levels of a metal nanoparticle. We analyze quantitatively the resonance energies, widths, and amplitudes, both in the regime where only one state is accessible for tunneling and in the non-equilibrium…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Mandar M. Deshmukh , Edgar Bonet , A. N. Pasupathy , D. C. Ralph