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Precise magnetic hysteresis measurements of small single crystals of Mn$_{12}$ acetate of spin 10 have been conducted down to 0.4 K using a high sensitivity Hall magnetometer. At higher temperature (>1.6K) step-like changes in magnetization…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Andrew D. Kent , Yicheng Zhong , Louisa Bokacheva , Daniel Ruiz , David N. Hendrickson , M. P. Sarachik

Thin films of the Single Molecule Magnet (Mn12-acetate) have been fabricated on a Si-substrate by the Dip-and-Dry method, a simple and robust technique. Atomic force microscopy and X-ray photoelectron spectroscopy characterizations reveal…

Other Condensed Matter · Physics 2009-11-11 D. M. Seo , V. Meenakshi , W. Teizer , H. Zhao , K. R. Dunbar

We used a Josephson junction as a radiation detector to look for evidence of the emission of electromagnetic radiation during magnetization avalanches in a crystal assembly of Mn_12-Acetate. The crystal assembly exhibits avalanches at…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 M. Bal , Jonathan R. Friedman , K. Mertes , W. Chen , E. M. Rumberger , D. N. Hendrickson , N. Avraham , Y. Myasoedov , H. Shtrikman , E. Zeldov

The magnetization of the prototypical molecular magnet Mn12-acetate exhibits a series of sharp steps at low temperatures due to quantum tunneling at specific resonant values of magnetic field applied along the easy c-axis. An abrupt…

Mesoscale and Nanoscale Physics · Physics 2010-01-21 M. P. Sarachik , S. McHugh

Microwave radiation applied to single-molecule magnets can induce large magnetization changes when the radiation is resonant with transitions between spin levels. These changes are interpreted as due to resonant heating of the sample by the…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 M. Bal , Jonathan R. Friedman , E. M. Rumberger , S. Shah , D. N. Hendrickson , N. Avraham , Y. Myasoedov , H. Shtrikman , E. Zeldov

Thin films of the molecular magnet Mn12-acetate, [Mn12 O12(CH3COO)16 (H2O)4] 2CH3COOH 4H2O, have been prepared using a laser ablation technique with a nitrogen laser at low laser energies of 0.8 and 2 mJ. Chemical and magnetic…

Electromagnetic radiation produced by avalanches in the magnetization reversal of Mn12-Acetate has been measured. Short bursts of radiation have been detected, with intensity significantly exceeding the intensity of the black-body radiation…

Materials Science · Physics 2009-11-10 J. Tejada , E. M. Chudnovsky , J. M. Hernandez , R. Amigo

We report the far-infrared spectra of the molecular nanomagnet Mn_12-acetate (Mn_12) as a function of temperature (5-300 K) and magnetic field (0-17 T). The large number of observed vibrational modes is related to the low symmetry of the…

Strongly Correlated Electrons · Physics 2009-11-07 A. B. Sushkov , B. R. Jones , J. L. Musfeldt , Y. J. Wang , R. M. Achey , N. S. Dalal

Using micron-sized thermometers and Hall bars, we report time-resolved studies of the local temperature and local magnetization for two types of magnetic avalanches (abrupt spin reversals) in the molecular magneti Mn12-acetate,…

Materials Science · Physics 2009-04-27 S. McHugh , R. Jaafar , M. P. Sarachik , Y. Myasoedov , A. Finkler , E. Zeldov , R. Bagai , G. Christou

Resonant microwave radiation applied to a single crystal of the molecular magnet Fe_8 induces dramatic changes in the sample's magnetization. Transitions between excited states are found even though at the nominal system temperature these…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 M. Bal , Jonathan R. Friedman , Y. Suzuki , E. M. Rumberger , D. N. Hendrickson , N. Avraham , Y. Myasoedov , H. Shtrikman , E. Zeldov

Films of the molecular nanomagnet, Mn12-acetate, have been deposited using pulsed laser deposition and a novel variant, matrix assisted pulsed laser evaporation. The films have been characterized by X-ray photoelectron spectroscopy, mass…

Materials Science · Physics 2009-11-10 V. Meenakshi , W. Teizer , D. G. Naugle , H. Zhao , K. R. Dunbar

The magnetocaloric effect (MCE) in the A-site ordered manganite NdBaMn2O6 is studied. The MCE in this compound has an anomalous behavior. In low magnetic fields, the abrupt transitions between direct and inverse magnetocaloric effect are…

Materials Science · Physics 2012-02-20 A. M. Aliev , A. G. Gamzatov , V. S. Kalitka , A. R. Kaul

We use neutron diffraction to probe the magnetization components of a crystal of Mn12 single-molecule magnets. Each of these molecules behaves, at low temperatures, as a nanomagnet with spin S = 10 and strong anisotropy along the…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 F. Luis , J. Campo , J. Gomez , G. J. McIntyre , J. Luzon , D. Ruiz-Molina

The magnetocaloric effect (MCE) in paramagnetic materials has been widely used for attaining very low temperatures by applying a magnetic field isothermally and removing it adiabatically. The effect can be exploited also for room…

We report on the anomalous magnetization reversal under hydrostatic pressure in the lightly electron-doped manganite compound (Ca$_{1-x}$Sr$_{x}$)Mn$_{0.95}$Sb$_{0.05}$O$_{3}$ with its fixed carrier content. In a weakly magnetic field…

We report measurements on magnetization reversal in the Fe$_8$ molecular magnet using fast pulsed magnetic fields of 1.5 kT/s and in the temperature range of 0.6-4.1 K. We observe and analyze the temperature dependence of the reversal…

Mesoscale and Nanoscale Physics · Physics 2014-09-11 S. N. Jammalamadaka , J. Vanacken , V. V. Moshchalkov , Saül Vélez , J. Tejada , Ferran Macià

The longitudinal magnetic susceptibility of single crystals of the molecular magnet Mn$_{12}$-acetate obeys a Curie-Weiss law, indicating a transition to a ferromagnetic phase due to dipolar interactions. With increasing magnetic field…

Mesoscale and Nanoscale Physics · Physics 2010-09-02 Bo Wen , P. Subedi , Lin Bo , Y. Yeshurun , M. P. Sarachik , A. D. Kent , C. Lampropoulos , G. Christou

35 years after its synthesis magnetic observables are calculated for the first time for the molecular nanomagnet Mn12-acetate using a spin-Hamiltonian that contains all spins. Starting from a very advanced DFT parameterization [Phys. Rev. B…

Strongly Correlated Electrons · Physics 2015-08-31 O. Hanebaum , J. Schnack

The local magnetic field distribution on the subsurface of a single-molecule magnet crystal, SMM, above blocking temperature (T >> Tb) detected for a very short time interval (~ 10-10 s), has been investigated. Electron Paramagnetic…

Materials Science · Physics 2012-02-17 Dijana Zilic , Boris Rakvin , Naresh S. Dalal

High quality epitaxial thin films of Gd0.67Ca0.33MnO3 have been deposited onto (100) SrTiO3 substrates by pulsed-laser deposition. Enhanced properties in comparison with bulk samples were observed. The magnetic transition temperature (Tc)…

Strongly Correlated Electrons · Physics 2009-11-11 Yanwei MA , M. Guilloux-Viry , P. Barahona , O. Pena , C. Moure
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