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Related papers: Anomalous layering at the liquid Sn surface

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Over the past two decades synchrotron facilities dedicated to the generation of x-rays for study of atoms, molecules and condensed matter have proliferated all over the world. As a result of the special properties of x-rays produced by…

Statistical Mechanics · Physics 2009-09-29 Oleg G. Shpyrko

X-ray reflectivity studies reveal atomic-level surface-segregation at the free surface of the eutectic Au71Sn29 liquid alloy. The surface-segregation extends up to three layers, in which the top layer is almost a pure monolayer of Sn, the…

We present x-ray reflectivity and diffuse scattering measurements from the liquid surface of pure potassium. They strongly suggest the existence of atomic layering at the free surface of a pure liquid metal with low surface tension. Prior…

Statistical Mechanics · Physics 2007-05-23 Oleg Shpyrko , Patrick Huber , Peter S. Pershan , Holger Tostmann , Alexei Grigoriev , Ben Ocko , Moshe Deutsch

We present the first resonant x-ray reflectivity measurements from a liquid surface. The surface structure of the liquid Hg-Au alloy system just beyond the solubility limit of 0.14at% Au in Hg had previously been shown to exhibit a unique…

Oscillatory density profiles (layers) have previously been observed at the free surfaces of liquid metals, but not in other isotropic liquids. We have used x-ray reflectivity to study a molecular liquid, tetrakis(2-ethylhexoxy)silane. When…

Soft Condensed Matter · Physics 2007-05-23 Haiding Mo , Guennadi Evmenenko , Sumit Kewalramani , Kyungil Kim , Steven N. Ehrlich , Pulak Dutta

Recent measurements show that the free surfaces of liquid metals and alloys are always layered, regardless of composition and surface tension; a result supported by three decades of simulations and theory. Recent theoretical work claims,…

Soft Condensed Matter · Physics 2007-05-23 Oleg Shpyrko , Masafumi Fukuto , Peter Pershan , Ben Ocko , Ivan Kuzmenko , Thomas Gog , Moshe Deutsch

We report x-ray reflectivity (XR) and small angle off-specular diffuse scattering (DS) measurements from the surface of liquid Indium close to its melting point of $156^\circ$C. From the XR measurements we extract the surface structure…

Materials Science · Physics 2009-11-10 Holger Tostmann , Oleg Shpyrko , Peter S. Pershan , Elaine Dimasi , Ben Ocko , Moshe Deutsch

Measurements of the surface x-ray scattering from several pure liquid metals (Hg, Ga, and In) and from three alloys (Ga-Bi, Bi-In, and K-Na) with different heteroatomic chemical interactions in the bulk phase are reviewed. Surface-induced…

Soft Condensed Matter · Physics 2007-05-23 Elaine DiMasi , Holger Tostmann , Oleg G. Shpyrko , Peter S. Pershan , Benjamin M. Ocko , Moshe Deutsch

The authors study theoretically reflection on the surface of a metamaterial with a hyperbolic dispersion. It is found that reflection is strongly dependent on how the surface is terminated with respect to the asymptote of the hyperbolic…

Optics · Physics 2008-11-10 Xin Li , Zixian Liang , Xiaohan Liu , Xunya Jiang , Jian Zi

We report and discuss the first neutron reflection measurements from the free surface of normal and superfluid 4He and of liquid 3He-4He mixture. In case of liquid 4He the surface roughness is different above and below the lambda…

Other Condensed Matter · Physics 2008-11-20 T. R. Charlton , R. M. Dalgliesh , A. Ganshin , O. Kirichek , S. Langridge , P. V. E. McClintock

The reflection of neutrons from a helium surface has been observed for the first time. The 4He surface is smoother in the superfluid state at 1.54 K than in the case of the normal liquid at 2.3 K. In the superfluid state we also observe a…

Soft Condensed Matter · Physics 2007-12-06 T. R. Charlton , R. M. Dalgliesh , A. Ganshin , O. Kirichek , S. Langridge , P. V. E. McClintock

We report the results of an x-ray scattering study that reveals oxidation kinetics and formation of a previously unreported crystalline phase of SnO at the liquid-vapour interface of Sn. Our experiments reveal that the pure liquid Sn…

We simulate the liquid silicon surface with first-principles molecular dynamics in a slab geometry. We find that the atom-density profile presents a pronounced layering, similar to those observed in low-temperature liquid metals like Ga and…

Soft Condensed Matter · Physics 2009-10-31 G. Fabricius , E. Artacho , D. Sanchez-Portal , P. Ordejon , D. A. Drabold , J. M. Soler

Accumulation layers with very large concentrations of electrons where many subbands are filled became recently available due to ionic liquid and other new methods of gating. The low temperature mobility in such layers is limited by the…

Mesoscale and Nanoscale Physics · Physics 2016-07-08 Han Fu , K. V. Reich , B. I. Shklovskii

The specular reflectivity of slow, metastable neon atoms from a silicon surface was found to increase markedly when the flat surface was replaced by a grating structure with parallel narrow ridges. For a surface with ridges that have a…

Atomic Physics · Physics 2015-05-11 Fujio Shimizu , Jun-ichi Fujita

We propose that extended orientational correlations can appear at the surface of supercooled heavy noble liquid metals, due to the same compressive forces that cause reconstruction of their crystal surfaces. Simulations for liquid Au show a…

Materials Science · Physics 2009-10-30 Franck Celestini , Furio Ercolessi , Erio Tosatti

Second harmonic generation (SHG) spectroscopy has been applied to probe the fused silica/water interface at pH 7 and the uncharged 11bar02 sapphire/water interface at pH 5.2 in contact with aqueous solutions of NaCl, NaBr, NaI, KCl, RbCl,…

Materials Science · Physics 2018-03-28 Mavis D. Boamah , Paul E. Ohno , Franz M. Geiger , Kenneth B. Eisenthal

We investigate theoretically the optical response of bulk samples and thin films of the MAX phases materials, accounting for their large electrical anisotropy. We reveal the unusual behaviour of the reflection and transmittion spectra as a…

Materials Science · Physics 2011-10-14 O. Kyriienko , I. A. Shelykh

Electrons can be reflected at an interface between two metals because of a dielectric barrier or different properties of the Fermi surface. Andreev reflection allows to directly measure normal reflection when one of the metals is a…

Mesoscale and Nanoscale Physics · Physics 2015-05-30 Elina Tuuli , Kurt Gloos

The structure of the adsorbed layer of alkali ions on the surface of colloidal silica solutions with a particle size of ~27 nm has been studied by reflectometry and diffuse scattering of synchrotron radiation with a photon energy of about…

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