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We have used a first-principles-based scheme to compute the temperature-versus-misfit strain ``Pertsev'' phase diagram of ultrathin films of {\sl incipient} ferroelectric KTaO$_3$. Our results suggest that, at variance with the bulk…

Materials Science · Physics 2009-11-13 A. R. Akbarzadeh , L. Bellaiche , Jorge Íñiguez , David Vanderbilt

The phase transition behaviour of PbTiO3 and BaTiO3 under (111) epitaxial strain is investigated using density-functional theory calculations. From tensile strains of +0.015 to compressive strains of -0.015, PbTiO3 undergoes phase…

Materials Science · Physics 2009-11-13 Riku Oja , Karen Johnston , Johannes Frantti , Risto M. Nieminen

The spin states of Co$^{3+}$ ions in perovskite-type LaCoO$_3$, governed by complex interplay between the electron-lattice interactions and the strong electron correlations, still remain controversial due to the lack of experimental…

Strongly Correlated Electrons · Physics 2018-05-23 Y. Yokoyama , Y. Yamasaki , M. Taguchi , Y. Hirata , K. Takubo , J. Miyawaki , Y. Harada , D. Asakura , J. Fujioka , M. Nakamura , H. Daimon , M. Kawasaki , Y. Tokura , H. Wadati

The effect of in-plane strain on the nonlinear dielectric properties of SrTiO3 epitaxial thin films is calculated using density-functional theory within the local-density approximation. Motivated by recent experiments, the structure,…

Materials Science · Physics 2009-11-10 Armin Antons , J. B. Neaton , Karin M. Rabe , David Vanderbilt

We theoretically investigate the influence of internal and external strain on topological phases in (LaNiO$_3$)$_2$/(LaAlO$_3$)$_N$ heterostructures grown along the [111] direction. At the Hartree-Fock level, topological phases originate…

Strongly Correlated Electrons · Physics 2013-10-02 Andreas Rüegg , Chandrima Mitra , Alexander A. Demkov , Gregory A. Fiete

Elemental defects in transition metal oxides is an important and intriguing subject that result in modifications in variety of physical properties including atomic and electronic structure, optical and magnetic properties. Understanding the…

Understanding new superconductors requires high-quality epitaxial thin films to explore intrinsic electromagnetic properties, control grain boundaries and strain effects, and evaluate device applications. So far superconducting properties…

Many dipolar topological structures have been experimentally demonstrated in (PbTiO$_3$)$_n$/(SrTiO$_3$)$_n$ superlattices, such as flux-closure, vortice, and skyrmion. In this work, we employ deep potential molecular dynamics (MD) to…

Materials Science · Physics 2025-01-07 Jiyuan Yang , Shi Liu

High quality stoichiometric magnetite (Fe3O4) films grown by infrared pulsed laser deposition (IR-PLD) on different surfaces were investigated in order to study the influence of the substrate, orientation, and thickness on their magnetic…

We study cubic ferroelectrics films that become uniaxial with a polar axis perpendicular to the film because of a misfit strain due to a substrate. The main present result is the analytical account for the elastic anisotropy as well as the…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 A. M. Bratkovsky , A. P. Levanyuk

Materials with strong electronic correlations host remarkable -- and technologically relevant -- phenomena such as magnetism, superconductivity and metal-insulator transitions. Harnessing and controlling these effects is a major challenge,…

Recent works have shown that the domain walls of room-temperature multiferroic BiFeO3 (BFO) thin films can display distinct and promising functionalities. It is thus important to understand the mechanisms underlying domain formation in…

Materials Science · Physics 2015-05-14 C. J. M. Daumont , S. Farokhipoor , A. Ferri , J. C. Wojdel , Jorge Iniguez , B. J. Kooi , B. Noheda

SrVO3 thin films with a high figure of merit for applications as transparent conductors were crystallized from amorphous layers using solid phase epitaxy (SPE). Epitaxial SrVO3 films crystallized on SrTiO3 using SPE exhibit a room…

A Landau-Ginsburg-Devonshire-type nonlinear phenomenological theory is presented, which enables the thermodynamic description of dense laminar polydomain states in epitaxial ferroelectric thin films. The theory explicitly takes into account…

Materials Science · Physics 2007-05-23 V. G. Koukhar , N. A. Pertsev , R. Waser

We present the first analytical study of phase transitions in ferroelastic-ferroelectric epitaxial thin films on exactly solvable model. The emerging domain structure with domains of equal width (which may be exponentially large on a "soft"…

Statistical Mechanics · Physics 2009-10-31 A. M. Bratkovsky , A. P. Levanyuk

Using first principles calculations, we determined the epitaxial-strain dependence of the ground state of the 1:1 SrCrO$_3$/SrTiO$_3$ superlattice. The superlattice layering leads to significant changes in the electronic states near the…

Materials Science · Physics 2015-09-16 Yuanjun Zhou , Karin M. Rabe

We present angle-resolved photoemission spectroscopy results for thin films of the three-dimensional manganese perovskite La$_{1-x}$Sr$_{x}$MnO$_{3}$. We show that the transition temperature ($T_c$) from the paramagnetic insulating to…

Strongly Correlated Electrons · Physics 2008-04-23 M. Shi , M. C. Falub , P. R. Willmott , J. Krempasky , R. Herger , L. Patthey , K. Hricovini , C. Falub , M. Schneider

We report the temperature dependent capacitance-voltage characteristics of Pt/SrTiO3 Schottky diodes fabricated using compressively strained SrTiO3 thin films grown on (LaAlO3)0.3(Sr2AlTaO6)0.7 (LSAT) substrates. The measurements reveal a…

Materials Science · Physics 2015-11-10 Amit Verma , Santosh Raghavan , Susanne Stemmer , Debdeep Jena

We report the characterization of the crystal structure, low-temperature charge and orbital ordering, transport, and magnetization of Pr_{0.6}Ca_{0.4}MnO_{3} films grown on LaAlO_{3}, NdGaO_{3}, and SrTiO_{3} substrates, which provide…

With recent advances in strain engineering and its widespread applications, it is becoming increasingly important to understand the effect of biaxial strain on the most common structural phase of perovskites -- the orthorhombic $Pnma$…

Materials Science · Physics 2023-11-23 Amartyajyoti Saha , Turan Birol