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Polar perovskite oxide surfaces are subject to structural reconstruction as a possible stabilisation mechanisms, which changes the surface structure and hence the surface chemistry. To investigate this effect, we study the oxygen evolution…

Materials Science · Physics 2019-04-08 Hassan Ouhbi , Ulrich Aschauer

Combining high-resolution core-level spectroscopy (HRCLS), scanning tunneling microscopy (STM) and density-functional theory (DFT) calculations we reanalyze the Pd(100)-(SQRT(5) x SQRT(5) R27^o)-O surface oxide phase. We find that the…

Soft X-ray resonant scattering studies at the Mn $L_{\texttt{II, III}}$- and the La $M_{\texttt{IV, V}}$- edges of single-crystal LaSr$_2$Mn$_2$O$_7$ are reported. At low temperatures, below $T_\texttt{N} \approx 160$ K, energy scans with a…

Strongly Correlated Electrons · Physics 2014-07-08 H. -F. Li , Y. Su , Tapan Chatterji , A. Nefedov , J. Persson , P. Meuffels , Y. Xiao , Th. Brückel

Kinetics of silicon dry oxidation are investigated theoretically and experimentally at low temperature in the nanometer range where the limits of the Deal and Grove model becomes critical. Based on a fine control of the oxidation process…

Materials Science · Physics 2012-10-08 Christophe Krzeminski , Guilhem Larrieu , Julien Penaud , Evelyne Lampin , Emmanuel Dubois

Using density-functional theory we assess the stability of bulk and surface oxides of the late 4d transition metals in a ``constrained equilibrium'' with a gas phase formed of O2 and CO. While the stability range of the most stable bulk…

Materials Science · Physics 2009-11-10 Karsten Reuter , Matthias Scheffler

Surface enhanced Raman scattering (SERS) effects on tin dioxide in the form of bulk material, nanostructured thin films and colloidal solutions were investigated. Raman spectra are characterized by the three Raman scattering peaks at 478,…

Materials Science · Physics 2015-06-03 Enza Fazio , Fortunato Neri , Salvatore Savasta , Salvatore Spadaro , Sebastiano Trusso

The response of Newtonian liquids to small perturbations is usually considered to be fully described by homogeneous transport coefficients like shear and dilatational viscosity. However, the presence of strong density gradients at the…

Soft Condensed Matter · Physics 2023-03-29 Paolo Malgaretti , Ubaldo Bafile , Renzo Vallauri , Pál Jedlovszky , Marcello Sega

The oxygen evolution reaction (OER) plays an important role in evaluating a photocatalyst and to understand its surface chemistry. In this work we present a comparative study of the OER on the oxide NaTaO$_3$ (113) surface and the…

Materials Science · Physics 2018-10-17 Hassan Ouhbi , Ulrich Aschauer

Understanding the wetting properties of premelting films requires knowledge of the film's equation of state, which is not usually available. Here we calculate the disjoining pressure curve of premelting films, and perform a detailed…

Soft Condensed Matter · Physics 2020-09-09 Pablo Llombart , Eva G. Noya , David N. Sibley , Andrew J. Archer , Luis G. MacDowell

Post deposition variation in film resistance of Sb2Te3 films deposited on glass substrates at room temperature and an elevated temperature (110oC) are investigated. The resistance of films grown at room temperature shows a non-linear…

Condensed Matter · Physics 2009-11-10 P. Arun , Pankaj Tyagi , A. G. Vedeshwar , Vinod Kumar Paliwal

Emergent behavior at complex oxide interfaces has driven much of the research in the oxide thin film community for the past twenty years. Interfaces have been engineered for potential applications in spintronics, topological quantum…

Materials Science · Physics 2021-07-06 Suresh Thapa , Rajendra Paudel , Miles D. Blanchet , Patrick T. Gemperline , Ryan B. Comes

The possible importance of oxide formation for the catalytic activity of transition metals in heterogenous oxidation catalysis has evoked a lively discussion over the recent years. On the more noble transition metals (like Pd, Pt or Ag) the…

Materials Science · Physics 2009-11-13 Jutta Rogal , Karsten Reuter , Matthias Scheffler

Understanding how protective oxide scales evolve over time is necessary for improving the long term resistance of superalloys. This work investigates the time-dependent oxidation behavior of an ingot-processable Co/Ni-based superalloy…

The efficacy of oxygen (O) surface terminations on diamond is an important factor for the performance and stability for diamond-based quantum sensors and electronics. Given the wide breadth of O-termination techniques, it can be difficult…

Complex oxide functionality, such as ferroelectricity, magnetism or superconductivity is often achieved in epitaxial thin-film geometries. Oxygen vacancies tend to be the dominant type of defect in these materials but a fundamental…

Materials Science · Physics 2022-02-23 Moloud Kaviani , Ulrich Aschauer

We report an experimental and theoretical analysis of the sqrt(3)x sqrt(3)-R30 and 2x2 reconstructions on the NiO (111) surface combining transmission electron microscopy, x-ray photoelectron spectroscopy, and reasonably accurate density…

Materials Science · Physics 2015-05-13 J. Ciston , A. Subramanian , D. M. Kienzle , L. D. Marks

The surface structure of SrTiO3(001) thin films homoepitaxially grown by PLD in step-flow mode was characterized using low temperature STM. It was found that one-dimensional (1D) TiOx-based nanostructures were formed on the thin film…

Materials Science · Physics 2015-05-18 Katsuya Iwaya , Takeo Ohsawa , Ryota Shimizu , Tomihiro Hashizume , Taro Hitosugi

The measurement of the lattice-parameter of silicon by x-ray interferometry assumes the use of strain-free crystals. This might not be the case because surface relaxation, reconstruction, and oxidation cause strains without the application…

Computational Physics · Physics 2016-11-23 C Melis , S Giordano , L Colombo , G Mana

The process of environmental oxidation is pivotal in determining the physical and chemical properties of two-dimensional (2D) materials. Its impact holds great significance for the practical application of these materials in nanoscale…

Materials Science · Physics 2024-03-20 Soumendra Kumar Das , Lokanath Patra , Prasanjit Samal , Pratap Kumar Sahoo

Degradation of co-evaporated CH3NH3PbI3 thin films was investigated with x-ray photoelectron spectroscopy (XPS) and x-ray diffraction (XRD) as the films were subjected to exposure of oxygen, dry air, ambient, or H2O. The co-evaporated thin…

Materials Science · Physics 2015-06-23 Youzhen Li , Xuemei Xu , Chenggong Wang , Congcong Wang , Fangyan Xie , Yongli Gao
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