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We present an experimental study of the {\em nonlinear} susceptibility of Mn$_{12}$ single-molecule magnets. We investigate both their thermal-equilibrium and dynamical nonlinear responses. The equilibrium results show the sensitivity of…

Mesoscale and Nanoscale Physics · Physics 2016-08-16 R. López-Ruiz , F. Luis , V. González , A. Millán , J. L. García-Palacios

Quantum nanomagnets can show a field dependence of the relaxation time very different from their classical counterparts, due to resonant tunneling via excited states (near the anisotropy barrier top). The relaxation time then shows minima…

Mesoscale and Nanoscale Physics · Physics 2013-05-29 R. Lopez-Ruiz , F. Luis , A. Millan , C. Rillo , D. Zueco , J. L. Garcia-Palacios

The weak field average magnetic susceptibility of square shaped mesoscopic conductors is studied within a semiclassical framework. Long semiclassical trajectories are strongly affected by static disorder and differ sharply from those of…

Condensed Matter · Physics 2009-10-22 Yuval Gefen , Daniel Braun , Gilles Montambaux

A new type of mesoscopic quantum effect in large-spin molecules possessing easy-axis anisotropy, such as Mn12, is predicted. The response of such a system to an external field applied perpendicular to the easy axis is considered. It is…

Statistical Mechanics · Physics 2009-10-31 A. K. Zvezdin , V. V. Dobrovitski , B. N. Harmon , M. I. Katsnelson

A single-molecule magnet placed in a magnetic field perpendicular to its anisotropy axis can be truncated to an effective two-level system, with easily tunable energy splitting. The quantum coherence of the molecular spin is largely…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 A. Morello , A. Millán , L. J. de Jongh

This thesis contains a thorough investigation of the quantum spin dynamics in Mn12-ac and Mn6 Single-molecule magnets. In particular, we have investigated the interplay between quantum tunneling of magnetization and nuclear spin dynamics in…

Mesoscale and Nanoscale Physics · Physics 2009-09-29 Andrea Morello

Common models describing magnetotransport properties of periodically modulated two--dimensional systems often either directly start from a semiclassical approach or give results well conceivable within the semiclassical framework. Recently,…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Karel Vyborny , Ludvik Smrcka

The dependence of the magnetic susceptibility on the magnetic field is investigated for the single molecular magnet [Mn(hfac)$_2$NITPh]$_6$. The spikes of the susceptibility detected in a magnetic field ranging from 90 T to 285 T are…

The magnetization reversal in a single molecular magnet (SMM) weakly coupled to an electrode with spin-dependent splitting of chemical potentials (spin bias) is theoretically investigated by means of the rate equation. A microscopic…

Mesoscale and Nanoscale Physics · Physics 2009-05-14 Hai-Zhou Lu , Bin Zhou , Shun-Qing Shen

The linear response theory is used to describe magnetoresistance oscillations of short-period unilateral superlattices with strong modulation (or alternatively arrays of coupled quantum wires). The semiclassical description of this system…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Karel Vyborny , Ludvik Smrcka , Rainer A. Deutschmann

The spin relaxation in the molecular magnet \Mn12 is investigated by a novel type of high-frequency magnetic spectroscopy. By reversing the external magnetic field the intensities of the $|\pm 10>\to |\pm 9>$ transitions within the ground…

Strongly Correlated Electrons · Physics 2016-08-31 M. Dressel , B. Gorshunov , K. Rajagopal , S. Vongtragool , A. A. Mukhin

We use neutron diffraction to probe the magnetization components of a crystal of Mn12 single-molecule magnets. Each of these molecules behaves, at low temperatures, as a nanomagnet with spin S = 10 and strong anisotropy along the…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 F. Luis , J. Campo , J. Gomez , G. J. McIntyre , J. Luzon , D. Ruiz-Molina

Dynamic nonlinear (cubic) susceptibility in quantum d-dimensional Ising spin glass with short-range interactions is investigated on the basis of quantum droplet model and quantum-mechanical nonlinear response theory. Nonlinear response…

Disordered Systems and Neural Networks · Physics 2009-11-07 G. Busiello , R. V. Saburova , V. G. Sushkova

The magnetic behavior of molecular Single-Chain Magnets is investigated in the framework of a one-dimensional Ising model with single spin-flip Glauber dynamics. Opportune modifications to the original theory are required in order to…

Materials Science · Physics 2011-04-21 Alessandro Vindigni , Maria Gloria Pini

We present a model to probe metamagnetic properties in systems with an arbitrary number of interacting spins. Thermodynamic properties such as the magnetization per particle $m(B,T,N)$, linear susceptibility $\chi_1(T)$, nonlinear…

Statistical Mechanics · Physics 2018-08-15 Pradeep Kumar , Christopher E. Wagner

The equilibrium susceptibility of uniaxial paramagnets is studied in a unified framework which permits to connect traditional results of the theory of quantum paramagnets, $\Sm=1/2, 1, 3/2$, ..., with molecular magnetic clusters, $\Sm\sim5,…

Statistical Mechanics · Physics 2015-05-13 J. L. Garcia-Palacios , J. B. Gong , F. Luis

Magnetic damping is a key metric for emerging technologies based on magnetic nanoparticles, such as spin torque memory and high-resolution biomagnetic imaging. Despite its importance, understanding of magnetic dissipation in nanoscale…

Mesoscale and Nanoscale Physics · Physics 2019-10-29 I. Barsukov , H. K. Lee , A. A. Jara , Y. -J. Chen , A. M. Gonçalves , C. Sha , J. A. Katine , R. E. Arias , B. A. Ivanov , I. N. Krivorotov

The linear and cubic dynamic susceptibilities of solid dispersions of nano-sized maghemite particles have been measured for three samples with a volume concentration of magnetic particles ranging from 0.3 % to 17 %, in order to study the…

Materials Science · Physics 2016-08-15 P. Jönsson , T. Jonsson , J. L. García-Palacios , P. Svedlindh

We study the magnetic susceptibility of an ensemble of non-interacting electrons confined by parabolic potentials and subjected to a perpendicular magnetic field at finite temperatures. We show that the behavior of the average…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 M. O. Terra , M. L. Tiago , M. A. M. de Aguiar

We study the evolution of low-temperature magnetoresistance in double quantum wells in the region below 1 Tesla as the applied current density increases. A flip of the magneto-intersubband oscillation peaks, which occurs as a result of the…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 N. C. Mamani , G. M. Gusev , O. E. Raichev , T. E. Lamas , A. K. Bakarov
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