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We study the adsorption of polymer chains on a fluctuating surface. Physical examples are provided by polymer adsorption at the rough interface between two non-miscible liquids, or on a membrane. In a mean-field approach, we find that the…

Condensed Matter · Physics 2009-10-22 T. Garel , Mehran Kardar , H. Orland

The phase behavior of fluids near weakly attractive substrates is studied by computer simulations of the coexistence curve of a Lennard-Jones (LJ) fluid confined in a slitlike pore. The temperature dependence of the density profiles of the…

Statistical Mechanics · Physics 2009-11-10 I. Brovchenko , A. Geiger , A. Oleinikova

The effect of the surface coupling $J_s$ on the dependency of the layering transition temperature $T_L$ as a function of the thickness $N$, of a spin-1/2 Ising film, is studied using the mean field theory. It is found that for $J_s$ greater…

Soft Condensed Matter · Physics 2009-11-07 L. Bahmad , A. Benyoussef , H. Ez-Zahraouy

A monte carlo density functional theory is developed for chain molecules which both intra and intermolecularly associate. The approach can be applied over a range of chain lengths. The theory is validated for the case of an associating…

Soft Condensed Matter · Physics 2013-08-30 B. D. Marshall , A. J. Garcia-Cuellar , W. G. Chapman

We study the vicinal surface with adsorption below the roughening temperature, using the restricted solid-on-solid model coupled with the Ising model. By the product-wavefunction renormalization group method, we calculate the surface…

Statistical Mechanics · Physics 2009-10-31 Noriko Akutsu , Yasuhiro Akutsu , Takao Yamamoto

The rational function approximation method, density functional theory, and NVT Monte Carlo simulation are used to obtain the density profiles of multicomponent hard-sphere mixtures near a planar hard wall. Binary mixtures with a size ratio…

Statistical Mechanics · Physics 2007-06-06 Alexandr Malijevsky , Santos B. Yuste , Andres Santos , Mariano Lopez de Haro

This study explores atomic and molecular adsorption on a number of early transition-metal carbides (TMC's) by means of density-functional theory calculations. Trend studies are conducted with respect to both period and group in the periodic…

Materials Science · Physics 2012-05-14 Aleksandra Vojvodic , Carlo Ruberto , Bengt I. Lundqvist

In this paper we present the molecular theory of viscosity of confined fluids in small or nano systems. This theory is also applicable to the interfacial viscosity. The basis of this research work is the Enskog kinetic theory and the…

Statistical Mechanics · Physics 2008-06-16 B. Mirzayi , G. A. Mansoori , M. Vafaie-Sefti

The evaporation of a tiny amount of water on the solid surface with different wettability has been studied by molecular dynamics simulations. We found that, as the surface changed from hydrophobicity to hydrophility, the evaporation speed…

Soft Condensed Matter · Physics 2012-03-09 Shen Wang , Yusong Tu , Rongzheng Wan , Haiping Fang

We present a numerical study of the structural correlations associated to gas adsorption/desorption in silica aerogels in order to provide a theoretical interpretation of scattering experiments. Following our earlier work, we use a…

Disordered Systems and Neural Networks · Physics 2016-08-31 F. Detcheverry , E. Kierlik , M. L. Rosinberg , G. Tarjus

The adsorption of a bottle-brush polymer end-grafted with one chain end of its backbone to a flat substrate surface is studied by Monte Carlo simulation of a coarse-grained model, that previously has been characterized in the bulk, assuming…

Soft Condensed Matter · Physics 2010-10-13 Hsiao-Ping Hsu , Wolfgang Paul , Kurt Binder

We examine the reversible adsorption of hard spheres on a random site surface in which the adsorption sites are uniformly and randomly distributed on a plane. Each site can be occupied by one solute provided that the nearest occupied site…

Statistical Mechanics · Physics 2015-06-25 C. Oleyar , J. Talbot

The surface phase behavior of binary mixtures of colloidal hard rods in contact with a solid substrate (hard wall) is studied, with special emphasis on the region of the phase diagram that includes the smectic A phase. The colloidal rods…

Soft Condensed Matter · Physics 2010-12-17 Daniel de las Heras , Yuri Martínez-Ratón , Enrique Velasco

We have used the density-functional theory to locate the freezing transitions and calculate the values of freezing parameters for a system of long elongated molecules which interact via the Gay-Berne pair potential. The pair correlation…

Statistical Mechanics · Physics 2007-05-23 Pankaj Mishra , Jokhan Ram , Yashwant Singh

The interfacial tension between immiscible liquids is studied as a function of a model linear surfactant length and concentration using coarse grained, dissipative particle dynamics numerical simulations. The adsorption isotherms obtained…

Density functional theory for a simple model of dendrimers is proposed. The theory is based on fundamental measure theory which accounts for the hard-sphere repulsion of the segments and on the Wertheim first-order perturbation theory for…

Soft Condensed Matter · Physics 2012-11-12 Alexandr Malijevsky

The dynamics and rheology of a vesicle confined in a channel under shear flow are studied at finite temperature. The effect of finite temperature on vesicle motion and system viscosity is investigated. A two-dimensional numerical model,…

Soft Condensed Matter · Physics 2022-10-04 A. Lamura

The density linear response function for an inhomogeneous system of electrons in equilibrium with an array of fixed ions is considered. Two routes to its evaluation for extreme conditions (e.g., warm dense matter) are considered. The first…

Statistical Mechanics · Physics 2018-09-12 James Dufty , Kai Luo , S. B. Trickey

The formation of an adatom adsorption structure in dynamic force microscopy experiment is shown as a result of the spontaneous appearance of shear strain caused by external supercritical heating. This transition is described by the…

Materials Science · Physics 2014-10-23 Alexei V. Khomenko

We investigate the behavior of a patchy particle model close to a hard-wall via Monte Carlo simulation and density functional theory (DFT). Two DFT approaches, based on the homogeneous and inhomogeneous versions of Wertheim's first order…