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First principles linear combinations of Gaussian type orbitals-fitting function (LCGTO-FF) electronic structure calculations are used to study thickness dependencies in the surface energies and work functions of ultra-thin (111) films of…

Strongly Correlated Electrons · Physics 2009-11-10 A. K. Ray , J. C. Boettger

The electronic properties of bulk fcc americium and the (111) surface have been investigated with the full-potential linearized augmented plane wave (FP-LAPW) method as implemented in the WIEN2K suite of programs. The study is carried out…

Superconductivity · Physics 2007-05-23 Da Gao , Asok K. Ray

The zero-presssure zero-temperature equilibrium volume and bulk modulus are calculated for fcc Th and Pu by two independent all-electron, full-potential, electronic-structure methods: the full-potential linear augmented-plane-wave (FLAPW)…

Materials Science · Physics 2007-05-23 J. C. Boettger , M. D. Jones , R. C. Albers , D. J. Singh

Electron momentum density and Compton profiles in Lithium along $<100 >$, $<110>$, and $<111>$ directions are calculated using Full-Potential Linear Augmented Plane Wave basis within generalized gradient approximation. The profiles have…

Materials Science · Physics 2009-10-31 Tunna Baruah , Rajendra R. Zope , Anjali Kshirsagar

Adsorption of carbon, nitrogen, and oxygen on the (111) surface of delta-Plutonium has been studied within the framework of density functional theory using the full-potential linear augmented plane wave plus local basis (FP-LAPW+lo) method.…

Strongly Correlated Electrons · Physics 2007-10-29 Raymond Atta-Fynn , Asok K. Ray

We provide a straightforward and numerically efficient procedure to perform local density approximation + Hubbard I (LDA+HIA) calculations, including self-consistency over the charge density, within the full potential linearized augmented…

Materials Science · Physics 2009-09-03 Alexander B. Shick , Jindrich Kolorenč , Alexander I. Lichtenstein , Ladislav Havela

We have carried out a comparative study of the electronic specific heat and electronic structure of $\alpha$ and $\delta$-plutonium using dynmical mean field theory (DMFT). We use the perturbative T-matrix and fluctuating exchange (T-matrix…

Strongly Correlated Electrons · Physics 2009-11-13 L. V. Pourovskii , G. Kotliar , M. I. Katsnelson , A. I. Lichtenstein

By combining the local density approximation (LDA) with dynamical mean field theory (DMFT), we report a systematic analysis of the spectral properties of $\delta$-plutonium with varying $5f$ occupancy. The LDA Hamiltonian is extracted from…

Strongly Correlated Electrons · Physics 2009-11-13 Jian-Xin Zhu , A. K. McMahan , M. D. Jones , T. Durakiewicz , J. J. Joyce , J. M. Wills , R. C. Albers

Plutonium is a critically important material as the behavior of its 5f-electrons stands midway between the metallic-like itinerant character of the light actinides and localized atomic-core-like character of the heavy actinides. The…

Strongly Correlated Electrons · Physics 2020-07-01 Roxanne Tutchton , Wei-ting Chiu , R. C. Albers , G. Kotliar , Jian-Xin Zhu

We present results for the electronic structure of plutonium by using a recently developed quasiparticle self-consistent $GW$ method (\qsgw). We consider a paramagnetic solution without spin-orbit interaction as a function of volume for the…

Strongly Correlated Electrons · Physics 2009-07-23 A. N. Chantis , R. C. Albers , A. Svane , N. E. Christensen

Electronic and magnetic structure of $(100)$ films of K and Cs are calculated within the plane-wave projector augmented wave (PAW) formalism of the density functional theory (DFT) using both local spin density approximation (LSDA) and the…

Materials Science · Physics 2007-11-30 Prasenjit Sen

Understanding the atomic-scale structure and dynamics of amorphous oxide surfaces is essential for interpreting their chemical reactivity, mechanical stability, and interfacial behavior, yet direct experimental characterization remains…

Materials Science · Physics 2026-05-08 Zheng Yu , Jiayan Xu , Abhirup Patra , Sharan Shetty , Detlef Hohl , Roberto Car

Electronic and magnetic properties of the fcc Americium (001) surface have been investigated via full-potential all-electron density-functional electronic structure calculations at both scalar and fully relativistic levels. Effects of…

Strongly Correlated Electrons · Physics 2009-11-11 Da Gao , Asok K. Ray

We report the bulk and surface properties of lithium computed within a full potential LCGTO formalism using both density functional theory and the Hartree-Fock approximation. We examine the convergence of computed properties with respect to…

Materials Science · Physics 2009-10-31 K. Doll , N. M. Harrison , V. R. Saunders

The electronic and geometrical properties of bulk americium and square and hexagonal americium monolayers have been studied with the full-potential linearized augmented plane wave (FP-LAPW) method. The effects of several common…

Strongly Correlated Electrons · Physics 2009-11-11 Da Gao , Asok K. Ray

Plutonium (Pu), in which the 5$f$ valence electrons always wander the boundary between localized and itinerant states, exhibits quite complex crystal structures and unprecedentedly anomalous properties with respect to temperature and…

Strongly Correlated Electrons · Physics 2020-03-26 Li Huang , Haiyan Lu

Structural, electronic and magnetic properties were calculated for the optimized $\alpha$-U/W(110) thin films (TFs) within the density functional theory. Our optimization for 1U/7W(110) shows that the U-W vertical interlayer spacing (ILS)…

Mesoscale and Nanoscale Physics · Physics 2012-01-12 M. Zarshenas , S. Jalali Asadabadi

The $GW$ approach of many-body perturbation theory (MBPT) has become a common tool for calculating the electronic structure of materials. However, with increasing number of published results, discrepancies between the values obtained by…

Materials Science · Physics 2016-08-03 Dmitrii Nabok , Andris Gulans , Claudia Draxl

We develop a new implementation of the Gutzwiller approximation (GA) and interface it with the local density approximation (LDA). This formulation enables us to study complex $4f$ and $5f$ systems. We perform calculations of praseodymium…

Strongly Correlated Electrons · Physics 2015-05-11 Nicola Lanatà , Yongxin Yao , Cai-Zhuang Wang , Kai-Ming Ho , Gabriel Kotliar

The full potential all electron linearized augmented plane wave plus local orbitals (FP-LAPW + lo) method, as implemented in the suite of software WIEN2K, has been used to systematically investigate the structural, electronic, and magnetic…

Strongly Correlated Electrons · Physics 2015-05-14 Raymond Atta-Fynn , Asok K. Ray
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